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At partial fillings of its flat electronic bands, magic-angle twisted bilayer graphene (MATBG) hosts a rich variety of competing correlated phases that show sample-to-sample variations. Divergent phase diagrams in MATBG are often attributed to the sublattice polarization energy scale, tuned by the degree of alignment of the hexagonal boron nitride (hBN) substrates typically used in van der Waals devices. Unaligned MATBG exhibits unconventional superconductor and correlated insulator phases, while nearly perfectly aligned MATBG/hBN exhibits zero-field Chern insulating phases and lacks superconductivity. Here we use scanning tunneling microscopy and spectroscopy (STM/STS) to observe gapped phases at partial fillings of the flat bands of MATBG in a new intermediate regime of sublattice polarization, observed when MATBG is only partially aligned (θGr-hBN ≈ 1.65°) to the underlying hBN substrate. Under this condition, MATBG hosts not only phenomena that naturally interpolate between the two sublattice potential limits, but also unexpected gapped phases absent in either of these limits. At charge neutrality, we observe an insulating phase with a small energy gap (Δ < 5 meV) likely related to weak sublattice symmetry breaking from the hBN substrate. In addition, we observe new gapped phases near fractional fillings ν = ±1/3 and ν = ±1/6, which have not been previously observed in MATBG. Importantly, energy-resolved STS unambiguously identifies these fractional filling states to be of single-particle origin, possibly a result of the super-superlattice formed by two moiré superlattices. Our observations emphasize the power of STS in distinguishing single-particle gapped phases from many-body gapped phases in situations that could be easily confused in electrical transport measurements, and demonstrate the use of substrate engineering for modifying the electronic structure of a moiré flat-band material.
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Fractionalization as an alternate to charge ordering in electronic insulators
Incompressible insulating phases of electronic systems at partial filling of a lattice are often associated with charge ordering that breaks lattice symmetry. The resulting phases have an enlarged unit cell with an effective integer filling. Here we explore the possibility of insulating states—which we dub “quantum charge liquids” (QCLs)—at partial lattice filling that preserve lattice translation symmetry. Such QCL phases must necessarily either have gapped fractionally charged excitations and associated topological order or have gapless neutral excitations. We establish some general constraints on gapped fermionic QCL phases that restrict the nature of their topological order. We prove a number of results on the minimal topological order that is consistent with the lattice filling. In particular we show that, at rational fillings 𝜈=𝑝/𝑞 with 𝑞 an even integer, the minimal ground-state degeneracy on a torus of the fermionic QCL is 4𝑞2, four times larger than that of the bosonic QCL at the same filling. We comment on models and physical systems which may host fermionic QCL phases and discuss the phenomenology of these phases.
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- Award ID(s):
- 2206305
- PAR ID:
- 10650593
- Publisher / Repository:
- Physical Review B
- Date Published:
- Journal Name:
- Physical Review B
- Volume:
- 111
- Issue:
- 23
- ISSN:
- 2469-9950
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
-
Accepted Manuscript
- Journal Article:
- https://doi.org/10.1103/PhysRevB.111.235108
