Ever since the discovery of the charge density wave (CDW) transition in the kagome metal , the nature of its symmetry breaking has been under intense debate. While evidence suggests that the rotational symmetry is already broken at the CDW transition temperature ( ), an additional electronic nematic instability well below has been reported based on the diverging elastoresistivity coefficient in the anisotropic channel ( ). Verifying the existence of a nematic transition below is not only critical for establishing the correct description of the CDW order parameter, but also important for understanding low-temperature superconductivity. Here, we report elastoresistivity measurements of using three different techniques probing both isotropic and anisotropic symmetry channels. Contrary to previous reports, we find the anisotropic elastoresistivity coefficient is temperature independent, except for a step jump at . The absence of nematic fluctuations is further substantiated by measurements of the elastocaloric effect, which show no enhancement associated with nematic susceptibility. On the other hand, the symmetric elastoresistivity coefficient increases below , reaching a peak value of 90 at . Our results strongly indicate that the phase transition at is not nematic in nature and the previously reported diverging elastoresistivity is due to the contamination from the channel. Published by the American Physical Society2024
more »
« less
This content will become publicly available on January 1, 2027
Lattice-Charge Coupling in a Trilayer Nickelate with Intertwined Density Wave Order
Intertwined charge and spin correlations are ubiquitous in a wide range of transition metal oxides and are often perceived as intimately related to unconventional superconductivity. Theoretically envisioned as driven by strong electronic correlations, the intertwined order is usually found to be strongly coupled to the lattice as signaled by pronounced phonon softening. Recently, both charge and spin density waves (CDW and SDW) and superconductivity have been discovered in several Ruddlesden-Popper (RP) nickelates, in particular trilayer nickelates ( , La). The nature of the intertwined order and the role of lattice-charge coupling are at the heart of the debate about these materials. Using inelastic x-ray scattering, we mapped the low-energy phonon dispersions in and found no evidence of softening near the CDW wave vector over a wide temperature range, which contrasts with the pronounced anomalies frequently observed in cuprate superconductors. Calculations of the electronic susceptibility revealed a peak at the observed SDW ordering vector but not at the CDW wave vector. Our experimental and theoretical findings highlight the crucial role of the spin degree of freedom and establish a foundation for understanding the interplay between superconductivity and density-wave transitions in RP nickelate superconductors and beyond.
more »
« less
- Award ID(s):
- 2045826
- PAR ID:
- 10661017
- Publisher / Repository:
- APS
- Date Published:
- Journal Name:
- Physical Review X
- Volume:
- 16
- ISSN:
- 2160-3308
- Page Range / eLocation ID:
- 011013
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
The Hubbard and closely relatedt-Jmodels are exciting platforms for unconventional superconductivity (SC). Through state-of-the-art density matrix renormalization group calculations using the grand canonical ensemble, we address open issues regarding the ground-state phase diagram of the extendedt-Jmodel on a square lattice in the parameter regime relevant to cuprate superconductors. On large 8-leg cylinders, we demonstrate that the puret-Jmodel with only nearest-neighbor hoppings and superexchange interactions, for a wide range of doping ( ), hosts robust d-wave superconductivity possibly coexisting with weak unidirectional pair density wave. Furthermore, a small next nearest neighbor hopping suppresses pair and charge density waves, resulting in a uniform d-wave SC phase in both electron- and hole-doped cuprate model systems. Our work validates thet-Jmodel as a proper minimum model for the emergence of superconductivity in cuprate superconductors.more » « less
-
Spin-forbidden ( ) multiplet excitations and their coupling to magnetic properties are of increasing importance for magneto-optical studies of correlated materials. Nonetheless, the mechanisms for optically brightening these transitions and their generality remain poorly understood. Here, we report magnetic circular dichroism (MCD) spectroscopy on the van der Waals ferromagnet (FM) . Previously unreported spin-forbidden ( ) excitations are observed near the ligand-to-metal charge-transfer excitation threshold. The assignment of these excitations and their multiplet character is established through complementary Cr -edge resonant inelastic x-ray scattering measurements along with charge-transfer multiplet calculations and chemical trends in the chromium trihalide series ( , Cl, Br, I). We utilize the high sensitivity of MCD spectroscopy to study the thickness-dependent optical response. The spin-forbidden excitations remain robust down to the monolayer limit, and we observe a significant magnetic-field dependence of the MCD spectrum across the antiferromagnetic-to-FM transition in few-layer samples. We preliminarily attribute this behavior to changes in the metal-ligand covalency with magnetic state. Our results clarify the magneto-optical response of and identify covalency as a central mechanism for the brightening and field tunability of spin-forbidden multiplet excitations.more » « less
-
We explore leptogenesis during a cosmological epoch during which the electroweak force is confined. During weak confinement, there is only one conserved nonanomalous global charge, , which is a linear combination of lepton-number, baryon-number, and hypercharge. The inclusion of heavy Majorana neutrinos leads to an -charge and -violating interaction with a composite scalar, , and composite fermions, , allowing for the generation of an -charge asymmetry, which translates into a baryon asymmetry post deconfinement. Determining the resulting baryon asymmetry as a function of the model parameters, we find that the predicted baryon-asymmetry can match observations for a wide swath of parameter space: a weak confinement scale , the sum of the Standard Model Yukawa couplings , , and a coupling with complex phase . While leptogenesis under the assumption of a standard cosmology relies on the complex phase of the neutrino Yukawa couplings, the asymmetry generated in this novel background cosmology primarily depends on a strong phase from confinement, , and favors negligible -violation in the right-handed neutrino decays.more » « less
-
Beginning with high- cuprate materials, it has been observed that many superconductors exhibit so-called “Homes scaling,” in which the zero-temperature superfluid density is proportional to the product of the normal-state dc conductivity and the superconducting transition temperature . For conventional, -wave superconductors, such scaling has been shown to be a natural consequence of elastic-scattering disorder, not only in the extreme dirty limit, but across a broad range of scattering parameters. Here we show that when an analogous calculation is carried out for elastic scattering in -wave superconductors, a stark contrast emerges, with in the dirty limit, in apparent violation of Homes scaling. Within a simple approximate Migdal-Eliashberg treatment of inelastic scattering, we show how the observed Homes scaling is recovered. The normal-state behavior of near-optimally-doped cuprates is dominated by inelastic scattering, but significant deviations from Homes scaling occur for disorder-dominated cuprate systems, such as underdoped and overdoped , and in very clean materials with little inelastic scattering, such as . We present a revised analysis where both axes of the original Homes scaling plot are normalized by the Drude plasma weight and show that a new universal scaling emerges, in which the superfluid fractions of dirty -wave and dirty -wave superconductors coalesce to a single point at which normal-state scattering is occurring at the Planckian bound. The combined result is a new tool for classifying superconductors in terms of order parameter symmetry, as well as scattering strength and character. Although our model starts from a Fermi-liquid assumption, it describes underdoped cuprates surprisingly well.more » « less
An official website of the United States government
