Abstract The intrinsic magnetic topological insulator, Mn(Bi1−xSbx)2Te4, has been identified as a Weyl semimetal with a single pair of Weyl nodes in its spin-aligned strong-field configuration. A direct consequence of the Weyl state is the layer dependent Chern number,$$C$$ . Previous reports in MnBi2Te4thin films have shown higher$$C$$ states either by increasing the film thickness or controlling the chemical potential. A clear picture of the higher Chern states is still lacking as data interpretation is further complicated by the emergence of surface-band Landau levels under magnetic fields. Here, we report a tunable layer-dependent$$C$$ = 1 state with Sb substitution by performing a detailed analysis of the quantization states in Mn(Bi1−xSbx)2Te4dual-gated devices—consistent with calculations of the bulk Weyl point separation in the doped thin films. The observed Hall quantization plateaus for our thicker Mn(Bi1−xSbx)2Te4films under strong magnetic fields can be interpreted by a theory of surface and bulk spin-polarised Landau level spectra in thin film magnetic topological insulators.
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Magnetodynamics of short nanoparticle chains
In recent years, there has been increasing interest in the understanding and application of nanoparticle assemblies driven by external fields. Although these systems can exhibit marked transitions in behavior compared to non-interacting counterparts, it has often proven challenging to connect their dynamics with underlying physical mechanisms or even to verifiably establish their structure under realistic experimental conditions. We have studied colloidal iron oxide nanoparticles that assemble into ordered, few-particle linear chains under the influence of oscillating and pulsed magnetic fields. In this work, our goal has been to answer the following question: by what physical mechanisms does the magnetic switching of a linear chain evolve from the switching of its constituent particles? Cryo-TEM has been used to flash freeze and image the structures formed by oscillatory drive fields, and magnetic relaxometry has been used to extract the multiple time constants associated with magnetic switching of the short chains. Armed with the physical structure from microscopy and the field-dependent switching times from magnetic measurements, we have conducted extensive micromagnetic simulations, revealing probable physical mechanisms for each time constant regime spanning$$10^{6}$$($$\approx$$1 μs to 1 s) in time. These types of magnetic nanomaterials have great potential for biomedical technologies, particularly magnetic particle imaging and hyperthermia, and rigorous elucidation of their physics will hasten their optimization.
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- Award ID(s):
- 2038046
- PAR ID:
- 10673660
- Publisher / Repository:
- Nature
- Date Published:
- Journal Name:
- Scientific Reports
- Volume:
- 15
- Issue:
- 1
- ISSN:
- 2045-2322
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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