This study presents detailed time-integrated and time-resolved spectral analysis of the Fermi Gamma-ray Burst Monitor observations of the bright GRB 231129C. The results reveal its distinct spectral characteristics, featuring a hard low-energy spectral index (
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Abstract α ) and soft high-energy spectral index (β ), similar to GRB 090902B, suggesting a possible dominance of thermal emission. Further analysis indicates that 92% of the spectral indices exceed the synchrotron “line of death,” with the hardest index atα ∼ +0.44. Simultaneously, 53% of the spectra can be well fitted by the nondissipative photosphere model, supporting a potential origin from a nondissipative photosphere. Additionally, we observe strong correlations between the spectral indexα and peak energyE pwith flux. For theα −F relationship, we employF =F 0e (3.00±0.10)α to describe it, whereas theE p−F relationship requires a smoothly bending power-law function. Based on the framework proposed by Hascoët et al. and Gao & Zhang, the jet characteristics of this burst were studied, revealing that both methods support the suitability of a pure fireball model for this GRB at small initial jet radii.Free, publicly-accessible full text available September 1, 2025 -
Abstract Physical processes behind flow‐topography interactions and turbulent transitions are essential for parameterization in numerical models. We examine how the Kuroshio cascades energy into turbulence upon passing over a seamount, employing a combination of shipboard measurements, tow‐yo microstructure profiling, and high‐resolution mooring. The seamount, spanning 5 km horizontally with two summits, interacts with the Kuroshio, whose flow speed ranges from 1 to 2 m s−1, modulated by tides. The forward energy cascade process is commenced by forming a train of 2–3 nonlinear lee waves behind the summit with a wavelength of 0.5–1 km and an amplitude of 50–100 m. A train of Kelvin‐Helmholtz (KH) billows develops immediately below the lee waves and extends downstream, leading to enhanced turbulence. The turbulent kinetic energy dissipation rate is
O (10−7–10−4) W kg−1, varying in phase with the upstream flow speed modulated by tides. KH billows occur primarily at the lee wave's trailing edge, where the combined strong downstream shear and low‐stratification recirculation trigger the shear instability,Ri < 1/4. The recirculation also creates an overturn susceptible to gravitational instability. This scenario resembles the rotor, commonly found in atmospheric mountain waves but rarely observed in the ocean. A linear stability analysis further suggests that critical levels, where the KH instability extracts energy from the mean flow, are located predominantly at the strong shear layer of the lee wave's upwelling portion, coinciding with the upper boundary of the rotor. These novel observations may provide insights into flow‐topography interactions and improve physics‐based turbulence parameterization.Free, publicly-accessible full text available September 1, 2025 -
Abstract There is no consensus yet on whether the precursor and the main burst of gamma-ray bursts (GRBs) have the same origin, and their jet composition is still unclear. In order to further investigate this issue, we systematically search 21 Fermi GRBs with both a precursor and main burst for spectral analysis. We first perform Bayesian time-resolved spectral analysis and find that almost all the precursors and the main bursts (94.4%) exhibit thermal components and that the vast majority of them have a low-energy spectral index (
α ; 72.2%) that exceeds the limit of synchrotron radiation. We then analyze the evolution and correlation of the spectral parameters and find that approximately half of theα (50%) of the precursors and the main bursts evolve in a similar pattern, while peak energy (E p ; 55.6%) behaves similarly, and their evolution is mainly characterized by flux tracking; for theα −F (the flux) relation, more than half of the precursors and the main bursts (61.1%) exhibit roughly similar patterns; theE p −F relation in both the precursor and main burst (100%) exhibits a positive correlation of at least moderate strength. Next, we constrain the outflow properties of the precursors and the main bursts and find that most of them exhibit typical properties of photosphere radiation. Finally, we compare the time-integrated spectra of the precursors and the main bursts and find that nearly all of them are located in similar regions of the Amati relation and follow the Yonetoku relation. Therefore, we conclude that main bursts are continuations of precursors and may share a common physical origin.Free, publicly-accessible full text available July 1, 2025 -
Broadband frequency comb generation through cascaded quadratic nonlinearity remains experimentally untapped in free-space cavities with bulk χ(2)materials mainly due to the high threshold power and restricted ability of dispersion engineering. Thin-film lithium niobate (LN) is a good platform for nonlinear optics due to the tight mode confinement in a nano-dimensional waveguide, the ease of dispersion engineering, large quadratic nonlinearities, and flexible phase matching via periodic poling. Here we demonstrate broadband frequency comb generation through dispersion engineering in a thin-film LN microresonator. Bandwidths of 150 nm (80 nm) and 25 nm (12 nm) for center wavelengths at 1560 and 780 nm are achieved, respectively, in a cavity-enhanced second-harmonic generation (doubly resonant optical parametric oscillator). Our demonstration paves the way for pure quadratic soliton generation, which is a great complement to dissipative Kerr soliton frequency combs for extended interesting nonlinear applications.
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Free, publicly-accessible full text available January 1, 2025
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ChemPhysChem (Ed.)
Abstract Molecular clusters can function as nanoscale atoms/superatoms, assembling into superatomic solids, a new class of solid‐state materials with designable properties through modifications on superatoms. To explore possibilities on diversifying building blocks, here we thoroughly studied one representative superatom, Co6Se8(PEt3)6. We probed its structural, electronic, and magnetic properties and revealed its detailed electronic structure as valence electrons delocalize over inorganic [Co6Se8] core while ligands function as an insulated shell.59Co SSNMR measurements on the core and31P,13C on the ligands show that the neutral Co6Se8(PEt3)6is diamagnetic and symmetric, with all ligands magnetically equivalent. Quantum computations cross‐validate NMR results and reveal degenerate delocalized HOMO orbitals, indicating aromaticity. Ligand substitution keeps the inorganic core nearly intact. After losing one electron, the unpaired electron in [Co6Se8(PEt3)6]+1is delocalized, causing paramagnetism and a delocalized electron spin. Notably, this feature of electron/spin delocalization over a large cluster is attractive for special single‐electron devices.
Free, publicly-accessible full text available January 15, 2025 -
Transformation of multifunctional materials with control over site-selectivity and chemical diversity remains challenging. Herein, we present a metal-free, one-pot strategy for the defluorophosphorylation of polyfluoroalkyl peroxides that enables expedient construction of structurally diverse phosphoryl-containing heterocyclic libraries. By judicious choice of reaction conditions, C 3,4-diphosphoryl furans and C 4-monophosphoryl furans can be easily accessed. In addition, synthetic derivatization of the obtained organophosphorus heteroarenes to value-added monodentate and bidentate phosphines has been demonstrated. Mechanistic studies revealed that regioselective defluorophosphorylation allows divergent product formation in two reaction modes.more » « less