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ABSTRACT An abundance of CO significantly surpassing the abundance of H2O is observed in the comae of comets at large heliocentric distances. In these environments, CO molecules can be the most abundant species and they may be therefore the dominant projectiles inducing collisional excitation of the cometary molecules. It is thus of high interest to investigate the excitation of CO by CO. This article provides a new set of CO–CO collisional rate coefficients for temperatures up to 150 K and for CO rotational levels j1 up to 10. These data are obtained from quantum scattering calculations using the coupled states approximation. They are used in a simple radiative transfer model in order to test their impact on the excitation of cometary CO. Because mutual (de-)excitations of the target and projectile are important, the CO projectile was assumed to be thermalized at the kinetic temperature. We found that the non-local thermodynamical equilibrium regime extends for CO densities in the range 103–107 cm−3. We also observed that as soon as the CO/H2O ratio is larger than 70 per cent/30 per cent, the contribution of H2O collisions can be neglected. Similarly, the excitation of CO by CO may be ignored for relatively low CO/H2O density ratios (≤30 per cent/70 per cent). Finally, when the coma is a ∼50 per cent/50 per cent mixture of CO and H2O, the contribution of both colliders is similar and has to be considered. 

Abstract Galaxy clusters are expected to be both dark matter (DM) reservoirs and storage rooms for the cosmic-ray protons (CRp) that accumulate along the cluster's formation history. Accordingly, they are excellent targets to search for signals of DM annihilation and decay atγ-ray energies and are predicted to be sources of large-scaleγ-ray emission due to hadronic interactions in the intracluster medium (ICM).In this paper, we estimate the sensitivity of the Cherenkov Telescope Array (CTA) to detect diffuseγ-ray emission from the Perseus galaxy cluster.We first perform a detailed spatial and spectral modelling of the expected signal for both the DM and the CRp components. For each case, we compute the expected CTA sensitivity accounting for the CTA instrument response functions. The CTA observing strategy of the Perseus cluster is also discussed.In the absence of a diffuse signal (non-detection), CTA should constrain the CRp to thermal energy ratioX₅₀₀within the characteristic radiusR₅₀₀down to aboutX₅₀₀< 3 × 10^-3, for a spatial CRp distribution that follows the thermal gas and a CRp spectral index α_CRp= 2.3. Under the optimistic assumption of a pure hadronic origin of the Perseus radio mini-halo and depending on the assumed magnetic field profile, CTA should measure α_CRpdown to about Δα_CRp≃ 0.1 and the CRp spatial distribution with 10% precision, respectively. Regarding DM, CTA should improve the current ground-basedγ-ray DM limits from clusters observations on the velocity-averaged annihilation cross-section by a factor of up to ∼ 5, depending on the modelling of DM halo substructure. In the case of decay of DM particles, CTA will explore a new region of the parameter space, reaching models withτ_χ> 10²⁷s for DM masses above 1 TeV.These constraints will provide unprecedented sensitivity to the physics of both CRp acceleration and transport at cluster scale and to TeV DM particle models, especially in the decay scenario.