Search for: All records

The Xenon-Argon Technology (X-ArT) Collaboration presents a study on the dynamics of pure and xenon-doped liquid argon (LAr) scintillation. Using two types of silicon photomultipliers sensitive to different wavelength ranges, we provide evidence in favor of a contribution from long-lived ( $>10\mathrm{\mu }\mathrm{s}$) extreme ultraviolet (EUV) lines emitted from argon atomic states, which enhances the light yield. This component is present in both pure and xenon-doped LAr, becoming more pronounced at higher xenon concentrations, where it complements the traditional collisional energy transfer process. To explain this mechanism, we develop a comprehensive model of the Xe-doped LAr scintillation process that integrates both collisional and radiative contributions. Additionally, we investigate how xenon doping affects LAr scintillation light yield and pulse shape discrimination. Finally, we hypothesize that the EUV component may explain the emission of spurious electrons, a known challenge in light dark matter searches using noble liquids. By characterizing the scintillation dynamics in Xe-doped LAr, identifying the long-lived EUV component, and exploring the potential origin of spurious electrons, this work lays the groundwork for optimizing detector performance and advancing the design and sensitivity of future noble liquid particle detectors. Published by the American Physical Society2025 

The existence of dark matter in the universe is inferred from abundant astrophysical and cosmological observations. The Global Argon Dark Matter Collaboration (GADMC) aims to perform the searches for dark matter in the form of weakly interacting massive particles (WIMPs), whose collisions with argon nuclei would produce nuclear recoils with tens of keV energy. Argon has been considered an excellent medium for the direct detection of WIMPs as argon-based scintillation detectors can make use of pulse shape discrimination (PSD) to separate WIMP-induced nuclear recoil signals from electron recoil backgrounds with extremely high efficiency. However, argon-based direct dark matter searches must confront the presence of intrinsic³⁹Ar as the predominant source of electron recoil backgrounds (it is a beta-emitter with an endpoint energy of 565 keV and half-life of 269 years). Even with PSD, the³⁹Ar activity in atmospheric argon (AAr), mainly produced and maintained by cosmic ray-induced nuclear reactions, limits the ultimate size of argon-based detectors and restricts their ability to probe very-low-energy events. The discovery of argon from deep underground wells with significantly less³⁹Ar than that in AAr was an important step in the development of direct dark matter detection experiments using argon as the active target. Thanks to pioneering research and successful R&D, in 2012, the first 160 kg batch of underground argon (UAr) was extracted from a CO₂well in Cortez, Colorado. The DarkSide-50 experiment at the Gran Sasso National Laboratory (LNGS) in Italy, the first liquid argon detector ever operated with a UAr target, demonstrated a ∼ 1,400 suppression of the³⁹Ar activity with respect to the atmospheric argon. An even larger suppression is expected for⁴²Ar (another intrinsic beta-emitter with the⁴²K daughter isotope, also a beta-emitter) as its production is expected mainly in the upper atmosphere. Following the results of DarkSide-50, the GADMC initiated the UAr project for extraction from underground and cryogenic purification of 100 t of argon to be used as a target in the next-generation experiment DarkSide-20k. This paper contains a description of the Urania Plant in Cortez, Colorado, where UAr is extracted; the Aria Plant in Sardinia, Italy, an industrial-scale plant comprising a 350-m state-of-the-art cryogenic isotopic distillation column, designed for further purification of the extracted argon and further reduction of the isotopic abundance of³⁹Ar; and DArT, a facility for UAr radiopurity qualification at the Canfranc Underground Laboratory (LSC), Spain. Moreover, the high radiopurity of UAr leads to other possible applications, for instance, for those neutrinoless double-beta decay experiments using argon as shielding material or, more generally, for all those activities on argon-based detectors in high-energy physics or nuclear physics, which will be briefly discussed. 

Borexino could efficiently distinguish between $\alpha$and $\beta$radiation in its liquid scintillator by the characteristic time profile of its scintillation pulse. This $\alpha /\beta$discrimination, first demonstrated on the ton scale in the counting test facility prototype, was used throughout the lifetime of the experiment between 2007 and 2021. With this method, the $\alpha$events are identified and subtracted from the solar neutrino events similar to $\beta$. This is particularly important in liquid scintillators, as the $\alpha$scintillation is strongly quenched. In Borexino, the prominent ${}^{210}\mathrm{Po}$decay peak was a background in the energy range of electrons scattered from ${}^7\mathrm{Be}$solar neutrinos. Optimal $\alpha /\beta$discrimination was achieved with a , with a higher ability to leverage the timing information of the scintillation photons detected by the photomultiplier tubes. An event-by-event, high efficiency, stable, and uniform pulse shape discrimination was essential in characterizing the spatial distribution of background in the detector. This benefited most Borexino measurements, including solar neutrinos in the $pp$chain and the first direct observation of the CNO cycle in the Sun. This paper presents key milestones in $\alpha /\beta$discrimination in Borexino as a term of comparison for current and future large liquid scintillator detectors. Published by the American Physical Society2024 

Neutrino-nucleus cross section measurements are needed to improve interaction modeling to meet the precision needs of neutrino experiments in efforts to measure oscillation parameters and search for physics beyond the Standard Model. We review the difficulties associated with modeling neutrino-nucleus interactions that lead to a dependence on event generators in oscillation analyses and cross section measurements alike. We then describe data-driven model validation techniques intended to address this model dependence. The method relies on utilizing various goodness-of-fit tests and the correlations between different observables and channels to probe the model for defects in the phase space relevant for the desired analysis. These techniques shed light on relevant mismodeling, allowing it to be detected before it begins to bias the cross section results. We compare more commonly used model validation methods which directly validate the model against alternative ones to these data-driven techniques and show their efficacy with fake data studies. These studies demonstrate that employing data-driven model validation in cross section measurements represents a reliable strategy to produce robust results that will stimulate the desired improvements to interaction modeling. Published by the American Physical Society2025 

Abstract Directional sensitivity to nuclear recoils would provide a smoking gun for a possible discovery of dark matter in the form of WIMPs (Weakly Interacting Massive Particles). A hint of directional dependence of the response of a dual-phase argon Time Projection Chamber (TPC) was found in the SCENE experiment. Given the potential importance of such a capability in the framework of dark matter searches, a new dedicated experiment, ReD (Recoil Directionality), was designed by the Global Argon Dark Matter Collaboration, in order to scrutinise this hint. A small dual-phase argon TPC was irradiated with neutrons produced by the p(⁷Li,⁷Be)n reaction using the 15 MV TANDEM accelerator of the INFN - Laboratori Nazionali del Sud, Catania, Italy, so as to produce argon nuclear recoils in the range (20 - 100) keV of interest for dark matter searches. Energy and direction of nuclear recoils are inferred by the detection of the elastically-scattered neutron by a set of scintillation detectors. Events were selected by gating of the associated⁷Be, which is detected by a telescope of Si detectors. 

Abstract The scintillation time response of liquid argon has a key role in the discrimination of electronic backgrounds in dark matter search experiments. However, its extraordinary rejection power can be affected by various detector effects such as the delayed light emission of TetraPhenyl Butadiene, the most commonly used wavelength shifter, and the electric drift field applied in Time Projection Chambers. In this work, we characterized the TetraPhenyl Butadiene delayed response and the dependence of the pulse shape discrimination on the electric field, exploiting the data acquired with the ARIS, a small-scale single-phase liquid argon detector exposed to monochromatic neutron and gamma sources at the ALTO facility of IJC Lab in Orsay. 

Abstract The DarkSide-20k dark matter experiment, currently under construction at LNGS, features a dual-phase time projection chamber (TPC) with a ∼ 50 t argon target from an underground well. At this scale, it is crucial to optimise the argon flow pattern for efficient target purification and for fast distribution of internal gaseous calibration sources with lifetimes of the order of hours. To this end, we have performed computational fluid dynamics simulations and heat transfer calculations. The residence time distribution shows that the detector is well-mixed on time-scales of the turnover time (∼ 40 d). Notably, simulations show that despite a two-order-of-magnitude difference between the turnover time and the half-life of^83mKr of 1.83 h, source atoms have the highest probability to reach the centre of the TPC 13 min after their injection, allowing for a homogeneous distribution before undergoing radioactive decay. We further analyse the thermal aspects of dual-phase operation and define the requirements for the formation of a stable gas pocket on top of the liquid. We find a best-estimate value for the heat transfer rate at the liquid-gas interface of 62 W with an upper limit of 144 W and a minimum gas pocket inlet temperature of 89 K to avoid condensation on the acrylic anode. This study also informs the placement of liquid inlets and outlets in the TPC. The presented techniques are widely applicable to other large-scale, noble-liquid detectors. 

Large neutrino liquid argon time projection chamber (LArTPC) experiments can broaden their physics reach by reconstructing and interpreting MeV-scale energy depositions, or blips, present in their data. We demonstrate new calorimetric and particle discrimination capabilities at the MeV energy scale using reconstructed blips in data from the MicroBooNE LArTPC at Fermilab. We observe a concentration of low-energy ( $<3\mathrm{MeV}$) blips around fiberglass mechanical support struts along the time projection chamber edges with energy spectrum features consistent with the Compton edge of 2.614 MeV ${}^{208}\mathrm{Tl}$decay $\gamma$rays. These features are used to verify proper calibration of electron energy scales in MicroBooNE’s data to few percent precision and to measure the specific activity of ${}^{208}\mathrm{Tl}$in the fiberglass composing these struts, $(11.7\pm 0.2\left(\mathrm{stat}\right)\pm 3.1\left(\mathrm{syst}\right))\mathrm{Bq}/\mathrm{kg}$. Cosmogenically produced blips above 3 MeV in reconstructed energy are used to showcase the ability of large LArTPCs to distinguish between low-energy proton and electron energy depositions. An enriched sample of low-energy protons selected using this new particle discrimination technique is found to be smaller in data than in dedicated cosmic-ray simulations, suggesting either incorrect modeling of incident cosmic fluxes or particle transport modeling issues in eant4. Published by the American Physical Society2025 

Dark matter may induce an event in an Earth-based detector, and its event rate is predicted to show an annual modulation as a result of the Earth’s orbital motion around the Sun. We searched for this modulation signature using the ionization signal of the DarkSide-50 liquid argon time projection chamber. No significant signature compatible with dark matter is observed in the electron recoil equivalent energy range above $40{\mathrm{eV}}_{\mathrm{ee}}$, the lowest threshold ever achieved in such a search. Published by the American Physical Society2024