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Rosser, David ; Gerace, Dario ; Chen, Yueyang ; Liu, Yifan ; Whitehead, James ; Ryou, Albert ; Andreani, Lucio_C ; Majumdar, Arka ( , Optical Materials Express)
Establishing a coherent interaction between a material resonance and an optical cavity is a necessary first step to study semiconductor quantum optics. Here we report on the signature of a coherent interaction between a two-dimensional excitonic transition in monolayer MoSe2and a zero-dimensional, ultra-low mode volume (
V m ∼ 2(λ /n )3) on-chip photonic crystal nanocavity. This coherent interaction manifests as a dispersive shift of the cavity transmission spectrum, when the exciton-cavity detuning is decreased via temperature tuning. The exciton-cavity coupling is estimated to be ≈6.5 meV, with a cooperativity of ≈4.0 at 80 K, showing our material system is on the verge of strong coupling. The small mode-volume of the resonator is instrumental in reaching the strongly nonlinear regime, while on-chip cavities will help create a scalable quantum photonic platform. -
Chen, Yueyang ; Miao, Shengnan ; Wang, Tianmeng ; Zhong, Ding ; Saxena, Abhi ; Chow, Colin ; Whitehead, James ; Gerace, Dario ; Xu, Xiaodong ; Shi, Su-Fei ; et al ( , Nano Letters)null (Ed.)