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Lead-208 is the heaviest known doubly magic nucleus and its structure is therefore of special interest. Despite this magicity, which acts to provide a strong restorative force toward sphericity, it is known to exhibit both strong octupole correlations and some of the strongest quadrupole collectivity observed in doubly magic systems. In this Letter, we employ state-of-the-art experimental equipment to conclusively demonstrate, through four Coulomb-excitation measurements, the presence of a large, negative, spectroscopic quadrupole moment for both the vibrational octupole $3_1^{-}$and quadrupole $2_1^{+}$state, indicative of a preference for prolate deformation of the states. The observed quadrupole moment is discussed in the context of the expected splitting of the $3^{-}\otimes 3^{-}$two-phonon states, due to the coupling of the quadrupole and octupole motion. These results are compared with theoretical values from three different methods, which are unable to reproduce both the sign and magnitude of this deformation. Thus, in spite of its well-studied nature, ${}^{208}\mathrm{Pb}$remains a puzzle for our understanding of nuclear structure. Published by the American Physical Society2025 

The cross-section of the thermal neutron capture⁴¹Ar(n,γ)⁴²Ar(t_1/2=32.9 y) reaction was measured by irradiating a⁴⁰Ar sample at the high-flux reactor of Institut Laue-Langevin (ILL) Grenoble, France. The signature of the two-neutron capture has been observed by measuring the growth curve and identifying the 1524.6 keV γ-lines of the shorter-lived⁴²K(12.4 h) β⁻daughter of⁴²Ar. Our preliminary value of the⁴¹Ar(n,γ)⁴²Ar thermal cross section is 240(80) mb at 25.3 meV. For the first time, direct counting of⁴²Ar was performed using the ultra-high sensitivity technique of noble gas accelerator mass spectrometry (NOGAMS) at Argonne National Laboratory, USA. 

The thermodynamical conditions and the neutron density produced in a laser-induced implosion of a deuterium-tritium (DT) filled capsule at the National Ignition Facility (NIF) are the closest laboratory analog of stellar conditions. We plan to investigate neutron-induced reactions on 40 Ar, namely the 40 Ar( n , 2 n ) 39 Ar( t 1/2 =268 y), the 40 Ar( n , γ) 41 Ar(110 min) and the potential rapid two-neutron capture reaction 40 Ar(2 n , γ) 42 Ar(33 y) in an Ar-loaded DT capsule. The chemical inertness of noble gas Ar enables reliable collection of the reaction products.