The cross-section of the thermal neutron capture41Ar(n,γ)42Ar(t1/2=32.9 y) reaction was measured by irradiating a40Ar sample at the high-flux reactor of Institut Laue-Langevin (ILL) Grenoble, France. The signature of the two-neutron capture has been observed by measuring the growth curve and identifying the 1524.6 keV γ-lines of the shorter-lived42K(12.4 h) β−daughter of42Ar. Our preliminary value of the41Ar(n,γ)42Ar thermal cross section is 240(80) mb at 25.3 meV. For the first time, direct counting of42Ar was performed using the ultra-high sensitivity technique of noble gas accelerator mass spectrometry (NOGAMS) at Argonne National Laboratory, USA. more »« less
Paul, M.; Sahoo, R. N.; Tessler, M.; Jeet, J.; Velsko, C.; Zylstra, A.; Avila, M.; Dickerson, C.; Fougères, C.; Jayatissa, H.; et al
(, EPJ Web of Conferences)
Freeman, S.; Lederer-Woods, C.; Manna, A.; Mengoni, A.
(Ed.)
The thermodynamical conditions and the neutron density produced in a laser-induced implosion of a deuterium-tritium (DT) filled capsule at the National Ignition Facility (NIF) are the closest laboratory analog of stellar conditions. We plan to investigate neutron-induced reactions on 40 Ar, namely the 40 Ar( n , 2 n ) 39 Ar( t 1/2 =268 y), the 40 Ar( n , γ) 41 Ar(110 min) and the potential rapid two-neutron capture reaction 40 Ar(2 n , γ) 42 Ar(33 y) in an Ar-loaded DT capsule. The chemical inertness of noble gas Ar enables reliable collection of the reaction products.
Abratenko, P; Alterkait, O; Andrade_Aldana, D; Arellano, L; Asaadi, J; Ashkenazi, A; Balasubramanian, S; Baller, B; Barr, G; Barrow, D; et al
(, Journal of Instrumentation)
Abstract We present a novel methodology to search for intranuclear neutron-antineutron transition (n⟶n̅) followed byn̅-nucleon annihilation within an40Ar nucleus, using the MicroBooNE liquid argon time projection chamber (LArTPC) detector. A discovery of n⟶n̅transition or a new best limit on the lifetime of this process would either constitute physics beyond the Standard Model or greatly constrain theories of baryogenesis, respectively. The approach presented in this paper makes use of deep learning methods to select n⟶n̅events based on their unique features and differentiate them from cosmogenic backgrounds. The achieved signal and background efficiencies are (70.22 ± 6.04)% and (0.0020 ± 0.0003)%, respectively. A demonstration of a search is performed with a data set corresponding to an exposure of 3.32 ×1026neutron-years, and where the background rate is constrained through direct measurement, assuming the presence of a negligible signal. With this approach, no excess of events over the background prediction is observed, setting a demonstrative lower bound on the n⟶n̅lifetime in40Ar of τm≳ 1.1×1026years, and on the free n⟶n̅transition time of τn⟶n̅≳ 2.6×105s, each at the 90% confidence level. This analysis represents a first-ever proof-of-principle demonstration of the ability to search for this rare process in LArTPCs with high efficiency and low background.
Yan, Pei-Gen; Babb, James F
(, The Astrophysical Journal)
Abstract We calculate cross sections for fine-structure transitions of Ne+, Ar+, Ne2+, and Ar2+in collisions with atomic hydrogen by using quantum-mechanical methods. Relaxation rate coefficients are calculated for temperatures up to 10,000 K. The temperature-dependent critical densities for the relaxation of Ne+, Ar+, Ne2+, and Ar2+in collisions with H have been determined and compared to the critical densities for collisions with electrons. The present calculations will be useful for studies utilizing the infrared lines [Neii] 12.8, [Neiii] 15.6, [Neiii] 36.0, [Arii] 6.99, [Ariii] 8.99, and [Ariii] 21.8μm as diagnostics of, for example, planetary nebulae and star formation.
Holzer, Mark; DeVries, Timothy; Smethie, Jr., William
(, Geophysical Research Letters)
Abstract 39Ar with its 269‐year half‐life has great potential for constraining ocean ventilation and transport. Here we estimate the distribution of39Ar using a steady ocean circulation inverse model. Our estimates match available39Ar measurements to within an absolute error of ∼9% modern argon without major biases. We find that39Ar traces out the world ocean's ventilation pathways and that the39Ar age ΓArand the ideal mean age have broadly similar large‐scale patterns. At the surface,39Ar is close to saturated except at high latitudes. Undersaturation imparts a finite39Ar age to surface waters relative to the atmosphere, with peak values exceeding 100 years in Antarctic waters. This reservoir age is propagated into the interior with Antarctic Bottom Water, elevating ΓArby ∼50 years in the deep Pacific and Indian oceans. Our estimates identify the large‐scale gradients and uncertainty patterns of39Ar, thus providing guidance for future measurements.
Hou, S Q; Iliadis, C; Pignatari, M; Liu, J B; Trueman, T_C L; Li, J G; Xu, X X
(, Astronomy & Astrophysics)
Context.Accurate42Ti(p,γ)43V reaction rates are crucial for understanding the nucleosynthesis path of the rapid capture process (rpprocess) that occurs in X-ray bursts. Aims.We aim to improve the thermonuclear rates of42Ti(p,γ)43V based on more complete resonance information and a more accurate direct component, together with the recently released nuclear masses data. We also explore the impact of the newly obtained rates on therpprocess. Methods.We reevaluated the reaction rate of42Ti(p,γ)43V by the sum of the isolated resonance contribution instead of the Hauser-Feshbach statistical model. We used a Monte Carlo method to derive the associated uncertainties of new rates. The nucleosynthesis simulations were performed via the NuGrid post-processing code ppn. Results.The new rates differ from previous estimations due to the use of a series of updated resonance parameters and a direct S factor. Compared with the previous results from the Hauser-Feshbach statistical model, which assumes compound nucleus43V with a sufficiently high-level density in the energy region of astrophysical interest, large differences exist over the entire temperature region ofrp-process interest, up to two orders of magnitude. We consistently calculated the photodisintegration rate using our new nuclear masses via the detailed balance principle, and found the discrepancies among the different reverse rates are much larger than those for the forward rate, up to ten orders of magnitude at the temperature of 108K. Using a trajectory with a peak temperature of 1.95×109K, we performed therp-process nucleosynthesis simulations to investigate the impact of the new rates. Our calculations show that the adoption of the new forward and reverse rates result in abundance variations for Sc and Ca of 128% and 49%, respectively, compared to the variations for the statistical model rates. On the other hand, the overall abundance pattern is not significantly affected. The results of using new rates also confirm that therp-process path does not bypass the isotope43V. Conclusions.Our study found that the Hauser-Feshbach statistical model is inappropriate to the reaction rate evaluation for42Ti(p,γ)43V. The adoption of the new rates confirms that the reaction path of42Ti(p,γ)43V(p,γ)44Cr(β+)44V is a key branch of therpprocess in X-ray bursts.
Sahoo, R. N., Paul, M., Köster, U., Scott, R., Tessler, M., Zylstra, A., Avila, M. L., Dickerson, C., Jayatissa, H., Kohen, M.S., McLain, J., Pardo, R.C., Rehm, K. E., Tolstukhin, I., Vondrasek, R., Bailey, T., Callahan, L., Clark, A., Collon, P., Kashiv, Y., and Nelson, A. The 41 Ar(n,y) 42 Ar reaction. Retrieved from https://par.nsf.gov/biblio/10489621. EPJ Web of Conferences 284. Web. doi:10.1051/epjconf/202328401037.
Sahoo, R. N., Paul, M., Köster, U., Scott, R., Tessler, M., Zylstra, A., Avila, M. L., Dickerson, C., Jayatissa, H., Kohen, M.S., McLain, J., Pardo, R.C., Rehm, K. E., Tolstukhin, I., Vondrasek, R., Bailey, T., Callahan, L., Clark, A., Collon, P., Kashiv, Y., & Nelson, A. The 41 Ar(n,y) 42 Ar reaction. EPJ Web of Conferences, 284 (). Retrieved from https://par.nsf.gov/biblio/10489621. https://doi.org/10.1051/epjconf/202328401037
Sahoo, R. N., Paul, M., Köster, U., Scott, R., Tessler, M., Zylstra, A., Avila, M. L., Dickerson, C., Jayatissa, H., Kohen, M.S., McLain, J., Pardo, R.C., Rehm, K. E., Tolstukhin, I., Vondrasek, R., Bailey, T., Callahan, L., Clark, A., Collon, P., Kashiv, Y., and Nelson, A.
"The 41 Ar(n,y) 42 Ar reaction". EPJ Web of Conferences 284 (). Country unknown/Code not available: EDP Sciences. https://doi.org/10.1051/epjconf/202328401037.https://par.nsf.gov/biblio/10489621.
@article{osti_10489621,
place = {Country unknown/Code not available},
title = {The 41 Ar(n,y) 42 Ar reaction},
url = {https://par.nsf.gov/biblio/10489621},
DOI = {10.1051/epjconf/202328401037},
abstractNote = {The cross-section of the thermal neutron capture41Ar(n,γ)42Ar(t1/2=32.9 y) reaction was measured by irradiating a40Ar sample at the high-flux reactor of Institut Laue-Langevin (ILL) Grenoble, France. The signature of the two-neutron capture has been observed by measuring the growth curve and identifying the 1524.6 keV γ-lines of the shorter-lived42K(12.4 h) β−daughter of42Ar. Our preliminary value of the41Ar(n,γ)42Ar thermal cross section is 240(80) mb at 25.3 meV. For the first time, direct counting of42Ar was performed using the ultra-high sensitivity technique of noble gas accelerator mass spectrometry (NOGAMS) at Argonne National Laboratory, USA.},
journal = {EPJ Web of Conferences},
volume = {284},
publisher = {EDP Sciences},
author = {Sahoo, R. N. and Paul, M. and Köster, U. and Scott, R. and Tessler, M. and Zylstra, A. and Avila, M. L. and Dickerson, C. and Jayatissa, H. and Kohen, M.S. and McLain, J. and Pardo, R.C. and Rehm, K. E. and Tolstukhin, I. and Vondrasek, R. and Bailey, T. and Callahan, L. and Clark, A. and Collon, P. and Kashiv, Y. and Nelson, A.},
editor = {Mattoon, C.M. and Vogt, R. and Escher, J. and Thompson, I.}
}
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