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  1. Abstract

    With the rapid increase in lithium consumption for electric vehicle applications, its price soared during the past decade. To secure a reliable and cost-effective supply chain, it is critical to unlock alternative lithium extraction resources beyond conventional brine. In this study, we develop an electrochemical method to directly leach lithium from α-phase spodumene. We find the H2O2promoter can significantly reduce the leaching potential by facilitating the electron transfer and changing the reaction path. Upon leaching, β-phase spodumene shows a typical phase transformation to HAlSi2O6, while leached α-phase remains its original crystal phase with a lattice shrinkage. To demonstrate the scale-up potential of electrochemical leaching, we design a catalyst-modified high-throughput current collector for high loading of suspended spodumene, achieving a leaching current of 18 mA and a leaching efficiency of 92.2%. Electrochemical leaching will revolutionize traditional leaching and recycling processes by minimizing the environmental footprint and energy consumption.

     
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  2. Geospatial data conflation is the process of identifying and merging the corresponding features in two datasets that represent the same objects in reality. Conflation is needed in a wide range of geospatial analyses, yet it is a difficult task, often considered too unreliable and costly due to various discrepancies between GIS data sources. This study addresses the reliability issue of computerized conflation by developing stronger optimization-based conflation models for matching two network datasets with minimum discrepancy. Conventional models match roads on a feature-by-feature basis. By comparison, we propose a new node-arc conflation model that simultaneously matches road-center lines and junctions in a topologically consistent manner. Enforcing this topological consistency increases the reliability of conflation and reduces false matches. Similar to the well-known rubber-sheeting method, our model allows for the use of network junctions as “control” points for matching network edges. Unlike rubber sheeting, the new model is automatic and matches all junctions (and edges) in one pass. To the best of our knowledge, this is the first optimized conflation model that can match nodes and edges in one model. Computational experiments using six road networks in Santa Barbara, CA, showed that the new model is selective and reduces false matches more than existing optimized conflation models. On average, it achieves a precision of 94.7% with over 81% recall and achieves a 99.4% precision when enhanced with string distances. 
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    Free, publicly-accessible full text available January 1, 2025
  3. Abstract

    Geospatial data conflation is the process of combining multiple datasets about a geographic phenomenon to produce a single, richer dataset. It has received increased research attention due to its many applications in map making, transportation, planning, and temporal geospatial analyses, among many others. One approach to conflation, attempted from the outset in the literature, is the use of optimization‐based conflation methods. Conflation is treated as a natural optimization problem of minimizing the total number of discrepancies while finding corresponding features from two datasets. Optimization‐based conflation has several advantages over traditional methods including conciseness, being able to find an optimal solution, and ease of implementation. However, current optimization‐based conflation methods are also limited. A main shortcoming with current optimized conflation models (and other traditional methods as well) is that they are often too weak and cannot utilize the spatial context in each dataset while matching corresponding features. In particular, current optimal conflation models match a feature to targets independently from other features and therefore treat each GIS dataset as a collection of unrelated elements, reminiscent of the spaghetti GIS data model. Important contextual information such as the connectivity between adjacent elements (such as roads) is neglected during the matching. Consequently, such models may produce topologically inconsistent results. In this article, we address this issue by introducing new optimization‐based conflation models with structural constraints to preserve the connectivity and contiguity relation among features. The model is implemented using integer linear programming and compared with traditional spaghetti‐style models on multiple test datasets. Experimental results show that the new element connectivity (ec‐bimatching) model reduces false matches and consistently outperforms traditional models.

     
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  4. Spatial data conflation is aimed at matching and merging objects in two datasets into a more comprehensive one. Starting from the “map assignment problem” in the 1980s, optimized conflation models treat feature matching as a natural optimization problem of minimizing certain metrics, such as the total discrepancy. One complication in optimized conflation is that heterogeneous datasets can represent geographic features differently. Features can correspond to target features in the other dataset either on a one-to-one basis (forming full matches) or on a many-to-one basis (forming partial matches). Traditional models consider either full matching or partial matches exclusively. This dichotomy has several issues. Firstly, full matching models are limited and cannot capture any partial match. Secondly, partial matching models treat full matches just as partial matches, and they are more prone to admit false matches. Thirdly, existing conflation models may introduce conflicting directional matches. This paper presents a new model that captures both full and partial matches simultaneously. This allows us to impose structural constraints differently on full/partial matches and enforce the consistency between directional matches. Experimental results show that the new model outperforms conventional optimized conflation models in terms of precision (89.2%), while achieving a similar recall (93.2%). 
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  5. Citations of scientific papers and patents reveal the knowledge flow and usually serve as the metric for evaluating their novelty and impacts in the field. Citation Forecasting thus has various applications in the real world. Existing works on citation forecasting typically exploit the sequential properties of citation events, without exploring the citation network. In this paper, we propose to explore both the citation network and the related citation event sequences which provide valuable information for future citation forecasting. We propose a novel Citation Network and Event Sequence (CINES) Model to encode signals in the citation network and related citation event sequences into various types of embeddings for decoding to the arrivals of future citations. Moreover, we propose a temporal network attention and three alternative designs of bidirectional feature propagation to aggregate the retrospective and prospective aspects of publications in the citation network, coupled with the citation event sequence embeddings learned by a two-level attention mechanism for the citation forecasting. We evaluate our models and baselines on both a U.S. patent dataset and a DBLP dataset. Experimental results show that our models outperform the state-of-the-art methods, i.e., RMTPP, CYAN-RNN, Intensity-RNN, and PC-RNN, reducing the forecasting error by 37.76% - 75.32%. 
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  6. Research suggests that social relationships have substantial impacts on individuals’ health outcomes. Network intervention, through careful planning, can assist a network of users to build healthy relationships. However, most previous work is not designed to assist such planning by carefully examining and improving multiple network characteristics. In this paper, we propose and evaluate algorithms that facilitate network intervention planning through simultaneous optimization of network degree, closeness, betweenness, and local clustering coefficient, under scenarios involving Network Intervention with Limited Degradation - for Single target (NILD-S) and Network Intervention with Limited Degradation - for Multiple targets (NILD-M). We prove that NILD-S and NILD-M are NP-hard and cannot be approximated within any ratio in polynomial time unless P=NP. We propose the Candidate Re-selection with Preserved Dependency (CRPD) algorithm for NILD-S, and the Objective-aware Intervention edge Selection and Adjustment (OISA) algorithm for NILD-M. Various pruning strategies are designed to boost the efficiency of the proposed algorithms. Extensive experiments on various real social networks collected from public schools and Web and an empirical study are conducted to show that CRPD and OISA outperform the baselines in both efficiency and effectiveness. 
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  7. In this paper, we propose a novel representation learning framework, namely HIN2Vec, for heterogeneous information networks (HINs). The core of the proposed framework is a neural network model, also called HIN2Vec, designed to capture the rich semantics embedded in HINs by exploiting different types of relationships among nodes. Given a set of relationships specified in forms of meta-paths in an HIN, HIN2Vec carries out multiple prediction training tasks jointly based on a target set of relationships to learn latent vectors of nodes and meta-paths in the HIN. In addition to model design, several issues unique to HIN2Vec, including regularization of meta-path vectors, node type selection in negative sampling, and cycles in random walks, are examined. To validate our ideas, we learn latent vectors of nodes using four large-scale real HIN datasets, including Blogcatalog, Yelp, DBLP and U.S. Patents, and use them as features for multi-label node classification and link prediction applications on those networks. Empirical results show that HIN2Vec soundly outperforms the state-of-the-art representation learning models for network data, including DeepWalk, LINE, node2vec, PTE, HINE and ESim, by 6.6% to 23.8% ofmicro-f1 in multi-label node classification and 5% to 70.8% of MAP in link prediction. 
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