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Abstract Nepheline syenites from the ∼1.2 Ga Ilímaussaq Complex of southern Greenland are examined to assess the utility of anisotropy of magnetic susceptibility (AMS) fabrics as proxies for silicate petrofabrics. Mineral lamination is a relatively common structural feature in cumulate rocks, including in the Ilímaussaq intrusion, but there is little consensus on the process (or processes) responsible for its formation. The Ilímaussaq AMS data are combined with rock magnetic experiments and electron backscatter diffraction (EBSD) measurements to characterize the magnetic mineralogy and compare the magnetic fabrics obtained to the silicate petrofabric. The data show that Na-amphibole (arfvedsonite) is most likely the dominant control on the AMS fabrics in the coarse-grained nepheline syenites (referred to as kakortokites), and that the AMS fabric is inverse relative to the observed silicate fabric. The EBSD data for a kakortokite sample suggests that the petrofabric is defined by arfvedsonite and is wholly planar, with evidence of only weak cross-lineation of c axes. The fine-grained nepheline syenites (lujavrites), two of which have a well-developed lamination carried by Na-pyroxene (aegirine), appear to have composite AMS fabrics that are considered to be a consequence of a mixed aegirine (normal) and arfvedsonite (inverse) response. The combined datasets shed light on the mechanisms of fabric acquisition in both lithologies. In the kakortokites, the AMS fabrics and silicate crystallographic preferred orientations, as well as the lack of observed microstructural evidence for subsolidus intra-crystal deformation, support models invoking gravitationally controlled crystal mats in the development of the macro-rhythmic layering of these rocks. In the lujavrites, the strong planar fabrics revealed by both the AMS and EBSD datasets, with some evidence of subsolidus deformation, point to fabric formation and perhaps even aegirine crystallization at the postcumulus stage. The combination of EBSD and AMS fabric datasets is a powerful means of deciphering the processes responsible for mineral alignment in igneous cumulates.