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Optoelectronic devices combining single-layer graphene (SLG) and colloidal semiconducting nanocrystal (NC) heterojunctions have recently gained significant attention as efficient hybrid photodetectors. While most research has concentrated on systems using heavy metal-based semiconductor NCs, there is a need for further exploration of environmentally friendly nanomaterials, such as Cu2−xS. Chemical ligands play a crucial role in these hybrid photodetectors, as they enable charge transfer between the NCs and SLG. This study investigates the photoresponse of an SLG/Cu2−xS NCs heterojunction, comparing the effect of two short molecules—tetrabutylammonium iodide (TBAI) and 3,4-dimethylbenzenethiol (DMBT)—as surface ligands on the resulting structures. We have analysed charge transfer at the heterojunctions between SLG and the Cu2−xS NCs before and after modification with TBAI and DMBT using Raman spectroscopy and transconductance measurements under thermal equilibrium. The photoresponse of two hybrid devices based on three layers of Cu2₋xS NCs, deposited in one case on SLG/Cu2−xS/TBAI (“TBAI-only” device) and in the other on SLG/Cu2−xS/DMBT (“DMBT + TBAI” device), with a TBAI treatment applied, for both, after each layer deposition, has been evaluated under 450 nm laser diode illumination. The results indicate that the TBAI-only device exhibited a significant increase in photocurrent (4 μA), with high responsivity (40 mA/W) and fast response times (<1 s), while the DMBT + TBAI device had lower photocurrent (0.2 μA) and responsivity (2.4 μA), despite similar response speeds. The difference is attributed to DMBT’s π–π interactions with SLG, which enhances electronic coupling but reduces SLG’s mobility and responsivity.more » « less
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We present the strongest experimental limits to date on the mixing angle, , with which a new scalar particle, , mixes with the Higgs field in the mass range . This result uses the MicroBooNE liquid argon time projection chamber to search for decays of these Higgs-portal scalar particles through the channel with the decays of kaons in the NuMI neutrino beam acting as the source of the scalar particles. The analysis uses an exposure of protons on target of NuMI beam data including periods when the beam focusing system was configured to focus positively charged hadrons and separate periods when negatively charged hadrons were focused. The analysis searches for scalar particles produced from kaons decaying in flight in the beam’s decay volume and at rest in the target and absorber. At ( ) we set a limit of ( ) at the 95% confidence level.more » « lessFree, publicly-accessible full text available April 1, 2027
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Abstract Baryon number conservation is not guaranteed by any fundamental symmetry within the standard model, and therefore has been a subject of experimental and theoretical scrutiny for decades. So far, no evidence for baryon number violation has been observed. Large underground detectors have long been used for both neutrino detection and searches for baryon number violating processes. The next generation of large neutrino detectors will seek to improve upon the limits set by past and current experiments and will cover a range of lifetimes predicted by several Grand Unified Theories. In this White Paper, we summarize theoretical motivations and experimental aspects of searches for baryon number violation in neutrino experiments.more » « less
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We present an inclusive search for anomalous production of single-photon events from neutrino interactions in the MicroBooNE experiment. The search and its signal definition are motivated by the previous observation of a low-energy excess of electromagnetic shower events from the MiniBooNE experiment. We use the Wire-Cell reconstruction framework to select a sample of inclusive single-photon final-state interactions with a final efficiency and purity of 7.0% and 40.2%, respectively. We leverage simultaneous measurements of sidebands of charged current interactions and neutral current interactions producing mesons to constrain signal and background predictions and reduce uncertainties. We perform a blind analysis using a dataset collected from February 2016 to July 2018, corresponding to an exposure of protons on target from the Booster Neutrino Beam at Fermilab. In the full signal region, we observe agreement between the data and the prediction, with a goodness-of-fit value of 0.11. We then isolate a subsample of these events containing no visible protons, and observe data events above prediction, corresponding to just above local significance, concentrated at shower energies below 600 MeV.more » « lessFree, publicly-accessible full text available May 1, 2027
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The MicroBooNE experiment is an 85 tonne active mass liquid argon time projection chamber neutrino detector exposed to the on-axis Booster Neutrino Beam at Fermilab. One of MicroBooNE’s physics goals is the precise measurement of neutrino interactions on argon in the 1 GeV energy regime. Building on the capabilities of the MicroBooNE detector, this analysis identifies mesons, a key signature for the study of strange particle production in neutrino interactions. This measurement is furthermore valuable for background estimation for future nucleon decay searches and for improved reconstruction and particle identification capabilities in experiments such as the Deep Underground Neutrino Experiment. In this Letter, we present the first-ever measurement of a flux-integrated cross section for charged-current muon neutrino induced production on argon nuclei, determined to be based on an analysis of protons on target. This result was found to be consistent with model predictions from different neutrino event generators within the reported uncertainties.more » « lessFree, publicly-accessible full text available December 19, 2026
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The flux of cosmic ray muons at the Earth’s surface exhibits seasonal variations due to changes in the temperature of the atmosphere affecting the production and decay of mesons in the upper atmosphere. Using 1473 live days of data collected by the NuMI Off-axis Appearance (NOvA) Near Detector during 2018–2022, we studied the seasonal pattern in the multiple-muon event rate. The data confirm an anticorrelation between the multiple-muon event rate and effective atmospheric temperature, consistent across all the years of data. Previous analyses from MINOS and NOvA saw a similar anticorrelation but did not include an explanation. We find that this anticorrelation is driven by altitude–geometry effects as the average muon production height changes with the season. This has been studied with a CORSIKA cosmic ray simulation package by varying atmospheric parameters, and provides an explanation to a longstanding discrepancy between the seasonal phases of single and multiple-muon events.more » « lessFree, publicly-accessible full text available January 1, 2027
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Abstract The existence of three distinct neutrino flavours,νe,νμandντ, is a central tenet of the Standard Model of particle physics1,2. Quantum-mechanical interference can allow a neutrino of one initial flavour to be detected sometime later as a different flavour, a process called neutrino oscillation. Several anomalous observations inconsistent with this three-flavour picture have motivated the hypothesis that an additional neutrino state exists, which does not interact directly with matter, termed as ‘sterile’ neutrino,νs(refs. 3–9). This includes anomalous observations from the Liquid Scintillator Neutrino Detector (LSND)3experiment and Mini-Booster Neutrino Experiment (MiniBooNE)4,5, consistent withνμ → νetransitions at a distance inconsistent with the three-neutrino picture. Here we use data obtained from the MicroBooNE liquid-argon time projection chamber10in two accelerator neutrino beams to exclude the single light sterile neutrino interpretation of the LSND and MiniBooNE anomalies at the 95% confidence level (CL). Moreover, we rule out a notable portion of the parameter space that could explain the gallium anomaly6–8. This is one of the first measurements to use two accelerator neutrino beams to break a degeneracy betweenνeappearance and disappearance, which would otherwise weaken the sensitivity to the sterile neutrino hypothesis. We find no evidence for eitherνμ → νeflavour transitions orνedisappearance that would indicate non-standard flavour oscillations. Our results indicate that previous anomalous observations consistent withνμ → νetransitions cannot be explained by introducing a single sterile neutrino state.more » « lessFree, publicly-accessible full text available December 3, 2026
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This Letter reports measurements of muon-neutrino disappearance and electron-neutrino appearance and the corresponding antineutrino processes between the two NOvA detectors in the NuMI neutrino beam. These measurements use a dataset with double the neutrino mode beam exposure that was previously analyzed, along with improved simulation and analysis techniques. A joint fit to these samples in the three-flavor paradigm results in the most precise single-experiment constraint on the atmospheric neutrino mass splitting, if the mass ordering is normal (inverted). In both orderings, a region close to maximal mixing with is preferred. The NOvA data show a mild preference for the normal mass ordering with a Bayes factor of 2.4 (corresponding to 70% of the posterior probability), indicating that the normal ordering is 2.4 times more probable than the inverted ordering. When incorporating a 2D constraint based on Daya Bay data, this preference strengthens to a Bayes factor of 6.6 (87%).more » « lessFree, publicly-accessible full text available January 1, 2027
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We report results from an updated search for neutral current (NC) resonant baryon production and subsequent radiative decay (NC ). We consider events with and without final state protons; events with a proton can be compared with the kinematics of a baryon decay, while events without a visible proton represent a more generic phase space. In order to maximize sensitivity to each topology, we simultaneously make use of two different reconstruction paradigms, Pandora and Wire-Cell, which have complementary strengths, and select mostly orthogonal sets of events. Considering an overall scaling of the NC rate as an explanation of the MiniBooNE anomaly, our data exclude this hypothesis at 94.4% CL. When we decouple the expected correlations between NC events with and without final state protons, our data exclude an interpretation in which all excess events have associated protons at , and are consistent with an interpretation in which all excess events have no associated protons at .more » « lessFree, publicly-accessible full text available November 17, 2026
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Free, publicly-accessible full text available October 12, 2026
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