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Optoelectronic devices combining single-layer graphene (SLG) and colloidal semiconducting nanocrystal (NC) heterojunctions have recently gained significant attention as efficient hybrid photodetectors. While most research has concentrated on systems using heavy metal-based semiconductor NCs, there is a need for further exploration of environmentally friendly nanomaterials, such as Cu2−xS. Chemical ligands play a crucial role in these hybrid photodetectors, as they enable charge transfer between the NCs and SLG. This study investigates the photoresponse of an SLG/Cu2−xS NCs heterojunction, comparing the effect of two short molecules—tetrabutylammonium iodide (TBAI) and 3,4-dimethylbenzenethiol (DMBT)—as surface ligands on the resulting structures. We have analysed charge transfer at the heterojunctions between SLG and the Cu2−xS NCs before and after modification with TBAI and DMBT using Raman spectroscopy and transconductance measurements under thermal equilibrium. The photoresponse of two hybrid devices based on three layers of Cu2₋xS NCs, deposited in one case on SLG/Cu2−xS/TBAI (“TBAI-only” device) and in the other on SLG/Cu2−xS/DMBT (“DMBT + TBAI” device), with a TBAI treatment applied, for both, after each layer deposition, has been evaluated under 450 nm laser diode illumination. The results indicate that the TBAI-only device exhibited a significant increase in photocurrent (4 μA), with high responsivity (40 mA/W) and fast response times (<1 s), while the DMBT + TBAI device had lower photocurrent (0.2 μA) and responsivity (2.4 μA), despite similar response speeds. The difference is attributed to DMBT’s π–π interactions with SLG, which enhances electronic coupling but reduces SLG’s mobility and responsivity.more » « lessFree, publicly-accessible full text available January 1, 2026
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Neutrino-nucleus cross section measurements are needed to improve interaction modeling to meet the precision needs of neutrino experiments in efforts to measure oscillation parameters and search for physics beyond the Standard Model. We review the difficulties associated with modeling neutrino-nucleus interactions that lead to a dependence on event generators in oscillation analyses and cross section measurements alike. We then describe data-driven model validation techniques intended to address this model dependence. The method relies on utilizing various goodness-of-fit tests and the correlations between different observables and channels to probe the model for defects in the phase space relevant for the desired analysis. These techniques shed light on relevant mismodeling, allowing it to be detected before it begins to bias the cross section results. We compare more commonly used model validation methods which directly validate the model against alternative ones to these data-driven techniques and show their efficacy with fake data studies. These studies demonstrate that employing data-driven model validation in cross section measurements represents a reliable strategy to produce robust results that will stimulate the desired improvements to interaction modeling. Published by the American Physical Society2025more » « lessFree, publicly-accessible full text available May 1, 2026
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Abstract Baryon number conservation is not guaranteed by any fundamental symmetry within the standard model, and therefore has been a subject of experimental and theoretical scrutiny for decades. So far, no evidence for baryon number violation has been observed. Large underground detectors have long been used for both neutrino detection and searches for baryon number violating processes. The next generation of large neutrino detectors will seek to improve upon the limits set by past and current experiments and will cover a range of lifetimes predicted by several Grand Unified Theories. In this White Paper, we summarize theoretical motivations and experimental aspects of searches for baryon number violation in neutrino experiments.more » « less
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Double- and single-differential cross sections for inclusive charged-current -nucleus scattering are reported for the kinematic domain 0 to in three-momentum transfer and 0 to 2 GeV in available energy, at a mean energy of 1.86 GeV. The measurements are based on an estimated 995,760 charged-current (CC) interactions in the scintillator medium of the NOvA Near Detector. The subdomain populated by 2-particle-2-hole (2p2h) reactions is identified by the cross section excess relative to predictions for -nucleus scattering that are constrained by a data control sample. Models for 2-particle-2-hole processes are rated by comparisons of the predicted-versus-measured CC inclusive cross section over the full phase space and in the restricted subdomain. Shortfalls are observed in neutrino generator predictions obtained using the theory-based València and SuSAv2 2p2h models. Published by the American Physical Society2025more » « lessFree, publicly-accessible full text available March 1, 2026
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Large neutrino liquid argon time projection chamber (LArTPC) experiments can broaden their physics reach by reconstructing and interpreting MeV-scale energy depositions, or blips, present in their data. We demonstrate new calorimetric and particle discrimination capabilities at the MeV energy scale using reconstructed blips in data from the MicroBooNE LArTPC at Fermilab. We observe a concentration of low-energy ( ) blips around fiberglass mechanical support struts along the time projection chamber edges with energy spectrum features consistent with the Compton edge of 2.614 MeV decay rays. These features are used to verify proper calibration of electron energy scales in MicroBooNE’s data to few percent precision and to measure the specific activity of in the fiberglass composing these struts, . Cosmogenically produced blips above 3 MeV in reconstructed energy are used to showcase the ability of large LArTPCs to distinguish between low-energy proton and electron energy depositions. An enriched sample of low-energy protons selected using this new particle discrimination technique is found to be smaller in data than in dedicated cosmic-ray simulations, suggesting either incorrect modeling of incident cosmic fluxes or particle transport modeling issues in eant4. Published by the American Physical Society2025more » « lessFree, publicly-accessible full text available February 1, 2026
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We report a search for neutrino oscillations to sterile neutrinos under a model with three active and one sterile neutrinos ( model). This analysis uses the NOvA detectors exposed to the NuMI beam, running in neutrino mode. The data exposure, protons on target, doubles that previously analyzed by NOvA, and the analysis is the first to use charged-current interactions in conjunction with neutral-current interactions. Neutrino samples in the near and far detectors are fitted simultaneously, enabling the search to be carried out over a range extending 2 (3) orders of magnitude above (below) . NOvA finds no evidence for active-to-sterile neutrino oscillations under the model at 90% confidence level. New limits are reported in multiple regions of parameter space, excluding some regions currently allowed by IceCube at 90% confidence level. We additionally set the most stringent limits for anomalous appearance for . Published by the American Physical Society2025more » « lessFree, publicly-accessible full text available February 1, 2026
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Abstract Measuring observables to constrain models using maximum-likelihood estimation is fundamental to many physics experiments. Wilks' theorem provides a simple way to construct confidence intervals on model parameters, but it only applies under certain conditions. These conditions, such as nested hypotheses and unbounded parameters, are often violated in neutrino oscillation measurements and other experimental scenarios. Monte Carlo methods can address these issues, albeit at increased computational cost. In the presence of nuisance parameters, however, the best way to implement a Monte Carlo method is ambiguous. This paper documents the method selected by the NOvA experiment, the profile construction. It presents the toy studies that informed the choice of method, details of its implementation, and tests performed to validate it. It also includes some practical considerations which may be of use to others choosing to use the profile construction.more » « lessFree, publicly-accessible full text available February 1, 2026
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We present a measurement of neutral pion production in charged-current interactions using data recorded with the MicroBooNE detector exposed to Fermilab’s booster neutrino beam. The signal comprises one muon, one neutral pion, any number of nucleons, and no charged pions. Studying neutral pion production in the MicroBooNE detector provides an opportunity to better understand neutrino-argon interactions, and is crucial for future accelerator-based neutrino oscillation experiments. Using a dataset corresponding to protons on target, we present single-differential cross sections in muon and neutral pion momenta, scattering angles with respect to the beam for the outgoing muon and neutral pion, as well as the opening angle between the muon and neutral pion. Data extracted cross sections are compared to generator predictions. We report good agreement between the data and the models for scattering angles, except for an over-prediction by generators at muon forward angles. Similarly, the agreement between data and the models as a function of momentum is good, except for an underprediction by generators in the medium momentum ranges, 200–400 MeV for muons and 100–200 MeV for pions. Published by the American Physical Society2024more » « less
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We present a deep learning-based method for estimating the neutrino energy of charged-current neutrino-argon interactions. We employ a recurrent neural network (RNN) architecture for neutrino energy estimation in the MicroBooNE experiment, utilizing liquid argon time projection chamber (LArTPC) detector technology. Traditional energy estimation approaches in LArTPCs, which largely rely on reconstructing and summing visible energies, often experience sizable biases and resolution smearing because of the complex nature of neutrino interactions and the detector response. The estimation of neutrino energy can be improved after considering the kinematics information of reconstructed final-state particles. Utilizing kinematic information of reconstructed particles, the deep learning-based approach shows improved resolution and reduced bias for the muon neutrino Monte Carlo simulation sample compared to the traditional approach. In order to address the common concern about the effectiveness of this method on experimental data, the RNN-based energy estimator is further examined and validated with dedicated data-simulation consistency tests using MicroBooNE data. We also assess its potential impact on a neutrino oscillation study after accounting for all statistical and systematic uncertainties and show that it enhances physics sensitivity. This method has good potential to improve the performance of other physics analyses. Published by the American Physical Society2024more » « less
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This Letter reports a search for charge-parity ( ) symmetry violating nonstandard interactions (NSI) of neutrinos with matter using the NOvA Experiment, and examines their effects on the determination of the standard oscillation parameters. Data from and oscillation channels are used to measure the effect of the NSI parameters and . With 90% CL the magnitudes of the NSI couplings are constrained to be and . A degeneracy at is reported, and we observe that the presence of NSI limits sensitivity to the standard phase . Published by the American Physical Society2024more » « less
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