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Constraints on the thickness, transitional boundaries, and composition of Earth's crust are pivotal in studying its formation and evolution. We use data from 132 seismic installations throughout the northeastern US to explore how tectonic events, such as orogenesis and rifting, have altered the crust of the northeastern US and southeastern Canada, and to distinguish between Laurentia and the Appalachian terranes. We include data from seismic installations from the NEST and SEISConn experiments, spanning the Laurentia–Appalachian boundary, and present estimates of crustal thickness,V_p/V_s, and thickness of the transition between crustal and mantle rocks using Ps receiver functions. We find some first-order differences between Laurentia and Appalachian terranes, with Laurentia exhibiting thicker crust (c.39 v.c.33 km) and a broader crust–mantle transition thickness (c.3 v. <1.5 km). AverageV_p/V_svalues are similar between Laurentia (c.1.77) and Appalachian terranes (c.1.74); however, we identify anomalousV_p/V_sin a few regions, including highV_p/V_saround the Adirondack Mountains and lowV_p/V_sin southern New England. The southern New England region is also anomalous in terms of its systematically thinner crust and sharper crust–mantle transition, which may be a consequence of the formation and collapse of the Acadian altiplano during the mid-to-late Paleozoic.