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Aerosol radiative forcing is an important but often poorly understood component of regional climate. While glacier ice contains the most detailed archives of past atmospheric aerosol composition and temperature, no well-preserved ice records extending into the last climatic transition have been reported for the historically important European region. Here, we use an Alpine ice core to document changes in European aerosols and climate from the end of the last glacial age (LGA) through the Holocene. The core was drilled on a glacier dome in the French Alps called the Dôme du Goûter (DDG), and it provides a stratigraphically intact record of aerosol and climate extending to at least 12 kyears (ky) before present. Although dating near the base of the glacier is not well constrained, the oldest DDG ice layers reflect glacial conditions in western Europe during the LGA. In addition to changes in atmospheric transport, increased sea-salt and dust deposition in western Europe recorded in the LGA ice suggest enhanced westerly winds and more active dust sources, possibly including North Africa. Deposition of terrestrial biogenic indicators during the cold LGA climate was lower, however, consistent with strongly reduced European vegetation. The DDG record of terrestrial biogenic emissions also suggests a decline of European forests throughout the Holocene, resulting from deterioration of climatic conditions and more recently from establishment of the first agricultural societies. The pronounced changes in atmospheric aerosol recorded in Alpine ice imply large variations in aerosol radiative forcing in western Europe during the last 12 ky. 

Ancient texts and archaeological evidence indicate substantial lead exposure during antiquity that potentially impacted human health. Although lead exposure routes were many and included the use of glazed tablewares, paints, cosmetics, and even intentional ingestion, the most significant for the nonelite, rural majority of the population may have been through background air pollution from mining and smelting of silver and lead ores that underpinned the Roman economy. Here, we determined potential health effects of this air pollution using Arctic ice core measurements of Roman-era lead pollution, atmospheric modeling, and modern epidemiology-based relationships between air concentrations, blood lead levels (BLLs), and cognitive decline. Findings suggest air lead concentrations exceeded 150 ng/m³near metallurgical emission sources, with average enhancements of >1.0 ng/m³over Europe during the Pax Romana apogee of the Roman Empire. The result was blood lead enhancements in young children of about 2.4 µg/dl above an estimated Neolithic background of 1.0 µg/dl, leading to widespread cognitive decline including a 2.5-to-3 point reduction in intelligence quotient throughout the Roman Empire. 

Abstract Estimating fire emissions prior to the satellite era is challenging because observations are limited, leading to large uncertainties in the calculated aerosol climate forcing following the preindustrial era. This challenge further limits the ability of climate models to accurately project future climate change. Here, we reconstruct a gridded dataset of global biomass burning emissions from 1750 to 2010 using inverse analysis that leveraged a global array of 31 ice core records of black carbon deposition fluxes, two different historical emission inventories as a priori estimates, and emission-deposition sensitivities simulated by the atmospheric chemical transport model GEOS-Chem. The reconstructed emissions exhibit greater temporal variabilities which are more consistent with paleoclimate proxies. Our ice core constrained emissions reduced the uncertainties in simulated cloud condensation nuclei and aerosol radiative forcing associated with the discrepancy in preindustrial biomass burning emissions. The derived emissions can also be used in studies of ocean and terrestrial biogeochemistry.