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Hazardous atmospheric icing conditions occur at sub-zero temperatures when droplets come into contact with aircraft and freeze, degrading aircraft performance and handling, introducing bias into some of the vital measurements needed for aircraft operation (e.g., air speed). Nonetheless, government regulations allow certified aircraft to fly in limited icing environments. The capability of aircraft sensors to identify all hazardous icing environments is limited. To address the current challenges in aircraft icing detection and protection, we present herein a platform designed for in-flight testing of ice protection solutions and icing detection technologies. The recently developed Platform for Ice-accretion and Coatings Tests with Ultrasonic Readings (PICTUR) was evaluated using CFD simulations and installed on the National Research Council Canada (NRC) Convair-580 aircraft that has flown in icing conditions over North East USA, during February 2022. This aircraft is a flying laboratory, equipped with more than 40 sensors providing a comprehensive characterization of the flight environment including measurements of temperature, pressure, wind speed and direction, water droplet size and number distribution, and hydrometeor habits imagery. The flight tests of the platform included assessment of passive icephobic coatings as well as heat-assisted tests. Monitoring tools included visual high resolution, real-time inspection of the surface as well as detection of surface ice using NRC’s Ultrasonic Ice Accretion Sensors (UIAS). In this paper, we present the new platform and show some preliminary commissioning results of PICTUR, collected inflight under, predominantly, supercooled small droplets and supercooled large drops (SLD) icing conditions. The combination of the platform and the complementary sensors on the aircraft demonstrated an effective and unique technique for icing studies in a natural environment. 

Anthropogenic organic carbon emissions reporting has been largely limited to subsets of chemically speciated volatile organic compounds. However, new aircraft-based measurements revealed total gas-phase organic carbon emissions that exceed oil sands industry–reported values by 1900% to over 6300%, the bulk of which was due to unaccounted-for intermediate-volatility and semivolatile organic compounds. Measured facility-wide emissions represented approximately 1% of extracted petroleum, resulting in total organic carbon emissions equivalent to that from all other sources across Canada combined. These real-world observations demonstrate total organic carbon measurements as a means of detecting unknown or underreported carbon emissions regardless of chemical features. Because reporting gaps may include hazardous, reactive, or secondary air pollutants, fully constraining the impact of anthropogenic emissions necessitates routine, comprehensive total organic carbon monitoring as an inherent check on mass closure. 

Abstract During near-0°C surface conditions, diverse precipitation types (p-types) are possible, including rain, drizzle, freezing rain, freezing drizzle, ice pellets, wet snow, snow, and snow pellets. Near-0°C precipitation affects wide swaths of the United States and Canada, impacting aviation, road transportation, power generation and distribution, winter recreation, ecology, and hydrology. Fundamental challenges remain in observing, diagnosing, simulating, and forecasting near-0°C p-types, particularly during transitions and within complex terrain. Motivated by these challenges, the field phase of the Winter Precipitation Type Research Multi-scale Experiment (WINTRE-MIX) was conducted from 1 February – 15 March 2022 to better understand how multiscale processes influence the variability and predictability of p-type and amount under near-0°C surface conditions. WINTRE-MIX took place near the US / Canadian border, in northern New York and southern Quebec, a region with plentiful near-0°C precipitation influenced by terrain. During WINTRE-MIX, existing advanced mesonets in New York and Quebec were complemented by deployment of: (1) surface instruments, (2) the National Research Council Convair-580 research aircraft with W- and X-band Doppler radars and in situ cloud and aerosol instrumentation, (3) two X-band dual-polarization Doppler radars and a C-band dual-polarization Doppler radar from University of Illinois, and (4) teams collecting manual hydrometeor observations and radiosonde measurements. Eleven intensive observing periods (IOPs) were coordinated. Analysis of these WINTRE-MIX IOPs is illuminating how synoptic dynamics, mesoscale dynamics, and microscale processes combine to determine p-type and its predictability under near-0°C conditions. WINTRE-MIX research will contribute to improving nowcasts and forecasts of near-0°C precipitation through evaluation and refinement of observational diagnostics and numerical forecast models. 

Abstract A new method that automatically determines the modality of an observed particle size distribution (PSD) and the representation of each mode as a gamma function was used to characterize data obtained during the High Altitude Ice Crystals and High Ice Water Content (HAIC-HIWC) project based out of Cayenne, French Guiana, in 2015. PSDs measured by a 2D stereo probe and a precipitation imaging probe for particles with maximum dimension ( D max ) > 55 μ m were used to show how the gamma parameters varied with environmental conditions, including temperature ( T ) and convective properties such as cloud type, mesoscale convective system (MCS) age, distance away from the nearest convective peak, and underlying surface characteristics. Four kinds of modality PSDs were observed: unimodal PSDs and three types of multimodal PSDs (Bimodal1 with breakpoints 100 ± 20 μ m between modes, Bimodal2 with breakpoints 1000 ± 300 μ m, and Trimodal PSDs with two breakpoints). The T and ice water content (IWC) are the most important factors influencing the modality of PSDs, with the frequency of multimodal PSDs increasing with increasing T and IWC. An ellipsoid of equally plausible solutions in ( N o – λ–μ ) phase space is defined for each mode of the observed PSDs for different environmental conditions. The percentage overlap between ellipsoids was used to quantify the differences between overlapping ellipsoids for varying conditions. The volumes of the ellipsoid decrease with increasing IWC for most cases, and ( N o – λ–μ ) vary with environmental conditions related to distribution of IWC. HIWC regions are dominated by small irregular ice crystals and columns. The parameters ( N o – λ–μ ) in each mode exhibit mutual dependence. 

Abstract. Secondary ice production (SIP) is an important physicalphenomenon that results in an increase in the ice particle concentration and cantherefore have a significant impact on the evolution of clouds. In thisstudy, idealized simulations of a mesoscale convective system (MCS) wereconducted using a high-resolution (250 m horizontal grid spacing) mesoscalemodel and a detailed bulk microphysics scheme in order to examine theimpacts of SIP on the microphysics and dynamics of a simulated tropical MCS.The simulations were compared to airborne in situ and remote sensing observationscollected during the “High Altitude Ice Crystals – High Ice Water Content”(HAIC-HIWC) field campaign in 2015. It was found that the observed high icenumber concentration can only be simulated by models that include SIPprocesses. The inclusion of SIP processes in the microphysics scheme is crucialfor the production and maintenance of the high ice water content observed intropical convection. It was shown that SIP can enhance the strength of theexisting convective updrafts and result in the initiation of new updraftsabove the melting layer. Agreement between the simulations and observationshighlights the impacts of SIP on the maintenance of tropical MCSs in natureand the importance of including SIP parameterizations in models. 

Abstract Convective clouds play an important role in the Earth’s climate system and are a known source of extreme weather. Gaps in our understanding of convective vertical motions, microphysics, and precipitation across a full range of aerosol and meteorological regimes continue to limit our ability to predict the occurrence and intensity of these cloud systems. Towards improving predictability, the National Science Foundation (NSF) sponsored a large field experiment entitled “Experiment of Sea Breeze Convection, Aerosols, Precipitation, and Environment (ESCAPE).” ESCAPE took place between 30 May - 30 Sept. 2022 in the vicinity of Houston, TX because this area frequently experiences isolated deep convection that interacts with the region's mesoscale circulations and its range of aerosol conditions. ESCAPE focused on collecting observations of isolated deep convection through innovative sampling, and on developing novel analysis techniques. This included the deployment of two research aircraft, the National Research Council of Canada Convair-580 and the Stratton Park Engineering Company Learjet, which combined conducted 24 research flights from 30 May to 17 June. On the ground, three mobile X-band radars, and one mobile Doppler lidar truck equipped with soundings, were deployed from 30 May to 28 June. From 1 August to 30 Sept. 2022, a dual-polarization C-band radar was deployed and operated using a novel, multi-sensor agile adaptive sampling strategy to track the entire lifecycle of isolated convective clouds. Analysis of the ESCAPE observations has already yielded preliminary findings on how aerosols and environmental conditions impact the convective life cycle. 

Abstract. High ice water content (HIWC) regions in tropical deep convective clouds, composed of high concentrations of small ice crystals, were not reproduced by Weather Research and Forecasting (WRF) model simulations at 1 km horizontal grid spacing using four different bulk microphysics schemes (i.e., the WRF single‐moment 6‐class microphysics scheme (WSM6), the Morrison scheme and the Predicted Particle Properties (P3) scheme with one- and two-ice options) for conditions encountered during the High Altitude Ice Crystals (HAIC) and HIWC experiment. Instead, overestimates of radar reflectivity and underestimates of ice number concentrations were realized. To explore formation mechanisms for large numbers of small ice crystals in tropical convection, a series of quasi-idealized WRF simulations varying the model resolution, aerosol profile, and representation of secondary ice production (SIP) processes are conducted based on an observed radiosonde released at Cayenne during the HAIC-HIWC field campaign. The P3 two-ice category configuration, which has two “free” ice categories to represent all ice-phase hydrometeors, is used. Regardless of the horizontal grid spacing or aerosol profile used, without including SIP processes the model produces total ice number concentrations about 2 orders of magnitude less than observed at −10 ∘C and about an order of magnitude less than observed at −30 ∘C but slightly overestimates the total ice number concentrations at −45 ∘C. Three simulations including one of three SIP mechanisms separately (i.e., the Hallett–Mossop mechanism, fragmentation during ice–ice collisions, and shattering of freezing droplets) also do not replicate observed HIWCs, with the results of the simulation including shattering of freezing droplets most closely resembling the observations. The simulation including all three SIP processes produces HIWC regions at all temperature levels, remarkably consistent with the observations in terms of ice number concentrations and radar reflectivity, which is not replicated using the original P3 two-ice category configuration. This simulation shows that primary ice production plays a key role in generating HIWC regions at temperatures <-40 ∘C, shattering of freezing droplets dominates ice particle production in HIWC regions at temperatures between −15 and 0 ∘C during the early stage of convection, and fragmentation during ice–ice collisions dominates at temperatures between −15 and 0 ∘C during the later stage of convection and at temperatures between −40 and −20 ∘C over the whole convection period. This study confirms the dominant role of SIP processes in the formation of numerous small crystals in HIWC regions. 

Wildfire impacts on air quality and climate are expected to be exacerbatedby climate change with the most pronounced impacts in the boreal biome.Despite the large geographic coverage, there is limited information onboreal forest wildfire emissions, particularly for organic compounds, whichare critical inputs for air quality model predictions of downwind impacts.In this study, airborne measurements of 193 compounds from 15 instruments,including 173 non-methane organics compounds (NMOG), were used to providethe most detailed characterization, to date, of boreal forest wildfireemissions. Highly speciated measurements showed a large diversity ofchemical classes highlighting the complexity of emissions. Usingmeasurements of the total NMOG carbon (NMOGT), the ΣNMOG wasfound to be 50 % ± 3 % to 53 % ± 3 % of NMOGT, of which, theintermediate- and semi-volatile organic compounds (I/SVOCs) were estimatedto account for 7 % to 10 %. These estimates of I/SVOC emission factorsexpand the volatility range of NMOG typically reported. Despite extensivespeciation, a substantial portion of NMOGT remained unidentified(47 % ± 15 % to 50 % ± 15 %), with expected contributions from morehighly-functionalized VOCs and I/SVOCs. The emission factors derived in thisstudy improve wildfire chemical speciation profiles and are especiallyrelevant for air quality modelling of boreal forest wildfires. Theseaircraft-derived emission estimates were further linked with those derivedfrom satellite observations demonstrating their combined value in assessingvariability in modelled emissions. These results contribute to theverification and improvement of models that are essential for reliablepredictions of near-source and downwind pollution resulting from borealforest wildfires. 

Abstract. Regions with high ice water content (HIWC), composed of mainly small ice crystals, frequently occur over convective clouds in the tropics. Such regions can have median mass diameters (MMDs) <300 µm and equivalent radar reflectivities <20 dBZ. To explore formation mechanisms for these HIWCs, high-resolution simulations of tropical convective clouds observed on 26 May 2015 during the High Altitude Ice Crystals – High Ice Water Content (HAIC-HIWC) international field campaign based out of Cayenne, French Guiana, are conducted using the Weather Research and Forecasting (WRF) model with four different bulk microphysics schemes: the WRF single‐moment 6‐class microphysics scheme (WSM6), the Morrison scheme, and the Predicted Particle Properties (P3) scheme with one- and two-ice options. The simulations are evaluated against data from airborne radar and multiple cloud microphysics probes installed on the French Falcon 20 and Canadian National Research Council (NRC) Convair 580 sampling clouds at different heights. WRF simulations with different microphysics schemes generally reproduce the vertical profiles of temperature, dew-point temperature, and winds during this event compared with radiosonde data, and the coverage and evolution of this tropical convective system compared to satellite retrievals. All of the simulations overestimate the intensity and spatial extent of radar reflectivity by over 30 % above the melting layer compared to the airborne X-band radar reflectivity data. They also miss the peak of the observed ice number distribution function for 0.1<1 mm. Even though the P3 scheme has a very different approach representing ice, it does not produce greatly different total condensed water content or better comparison to other observations in this tropical convective system. Mixed-phase microphysical processes at −10 ∘C are associated with the overprediction of liquid water content in the simulations with the Morrison and P3 schemes. The ice water content at −10 ∘C increases mainly due to the collection of liquid water by ice particles, which does not increase ice particle number but increases the mass/size of ice particles and contributes to greater simulated radar reflectivity.