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Abstract Magnetic order in most materials occurs when magnetic ions with finite moments arrange in a particular pattern below the ordering temperature. Intriguingly, if the crystal electric field (CEF) effect results in a spin-singlet ground state, a magnetic order can still occur due to the exchange interactions between neighboring ions admixing the excited CEF levels. The magnetic excitations in such a state are spin excitons generally dispersionless in reciprocal space. Here we use neutron scattering to study stoichiometric Ni 2 Mo 3 O 8 , where Ni 2+ ions form a bipartite honeycomb lattice comprised of two triangular lattices, with ions subject to the tetrahedral and octahedral crystalline environment, respectively. We find that in both types of ions, the CEF excitations have nonmagnetic singlet ground states, yet the material has magnetic order. Furthermore, CEF spin excitons from the tetrahedral sites form a dispersive diffusive pattern around the Brillouin zone boundary, likely due to spin entanglement and geometric frustrations. 

We investigate the behavior of higher-form symmetries at variousquantum phase transitions. We consider discrete 1-form symmetries, whichcan be either part of the generalized concept “categorical symmetry”(labelled as \tilde{Z}_N^{(1)} Z ̃ N ( 1 ) )introduced recently, or an explicit Z_N^{(1)} Z N ( 1 ) 1-form symmetry. We demonstrate that for many quantum phase transitionsinvolving a Z_N^{(1)} Z N ( 1 ) or \tilde{Z}_N^{(1)} Z ̃ N ( 1 ) symmetry, the following expectation value \langle \left( O_\mathcal{C}\right)^2 \rangle ⟨ ( O 𝒞 ) 2 ⟩ takes the form \langle \left( \log O_\mathcal{C} \right)^2 \rangle \sim - \frac{A}{\epsilon} P + b \log P ⟨ ( log O 𝒞 ) 2 ⟩ ∼ − A ϵ P + b log P , where O_\mathcal{C} O 𝒞 is an operator defined associated with loop \mathcal{C} 𝒞 (or its interior \mathcal{A} 𝒜 ),which reduces to the Wilson loop operator for cases with an explicit Z_N^{(1)} Z N ( 1 ) 1-form symmetry. P P is the perimeter of \mathcal{C} 𝒞 ,and the b \log P b log P term arises from the sharp corners of the loop \mathcal{C} 𝒞 ,which is consistent with recent numerics on a particular example. b b is a universal microscopic-independent number, which in (2+1)d ( 2 + 1 ) d is related to the universal conductivity at the quantum phasetransition. b b can be computed exactly for certain transitions using the dualitiesbetween (2+1)d ( 2 + 1 ) d conformal field theories developed in recent years. We also compute the"strange correlator" of O_\mathcal{C} O 𝒞 : S_{\mathcal{C}} = \langle 0 | O_\mathcal{C} | 1 \rangle / \langle 0 | 1 \rangle S 𝒞 = ⟨ 0 | O 𝒞 | 1 ⟩ / ⟨ 0 | 1 ⟩ where |0\rangle | 0 ⟩ and |1\rangle | 1 ⟩ are many-body states with different topological nature. 

One dimensional (1d) interacting systems with local Hamiltonianscan be studied with various well-developed analytical methods.Recently novel 1d physics was found numerically in systems witheither spatially nonlocal interactions, or at the 1d boundary of2d quantum critical points, and the critical fluctuation in thebulk also yields effective nonlocal interactions at the boundary.This work studies the edge states at the 1d boundary of 2dstrongly interacting symmetry protected topological (SPT) states,when the bulk is driven to a disorder-order phase transition. Wewill take the 2d Affleck-Kennedy-Lieb-Tasaki (AKLT) state as anexample, which is a SPT state protected by the SO(3) spinsymmetry and spatial translation. We found that the original(1+1)d boundary conformal field theory of the AKLT state isunstable due to coupling to the boundary avatar of the bulkquantum critical fluctuations. When the bulk is fixed at thequantum critical point, within the accuracy of our expansionmethod, we find that by tuning one parameter at the boundary,there is a generic direct transition between the long rangeantiferromagnetic Néel order and the valence bond solid (VBS)order. This transition is very similar to the Néel-VBStransition recently found in numerical simulation of a spin-1/2chain with nonlocal spatial interactions. Connections between ouranalytical studies and recent numerical results concerning theedge states of the 2d AKLT-like state at a bulk quantum phasetransition will also be discussed.