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Wu, Dezhen ; Li, Jialu ; Yao, Libo ; Xie, Rongxuan ; Peng, Zhenmeng ( , ACS Applied Materials & Interfaces)
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Yao, Libo ; King, Jaelynne ; Wu, Dezhen ; Ma, Jiayang ; Li, Jialu ; Xie, Rongxuan ; Chuang, Steven S. C. ; Miyoshi, Toshikazu ; Peng, Zhenmeng ( , Nature Communications)
Abstract The evergrowing plastic production and the caused concerns of plastic waste accumulation have stimulated the need for waste plastic chemical recycling/valorization. Current methods suffer from harsh reaction conditions and long reaction time. Herein we demonstrate a non-thermal plasma-assisted method for rapid hydrogenolysis of polystyrene (PS) at ambient temperature and atmospheric pressure, generating high yield (>40 wt%) of C1–C3hydrocarbons and ethylene being the dominant gas product (Selectivity of ethylene,
S C2H4 > 70%) within ~10 min. The fast reaction kinetics is attributed to highly active hydrogen plasma, which can effectively break bonds in polymer and initiate hydrogenolysis under mild condition. Efficient hydrogenolysis of post-consumer PS materials using this method is also demonstrated, suggesting a promising approach for fast retrieval of small molecular hydrocarbon modules from plastic materials as well as a good capability to process waste plastics in complicated conditions. -
Pan, Ying ; Bhowmick, Antara ; Wu, Wei ; Zhang, Yuan ; Diao, Yuxia ; Zheng, Aiguo ; Zhang, Chen ; Xie, Rongxuan ; Liu, Zixiao ; Meng, Jianqiang ; et al ( , ACS Catalysis)