skip to main content


Search for: All records

Creators/Authors contains: "Butch, Nicholas P."

Note: When clicking on a Digital Object Identifier (DOI) number, you will be taken to an external site maintained by the publisher. Some full text articles may not yet be available without a charge during the embargo (administrative interval).
What is a DOI Number?

Some links on this page may take you to non-federal websites. Their policies may differ from this site.

  1. Topological defects are singularities in an ordered phase that can have a profound effect on phase transitions and serve as a window into the order parameter. Examples of topological defects include dislocations in charge density waves and vortices in a superconductor or pair density wave, where the latter is a condensate of Cooper pairs with finite momentum. Here we demonstrate the role of topological defects in the magnetic-field-induced disappearance of a charge density wave in the heavy-fermion superconductor UTe2. We reveal pairs of topological defects of the charge density wave with positive and negative phase winding. The pairs are directly correlated with zeros in the charge density wave amplitude and increase in number with increasing magnetic field. A magnetic field generates vortices of the superconducting and pair density wave orders that can create topological defects in the charge density wave and induce the experimentally observed melting of this charge order at the upper critical field. Our work reveals the important role of magnetic-field-generated topological defects in the melting of the charge density wave order parameter in UTe2 and provides support for the existence of a pair density wave order on the surface. 
    more » « less
    Free, publicly-accessible full text available March 20, 2025
  2. The intense interest in triplet superconductivity partly stems from theoretical predictions of exotic excitations such as non-Abelian Majorana modes, chiral supercurrents and half-quantum vortices1–4. However, fundamentally new and unexpected states may emerge when triplet superconductivity appears in a strongly correlated system. Here we use scanning tunnelling microscopy to reveal an unusual charge-density-wave (CDW) order in the heavy-fermion triplet superconductor UTe2 (refs. 5–8). Our high-resolution maps reveal a multi-component incommensurate CDW whose intensity gets weaker with increasing field, with the CDW eventually disappearing at the superconducting critical field Hc2. To understand the phenomenology of this unusual CDW, we construct a Ginzburg–Landau theory for a uniform triplet superconductor coexisting with three triplet pair-density-wave states. This theory gives rise to daughter CDWs that would be sensitive to magnetic field owing to their origin in a pair-density-wave state and provides a possible explanation for our data. Our discovery of a CDW state that is sensitive to magnetic fields and strongly intertwined with superconductivity provides important information for understanding the order parameters of UTe2. 
    more » « less
    Free, publicly-accessible full text available June 29, 2024
  3. Abstract

    The temperature dependence of the low-energy magnetic excitations in the spin-triplet superconductor UTe2was measured via inelastic neutron scattering in the normal and superconducting states. These excitations have a peak instensity at 4 meV, follow the Brillouin zone edges near the crystallographic b-axis, obey the paramagnetic structural symmetry, and track the temperature evolution of the heavy fermion bulk magnetic susceptibility. Thus, the imaginary part of the dynamic susceptibility follows the behavior of interband correlations in a hybridized Kondo lattice with an appropriate characteristic energy. These excitations are a lower-dimensional analog of phenomena observed in other Kondo lattice materials, such that their presence is not necessarily due to dominance of ferromagnetic or antiferromagnetic correlations. The onset of superconductivity alters the magnetic excitations noticeably on the same energy scales, suggesting that these changes originate from additional electronic structure modification.

     
    more » « less
  4. Abstract

    Ba3Yb2Zn5O11is exceptional among breathing pyrochlore compounds for being in the nearly-decoupled limit where inter-tetrahedron interactions are weak, hosting isolated clusters or molecular magnet-like tetrahedra of magnetic ytterbium (Yb3+) ions. In this work, we present the study carried out on single-crystal samples of the breathing pyrochlore Ba3Yb2Zn5O11, using a variety of magnetometry and neutron scattering techniques along with theoretical modeling. We employ inelastic neutron scattering to investigate the magnetic dynamics as a function of applied field (with respect to both magnitude and direction) down to a temperature of 70 mK, where inelastic scattering reveals dispersionless bands of excitations as found in earlier powder sample studies, in good agreement with a single-tetrahedron model. However, diffuse neutron scattering at zero field and dc-susceptibility at finite field exhibit features suggesting the presence of excitations at low-energy that are not captured by the single tetrahedron model. Analysis of the local structure down to 2 K via pair distribution function analysis finds no evidence of structural disorder. We conclude that effects beyond the single tetrahedron model are important in describing the low-energy, low-temperature physics of Ba3Yb2Zn5O11, but their nature remains undetermined.

     
    more » « less
  5. null (Ed.)
    Abstract Electrical magnetoresistance and tunnel diode oscillator measurements were performed under external magnetic fields up to 41 T applied along the crystallographic b axis (hard axis) of UTe 2 as a function of temperature and applied pressures up to 18.8 kbar. In this work, we track the field-induced first-order transition between superconducting and magnetic field-polarized phases as a function of applied pressure, showing suppression of the transition with increasing pressure until the demise of superconductivity near 16 kbar and the appearance of a pressure-induced ferromagnetic-like ground state that is distinct from the field-polarized phase and stable at zero field. Together with evidence for the evolution of a second superconducting phase and its upper critical field with pressure, we examine the confinement of superconductivity by two orthogonal magnetic phases and the implications for understanding the boundaries of triplet superconductivity. 
    more » « less