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Gas-phase molecules in cometary atmospheres (comae) originate primarily from (1) outgassing by the nucleus, (2) sublimation of icy grains in the near-nucleus coma, and (3) coma (photo)chemical processes. However, the majority of cometary gases observed at radio wavelengths have yet to be mapped, so their production/release mechanisms remain uncertain. Here we present observations of six molecular species toward comet 46P/Wirtanen, obtained using the Atacama Large Millimeter/submillimeter Array during the comet’s unusually close (∼0.1 au) approach to Earth in 2018 December. Interferometric maps of HCN, CH₃OH, CH₃CN, H₂CO, CS, and HNC were obtained at an unprecedented sky-projected spatial resolution of up to 25 km, enabling the nucleus and coma sources of these molecules to be accurately quantified. The HCN, CH₃OH, and CH₃CN spatial distributions are consistent with production by direct outgassing from (or very close to) the nucleus, with a significant proportion of the observed CH₃OH originating from sublimation of icy grains in the near-nucleus coma (at a scale lengthL_p= 36 ± 7 km). On the other hand, H₂CO, CS, and HNC originate primarily from distributed coma sources (withL_pvalues in the range 550–16,000 km), the identities of which remain to be established. The HCN, CH₃OH, and HNC abundances in 46P are consistent with the average values previously observed in comets, whereas the H₂CO, CH₃CN, and CS abundances are relatively low.

The coma of comet C/2016 R2 (PanSTARRS) is one of the most chemically peculiar ever observed, in particular due to its extremely high CO/H₂O and${\mathrm{N}}_2^{+}$/H₂O ratios, and unusual trace volatile abundances. However, the complex shape of its CO emission lines, as well as uncertainties in the coma structure and excitation, has lead to ambiguities in the total CO production rate. We performed high-resolution, spatially, spectrally, and temporally resolved CO observations using the James Clerk Maxwell Telescope and Submillimeter Array to elucidate the outgassing behavior of C/2016 R2. Results are analyzed using a new, time-dependent, three-dimensional radiative transfer code (SUBlimating gases in LIME; SUBLIME, based on the open-source version of the LIne Modeling Engine), incorporating for the first time, accurate state-to-state collisional rate coefficients for the CO–CO system. The total CO production rate was found to be in the range of (3.8 − 7.6) × 10²⁸s⁻¹between 2018 January 13 and February 1 (atr_H= 2.8–2.9 au), with a mean value of (5.3 ± 0.6) × 10²⁸s⁻¹. The emission is concentrated in a near-sunward jet, with a half-opening angle of ∼62° and an outflow velocity of 0.51 ± 0.01 km s⁻¹, compared to 0.25 ± 0.01 km s⁻¹in the ambient (and nightside) coma. Evidence was also found for an extended source of CO emission, possibly due to icy grain sublimation around 1.2 × 10⁵km from the nucleus. Based on the coma molecular abundances, we propose that the nucleus ices of C/2016 R2 can be divided into a rapidly sublimating apolar phase, rich in CO, CO₂, N₂, and CH₃OH, and a predominantly frozen (or less abundant), polar phase containing more H₂O, CH₄, H₂CO, and HCN.