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In the realm of quantum information processing, harnessing high-dimensional photonic systems provides a pathway to overcome limitations of traditional two-level systems. Orbital angular momentum (OAM) of light has emerged as a powerful tool for creating and manipulating high-dimensional entanglement, promising increased information capacity and enhanced security in quantum communication protocols. However, conventional methods like spontaneous parametric downconversion encounter challenges due to non-uniform production rates of Laguerre–Gaussian modes. This study explores the potential of spontaneous four-wave mixing in ring-core fibers (RCFs) as a viable platform for generating OAM photon pairs with tailored spectral and spatial properties. We show that by controlling the topological charge of pump photons, correlated, uncorrelated, and anti-correlated photon pairs can be engineered across arbitrary spectral ranges, essential for diverse quantum applications. Experimental noise characterization of the RCF-based source demonstrates a high coincidence-to-accidental ratio exceeding 4000, and a low heralded second-order correlation function (g_H⁽²⁾<0.005), which confirms its operation well into the single-photon regime. This work demonstrates the potential of RCFs as a versatile platform for generating structured photon pairs, paving the way for future high-dimensional quantum communication and information processing applications. 

Developing a quantum light source that carries more than one bit per photon is pivotal for expanding quantum information applications. Characterizing a high-dimensional multiple-degree-of-freedom source at the single-photon level is challenging due to the large parameter space as well as limited emission rates and detection efficiencies. Here, we characterize photon pairs generated in optical fiber in the transverse-mode and frequency degrees of freedom by applying stimulated emission in both degrees of freedom while detecting in one of them at a time. This method may be useful in the quantum state estimation and optimization of various photon-pair source platforms in which complicated correlations across multiple degrees of freedom may be present. 

Broadband quantum memory is critical to enabling the operation of emerging photonic quantum technology at high speeds. Here we review a central challenge to achieving broadband quantum memory in atomic ensembles—what we call the ‘linewidth-bandwidth mismatch’ problem—and the relative merits of various memory protocols and hardware used for accomplishing this task. We also review the theory underlying atomic ensemble quantum memory and its extensions to optimizing memory efficiency and characterizing memory sensitivity. Finally, we examine the state-of-the-art performance of broadband atomic ensemble quantum memories with respect to three key metrics: efficiency, memory lifetime, and noise. 

The purpose of this tutorial paper is to present a broad overview of photon-pair generation through the spontaneous four wave mixing (SFWM) process in optical fibers. Progress in optical fiber technology means that today we have at our disposal a wide variety of types of fiber, which, together with the fact that SFWM uses two pump fields, implies a truly remarkable versatility in the resulting possible photon-pair properties. We discuss how the interplay of frequency, transverse mode, and polarization degrees of freedom—the first linked to the latter two through fiber dispersion—leads to interesting entanglement properties both in individual degrees of freedom and also permitting hybrid and hyper entanglement in combinations of degrees of freedom. This tutorial covers methods for photon-pair factorability, frequency tunability, and SFWM bandwidth control, the effect of frequency non-degenerate and counterpropagating pumps, as well as methods for characterizing photon pairs generated in optical fibers. 

We measure 95.6±0.3% storage efficiency of ultrafast photons in a collisionally broadened barium vapor quantum memory. We measure 31±1% total efficiency, limited by control field power, and a 0.515(6) ns lifetime, limited by motional dephasing. 

We present our experimental results on generating photon pairs entangled in a transverse-mode Bell state in few-mode optical fiber by controlling the transverse mode of the pump to selectively excite spontaneous four-wave mixing processes. 

We examine the sensitivity of Λ-type optical quantum memories to experimental fluctuations using a variance-based analysis. The results agree with physical interpretations of quantum memory protocols, and are important for practical implementations.