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Planar alignment of disc‐like nanomaterials is required to transfer their superior anisotropic properties from microscopic individual structures to macroscopic collective assemblies. However, such alignment by electrical or magnetic field is challenging due to their additional degrees of orientational freedom compared to that of rod‐like nanostructures. Here, the realization of planar alignment of suspended graphene sheets using a rotating magnetic field produced by a pair of small NdFeB magnets and subsequent demonstration of high optical anisotropy and potential novel device applications is reported. Compared to partially aligned sheets with a static magnetic field, planar aligned graphene suspensions exhibit a near‐perfect order parameter, much higher birefringence and anisotropic absorption/transmission. A unique feature of discotic nanomaterial assemblies is that the observed order parameter and optical property can vary from isotropic to partial and complete alignment depending on the experimental configuration. By immobilizing and patterning aligned graphene in a UV‐curable polymer resin, we further demonstrated an all‐graphene permanent display, which exhibits wide‐angle, high dark‐bright contrast in either transmission or reflection mode without any polarizing optics. The ability to control and pattern graphene orientation in all three dimensions opens up new exploration and broad device applications of graphene.

The Brillouin instability (BI) caused by stimulated Brillouin scattering (SBS) can limit the output power of high-energy laser amplifiers. Pseudo-random bitstream (PRBS) phase modulation is an effective modulation technique to suppress BI. In this paper, we study the impact of the PRBS order and modulation frequency on the BI threshold for different Brillouin linewidths. PRBS phase modulation with a higher order will break the power into a larger number of frequency tones with a lower maximum power in each tone, leading to a higher BI threshold and a smaller tone spacing. However, the BI threshold may saturate when the tone spacing in the power spectra approaches the Brillouin linewidth. For a given Brillouin linewidth, our results allow us to determine the order of PRBS beyond which there is no further improvement in the threshold. When a specific threshold power is desired, the minimum PRBS order required decreases as the Brillouin linewidth increases. When the PRBS order is too large, the BI threshold deteriorates, and this deterioration occurs at smaller PRBS orders as the Brillouin linewidth increases. We investigate the dependence of the optimal PRBS order on the averaging time and fiber length, and we did not find a significant dependence. We also derive a simple equation that relates the BI threshold for different PRBS orders. Hence, the increase in BI threshold using an arbitrary order PRBS phase modulation may be predicted using the BI threshold from a lower PRBS order, which is computationally less time-consuming to compute.

The Brillouin instability (BI) due to stimulated Brillouin scattering (SBS) and the transverse (thermal) mode instability (TMI) due to stimulated thermal Rayleigh scattering (STRS) limit the achievable power in high-power lasers and amplifiers. The pump power threshold for BI increases as the core diameter increases, but the threshold for TMI may decrease as the core diameter increases. In this paper, we use a multi-time-scale approach to simultaneously model BI and TMI, which gives us the ability to find the fiber diameter with the highest power threshold. We formulate the equations to compare the thresholds of the combined and individual TMI and BI models. At the pump power threshold and below, there is a negligible difference between the full and individual models, as BI and TMI are not strong enough to interact with each other. The highest pump threshold occurs at the optimal core size of 43µm for the simple double-clad geometry that we considered. We found that both effects contribute equally to the threshold, and the full BI and TMI model yields a similar threshold as the BI or TMI model alone. However, once the reflectivity is sufficiently large, we find in the full BI and TMI model that BI may trigger TMI and reduce the TMI threshold to a value lower than is predicted in simulations with TMI alone. This result cannot be predicted by models that consider BI and TMI separately. Our approach can be extended to more complex geometries and used for their optimization.