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Award ID contains: 2103689

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  1. ; ; ; (, Physical Review Research)
    We report the suppression of nucleation in the nonphotochemical laser-induced nucleation of supersaturated aqueous potassium chloride solutions when the system pressure is above ambient pressure. The crystal yield at 51.7 bar is reduced to 5% of its value at 1 bar, and the crystal number dependence on pressure fits well to a semiempirical model based on the impurity-heating mechanism and the adiabatic compression of an ideal gas nanobubble. Our results complement recent findings by Barber and Alexander [] using high-speed imaging of bubbles preceding the observation of cesium chloride crystals. Together, these two studies provide compelling evidence for the impurity-heating mechanism. 
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    Free, publicly-accessible full text available October 1, 2026
  2. ; (, Crystal Growth & Design)
  3. ; ; ; (, Crystal Growth & Design)