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Abstract The mechanism of unconventional superconductivity in correlated materials remains a great challenge in condensed matter physics. The recent discovery of superconductivity in infinite-layer nickelates, as an analog to high-Tccuprates, has opened a new route to tackle this challenge. By growing 8 nm Pr0.8Sr0.2NiO2films on the (LaAlO3)0.3(Sr2AlTaO6)0.7substrate, we successfully raise the superconducting onset transition temperatureTcin the widely studied SrTiO3-substrated nickelates from 9 K into 15 K, which indicates compressive strain is an efficient protocol to further enhance superconductivity in infinite-layer nickelates. Additionally, the x-ray absorption spectroscopy, combined with the first-principles and many-body simulations, suggest a crucial role of the hybridization between Ni and O orbitals in the unconventional pairing. These results also suggest the increase ofTcbe driven by the change of charge-transfer nature that would narrow the origin of general unconventional superconductivity in correlated materials to the covalence of transition metals and ligands.more » « less
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Ultrafast optical spectroscopy is an effective experimental technique for accessing electronic and atomic motions in materials at their fundamental timescales and studying their responses to external perturbations. Despite the important insights that ultrafast techniques can provide on the microscopic physics of solids, undergraduate students' exposure to this area of research is still limited. In this article, we describe an ultrafast optical pump-probe spectroscopy experiment for the advanced undergraduate instructional laboratory, in which students can measure coherently excited vibrations of the crystal lattice and connect their observations to the microscopic properties of the investigated materials. We designed a simple table-top apparatus based on a commercial Er-fiber oscillator emitting 50-fs pulses at 1560 nm and at 100 MHz repetition rate. We split the output into two beams, using one of them as an intense “pump” to coherently excite phonons in selected crystals, and the other as a weaker, delayed “probe” to measure the transient reflectivity changes induced by the pump. We characterize the ultrafast laser pulses via intensity autocorrelation measurements and detect coherent phonon oscillations in the reflectivity of Bi, Sb, and 1T-TaS2. We then discuss the oscillation amplitude, frequency, and damping in terms of microscopic properties of these systems.more » « less
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The stability of the spin polaron quasiparticle, well established in studies of a single hole in the 2D antiferromagnets, is investigated in the 1D antiferromagnets using at -J model. We perform an exact slave fermion transformation to the holon-magnon basis, and diagonalize numerically the resulting model in the presence of a single hole. We demonstrate that the spin polaron collapses - and the spin-charge separation takes over - due to the specific role played by the magnon-magnon interactions and the magnon hard-core constraint in the 1Dt -J model. Moreover, we prove that the spin polaron is stable for any strength of the magnon-magnon interaction other than the unique value found in a 1D antiferromagnet with the continuous symmetry of the spin interactions. Fine-tuning to this unique value is extremely unlikely to occur in quasi-1D antiferromagnets, therefore the spin polaron is the stable quasiparticle of realistic 1D materials. Our results lead to a new interpretation of the ARPES spectra of quasi-1D antiferromagnets in the spin polaron language.more » « less
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Abstract This paper presents a roadmap to the application of AI techniques and big data (BD) for different modelling, design, monitoring, manufacturing and operation purposes of different superconducting applications. To help superconductivity researchers, engineers, and manufacturers understand the viability of using AI and BD techniques as future solutions for challenges in superconductivity, a series of short articles are presented to outline some of the potential applications and solutions. These potential futuristic routes and their materials/technologies are considered for a 10–20 yr time-frame.more » « less
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Abstract In high-temperature ( T c ) cuprate superconductors, many exotic phenomena are rooted in the enigmatic pseudogap state, which has been interpreted as consisting of preformed Cooper pairs or competing orders or a combination thereof. Observation of pseudogap phenomenologically in electron-doped Sr 2 IrO 4 —the 5d electron counterpart of the cuprates, has spurred intense interest in the strontium iridates as a testbed for exploring the exotic physics of the cuprates. Here, we examine the pseudogap state of electron-doped Sr 2 IrO 4 by angle-resolved photoemission spectroscopy (ARPES) and parallel theoretical modeling. Our analysis demonstrates that the pseudogap state of Sr 2 IrO 4 appears without breaking the particle–hole symmetry or inducing spectral broadening which are telltale signatures of competing orders in the cuprates. We find quasiparticle dispersion and its temperature dependence in the pseudogap state of Sr 2 IrO 4 to point to an electronic order with a zero scattering wave vector and limited correlation length. Particle–hole symmetric preformed Cooper pairs are discussed as a viable mechanism for such an electronic order. The potential roles of incommensurate density waves are also discussed.more » « less
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