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Abstract The sub‐Terahertz and Terahertz bands play a critical role in next‐generation wireless communication and sensing technologies, thanks to the large amount of available bandwidth in this spectral regime. While long‐wavelength (microwave to mm‐Wave) and short‐wavelength (near‐infrared to ultraviolet) devices are well‐established and studied, the sub‐THz to THz regime remains relatively underexplored and underutilized. Traditional approaches used in the aforementioned spectral regions are more difficult to replicate in the THz band, leading to the need for the development of novel devices and structures that can manipulate THz radiation effectively. Herein a novel organic, solid‐state electrochemical device is presented, capable of achieving modulation depths of over 90% from ≈500 nm of a conducting polymer that switches conductivity over a large dynamic range upon application of an electronically controllable external bias. The stability of such devices under long‐term, repeated voltage switching, as well as continuous biasing at a single voltage, is also explored. Switching stabilities and long‐term bias stabilities are achieved over two days for both use cases. Additionally, both depletion mode (always “ON”) and accumulation mode (always “OFF”) operation are demonstrated. These results suggest applications of organic electrochemical THz modulators in large area and flexible implementations. 

Owing to the substantial bandwidth they offer, the exploration of  100+ GHz frequencies for wireless communications has surged in recent years. These sub-Terahertz channels are susceptible to blockage, which makes reflected paths crucial for seamless connectivity. However, at such high frequencies, reflections deviate from the known mirror-like specular behavior as the signal wavelength becomes comparable to the height perturbation at the surface of the reflectors. Such reflectors are considered electromagnetically "rough" which results in random non-specular reflection components that are not well understood. In this dataset, we present experimental results on the impact of rough scattering on over-the-air data links as well as the characteristics of ultra-broadband THz reflection response.