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A range of ultrasonic techniques associated with the nondestructive evaluation of metals involves the propagation of low-frequency elastic waves. Metals that are isotropic and homogeneous in the macroscopic length scale contain elastic heterogeneities, such as grain boundaries within the microstructures. Ultrasonic waves propagating through such microstructures get scattered from the grain boundaries. As a result, the propagating ultrasound attenuates. The mass density and the elastic anisotropy in each constituent grain govern the degree of heterogeneity in the polycrystalline aggregates. Existing elastodynamic models consider first-order scattering effects from grain boundaries. This paper presents the improved attenuation formulae, for the first time, by including the next order of grain scattering effects. Results from investigating 759 polycrystals reveal a positive correlation between the effects of higher-order scattering from grain boundaries and the degree of heterogeneity. Thus, higher-order grain scattering effects are now known. These results motivate further investigation into higher frequencies and strongly scattering alloys in the future.