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Abstract The thermal Hall effect recently provided intriguing probes to the ground state of exotic quantum matters. These observations of transverse thermal Hall signals lead to the debate on the fermionic versus bosonic origins of these phenomena. The recent report of quantum oscillations (QOs) in Kitaev spin liquid points to a possible resolution. The Landau level quantization would most likely capture only the fermionic thermal transport effect. However, the QOs in the thermal Hall effect are generally hard to detect. In this work, we report the observation of a large oscillatory thermal Hall effect of correlated Kagome metals. We detect a 180-degree phase change of the oscillation and demonstrate the phase flip as an essential feature for QOs in the thermal transport properties. More importantly, the QOs in the thermal Hall channel are more profound than those in the electrical Hall channel, which strongly violates the Wiedemann–Franz (WF) law for QOs. This result presents the oscillatory thermal Hall effect as a powerful probe to the correlated quantum materials.more » « less
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Abstract Metals with kagome lattice provide bulk materials to host both the flat-band and Dirac electronic dispersions. A new family of kagome metals is recently discovered inAV6Sn6. The Dirac electronic structures of this material needs more experimental evidence to confirm. In the manuscript, we investigate this problem by resolving the quantum oscillations in both electrical transport and magnetization in ScV6Sn6. The revealed orbits are consistent with the electronic band structure models. Furthermore, the Berry phase of a dominating orbit is revealed to be aroundπ, providing direct evidence for the topological band structure, which is consistent with calculations. Our results demonstrate a rich physics and shed light on the correlated topological ground state of this kagome metal.more » « less
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Although electro-optic (EO) nonlinearities are essential for many quantum and classical photonics applications, a major challenge is inefficient modulation in cryogenic environments. Guided by the connection between phase transitions and nonlinearity, we identify the quantum paraelectric perovskite SrTiO3as a strong cryogenic EO [>500 picometers per volt (pm/V)] and piezo-electric material (>90 picocoulombs per newton) atT= 5 K, at frequencies to at least 1 megahertz. Furthermore, by tuning SrTiO3toward quantum criticality, we more than double the EO and piezo-electric effects, demonstrating a linear Pockels coefficient above 1000 pm/V. Our results probe the link between quantum phase transitions, dielectric susceptibility, and nonlinearity, unlocking opportunities in cryogenic optical and mechanical systems and providing a framework for discovering new nonlinear materials.more » « lessFree, publicly-accessible full text available October 23, 2026
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Free, publicly-accessible full text available October 1, 2026
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The spin- kagome Heisenberg antiferromagnets are believed to host exotic quantum entangled states. Recently, the reports of magnetization plateau and magnetic oscillations in a kagome antiferromagnet (YCOB) have made this material a promising candidate for experimentally realizing quantum spin liquid states. Here, we present measurements of the specific heat in YCOB in high magnetic fields (up to 41.5 T) down to 0.46 K, and the plateau feature has been confirmed. Moreover, the temperature dependence of in the vicinity of plateau region can be fitted by a linear in term which indicates the presence of a Dirac spectrum, together with a constant term, which indicates a finite density of states contributed by other spinon Fermi surfaces. Surprisingly, the constant term is highly anisotropic in the direction of the magnetic field. Additionally, we observe a double-peak feature near 30 T above the plateau which is another hallmark of fermionic excitations in the specific heat. This combination of gapless behavior and the double-peak structure strongly suggests that the plateau in YCOB is nontrivial and hosts fermionic quasiparticles.more » « lessFree, publicly-accessible full text available May 1, 2026
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