skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Title: Electron-phonon instability in graphene revealed by global and local noise probes
Understanding and controlling nonequilibrium electronic phenomena is an outstanding challenge in science and engineering. By electrically driving ultraclean graphene devices out of equilibrium, we observe an instability that is manifested as substantially enhanced current fluctuations and suppressed conductivity at microwave frequencies. Spatial mapping of the nonequilibrium current fluctuations using nanoscale magnetic field sensors reveals that the fluctuations grow exponentially along the direction of carrier flow. Our observations, including the dependence on density and temperature, are consistently explained by the emergence of an electron-phonon Cerenkov instability at supersonic drift velocities. These results offer the opportunity for tunable terahertz generation and active phononic devices based on two-dimensional materials.  more » « less
Award ID(s):
1734011
PAR ID:
10096595
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ;
Date Published:
Journal Name:
Science
ISSN:
1095-9203
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Coupling between chemical fuel consumption and phase separation can lead to condensation at a nonequilibrium steady state, resulting in phase behaviors that are not described by equilibrium thermodynamics. Theoretical models of such “chemically driven fluids” typically invoke near-equilibrium approximations at small length scales. However, because dissipation occurs due to both molecular-scale chemical reactions and mesoscale diffusive transport, it has remained unclear which properties of phase-separated reaction–diffusion systems can be assumed to be at an effective equilibrium. Here, we use microscopic simulations to show that mesoscopic fluxes are dependent on nonequilibrium fluctuations at phase-separated interfaces. We further develop a first-principles theory to predict nonequilibrium coexistence curves, localization of mesoscopic fluxes near phase-separated interfaces, and droplet size-scaling relations in good agreement with simulations. Our findings highlight the central role of interfacial properties in governing nonequilibrium condensation and have broad implications for droplet nucleation, coarsening, and size control in chemically driven fluids. 
    more » « less
  2. Abstract We perform a statistical analysis of observed magnetic spectra in the solar wind at 1 au with localized power elevations above the level of the ambient turbulent fluctuations. We show that the elevations are seen only when the intensity of the ambient fluctuations is sufficiently low. Assuming that the spectral elevations are caused by thermal-ion instabilities, this suggests that on average the effect of the solar wind background is strong enough to suppress the instability or obscure it or both. We then carry out nonlinear numerical simulations with particle ions and an electron fluid to model a thermal-ion instability coexisting with an ambient turbulence. The parameters of the simulation are taken from a known solar wind interval where an instability was assumed to exist based on the linear theory and a bi-Maxwellian fit of the observed distribution with core and secondary-beam protons. The numerical model closely matches the position of the observed spectral elevation in the wavenumber space. This confirms that the thermal-ion instability is responsible for the elevation. At the same time, the magnitude of the elevation turns out to be smaller than in the real solar wind. When higher intensity of the turbulence is used in the simulation, which is typical of solar wind in general, the power elevation is no longer seen. This is in agreement with the reduced observability of the elevations at higher intensities. However, the simulations show that the turbulence does not simply obscure the instability but also lowers its saturation level. 
    more » « less
  3. Abstract Direct printing of functional materials, structures, and devices on various platforms such as flexible to rigid substrates is of interest for applications ranging from electronics to energy and sensing to biomedical devices. Current additive manufacturing (AM) and printing processes are either limited by the available sources of functional materials or require to be in the form of precisely designed inks. Here, a novel laser‐based additive nanomanufacturing (ANM) system capable of in situ and on‐demand generations of nanoparticles that can serve as nanoscale building blocks for real‐time sintering and dry printing a variety of multifunctional materials and patterns at atmospheric pressure and room temperature is reported. The ability to print different functional materials on various rigid and flexible platforms is shown. This nonequilibrium process involves pulsed laser ablation of targets and in situ formation of pure amorphous nanoparticles’ stream that are guided through a nozzle onto the surface of the substrate, where they are sintered/crystallized in real‐time. Further, the process–structure relationship of the printed materials from nanoscale to microscale is shown. This new ANM concept opens up an opportunity for printing advanced functional materials and devices on rigid and flexible substrates that can be employed both on the earth and in space. 
    more » « less
  4. Popularization of the Internet-of-Things (IoT) has brought widespread concerns on IoT security, especially in face of several recent security incidents related to IoT devices. Due to the resource-constrained nature of many IoT devices, security offloading has been proposed to provide good-enough security for IoT with minimum overhead on the devices. In this paper, we investigate the inevitable risk associated with security offloading: the unprotected and unmonitored transmission from IoT devices to the offloaded security mechanisms. An important challenge in modeling the security risk is the dynamic nature of IoT due to demand fluctuations and infrastructure instability. We propose a stochastic model to capture both the expected and worst-case security risks of an IoT system. We then propose a framework to efficiently address the optimal robust deployment of security mechanisms in IoT. We use results from extensive simulations to demonstrate the superb performance and efficiency of our approach compared to several other algorithms. 
    more » « less
  5. Visco-resistive magnetohydrodynamic turbulence, driven by a two-dimensional unstable shear layer that is maintained by an imposed body force, is examined by decomposing it into dissipationless linear eigenmodes of the initial profiles. The down-gradient momentum flux, as expected, originates from the large-scale instability. However, continual up-gradient momentum transport by large-scale linearly stable but nonlinearly excited eigenmodes is identified, and found to nearly cancel the down-gradient transport by unstable modes. The stable modes effectuate this by depleting the large-scale turbulent fluctuations via energy transfer to the mean flow. This establishes a physical mechanism underlying the long-known observation that coherent vortices formed from nonlinear saturation of the instability reduce turbulent transport and fluctuations, as such vortices are composed of both the stable and unstable modes, which are nearly equal in their amplitudes. The impact of magnetic fields on the nonlinearly excited stable modes is then quantified. Even when imposing a strong magnetic field that almost completely suppresses the instability, the up-gradient transport by the stable modes is at least two-thirds of the down-gradient transport by the unstable modes, whereas for weaker fields, this fraction reaches up to 98% . These effects are persistent with variations in magnetic Prandtl number and forcing strength. Finally, continuum modes are shown to be energetically less important, but essential for capturing the magnetic fluctuations and Maxwell stress. A simple analytical scaling law is derived for their saturated turbulent amplitudes. It predicts the fall-off rate as the inverse of the Fourier wavenumber, a property which is confirmed in numerical simulations. 
    more » « less