Abstract Diamond has attracted great interest as an appealing material for various applications ranging from classical to quantum optics. To date, Raman lasers, single photon sources, quantum sensing and quantum communication have been demonstrated with integrated diamond devices. However, studies of the nonlinear optical properties of diamond have been limited, especially at the nanoscale. Here, a metasurface consisting of plasmonic nanogap cavities is used to enhance both χ (2) and χ (3) nonlinear optical processes in a wedge-shaped diamond slab with a thickness down to 12 nm. Multiple nonlinear processes were enhanced simultaneously due to the relaxation of phase-matching conditions in subwavelength plasmonic structures by matching two excitation wavelengths with the fundamental and second-order modes of the nanogap cavities. Specifically, third-harmonic generation (THG) and second-harmonic generation (SHG) are both enhanced 1.6 × 10 7 -fold, while four-wave mixing is enhanced 3.0 × 10 5 -fold compared to diamond without the metasurface. Even though diamond lacks a bulk χ (2) due to centrosymmetry, the observed SHG arises from the surface χ (2) of the diamond slab and is enhanced by the metasurface elements. The efficient, deeply subwavelength diamond frequency converter demonstrated in this work suggests an approach for conversion of color center emission to telecom wavelengths directly in diamond.
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Phase-matched nonlinear second-harmonic generation in plasmonic metasurfaces
Abstract The phase matching between the propagating fundamental and nonlinearly generated waves plays an important role in the efficiency of the nonlinear frequency conversion in macroscopic crystals. However, in nanoscale samples, such as nanoplasmonic structures, the phase-matching condition is often ignored due to the sub-wavelength nature of the materials. Here, we first show that the phase matching of the lattice plasmon modes at the fundamental and second-harmonic frequencies in a plasmonic nanoantenna array can effectively enhance the surface-enhanced second-harmonic generation. Additionally, a significant enhancement of the second-harmonic generation is demonstrated using stationary band-edge lattice plasmon modes with zero phase.
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- Award ID(s):
- 1741691
- NSF-PAR ID:
- 10123404
- Date Published:
- Journal Name:
- Nanophotonics
- Volume:
- 8
- Issue:
- 4
- ISSN:
- 2192-8614
- Page Range / eLocation ID:
- 607 to 612
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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Abstract Quadratic optical parametric processes form the foundation for various applications related to classical and quantum frequency conversion, and have attracted significant interest recently in on‐chip implementation. These processes rely on phase matching among the interacting guided modes, and refractive index engineering is a primary approach for this purpose. Unfortunately, modal phase‐matching approaches developed so far only produce parametric generation with fairly low efficiencies, due to the intrinsic modal mismatch of spatial symmetries. Here, a universal design and operation principle is proposed for highly efficient optical parametric generation on integrated photonic platforms. By breaking the spatial symmetry of the optical nonlinearity of the device, nonlinear parametric interactions can be dramatically enhanced. This principle is then employed to design and fabricate a heterogeneous titanium oxide/lithium niobate nanophotonic waveguide that is able to offer second‐harmonic generation with a theoretical normalized conversion efficiency as high as 2900, which enables the measurement of an experimental efficiency of 650, significantly beyond the reach of conventional modal phase‐matching approaches. Unlike nonlinearity domain engineering that is material selective, the proposed operation principle can be flexibly applied to any other on‐chip quadratic nonlinear platform, to support ultra‐highly efficient optical parametric generation.
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Abstract Optical second harmonic generation (SHG) is a nonlinear optical effect widely used for nonlinear optical microscopy and laser frequency conversion. Closed-form analytical solution of the nonlinear optical responses is essential for evaluating materials whose optical properties are unknown a priori. A recent open-source code, ♯SHAARP.
si , can provide such closed form solutions for crystals with arbitrary symmetries, orientations, and anisotropic properties at asingle interface. However, optical components are often in the form of slabs, thin films on substrates, and multilayer heterostructures with multiple reflections of both the fundamental and up to ten different SHG waves at each interface, adding significant complexity. Many approximations have therefore been employed in the existing analytical approaches, such as slowly varying approximation, weak reflection of the nonlinear polarization, transparent medium, high crystallographic symmetry, Kleinman symmetry, easy crystal orientation along a high-symmetry direction, phase matching conditions and negligible interference among nonlinear waves, which may lead to large errors in the reported material properties. To avoid these approximations, we have developed an open-source package named Second Harmonic Analysis of Anisotropic Rotational Polarimetry in Multilayers (♯SHAARP.ml ). The reliability and accuracy are established by experimentally benchmarking with both the SHG polarimetry and Maker fringes using standard and commonly used nonlinear optical materials as well as twisted 2-dimensional heterostructures. -
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High-fidelity periodic poling over long lengths is required for robust, quasi-phase-matched second-harmonic generation using the fundamental, quasi-TE polarized waveguide modes in a thin-film lithium niobate (TFLN) waveguide. Here, a shallow-etched ridge waveguide is fabricated in x-cut magnesium oxide doped TFLN and is poled accurately over 5 mm. The high fidelity of the poling is demonstrated over long lengths using a non-destructive technique of confocal scanning second-harmonic microscopy. We report a second-harmonic conversion efficiency of up to 939 %.W−1(length-normalized conversion efficiency 3757 %.W−1.cm−2), measured at telecommunications wavelengths. The device demonstrates a narrow spectral linewidth (1 nm) and can be tuned precisely with a tuning characteristic of 0.1 nm/°C, over at least 40 °C without measurable loss of efficiency.
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null (Ed.)Abstract We experimentally demonstrate the spatial self-cleaning of a highly multimode optical beam, in the process of second-harmonic generation in a quadratic nonlinear potassium titanyl phosphate crystal. As the beam energy grows larger, the output beam from the crystal evolves from a highly speckled intensity pattern into a single, bell-shaped spot, sitting on a low energy background. We demonstrate that quadratic beam cleanup is accompanied by significant self-focusing of the fundamental beam, for both positive and negative signs of the linear phase mismatch close to the phase-matching condition.more » « less
- Free Publicly Accessible Full Text
-
Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1515/nanoph-2018-0181
