Light elements in Earth’s core play a key role in driving convection and influencing geodynamics, both of which are crucial to the geodynamo. However, the thermal transport properties of iron alloys at high-pressure and -temperature conditions remain uncertain. Here we investigate the transport properties of solid hexagonal close-packed and liquid Fe-Si alloys with 4.3 and 9.0 wt % Si at high pressure and temperature using laser-heated diamond anvil cell experiments and first-principles molecular dynamics and dynamical mean field theory calculations. In contrast to the case of Fe, Si impurity scattering gradually dominates the total scattering in Fe-Si alloys with increasing Si concentration, leading to temperature independence of the resistivity and less electron–electron contribution to the conductivity in Fe-9Si. Our results show a thermal conductivity of ∼100 to 110 W⋅m −1 ⋅K −1 for liquid Fe-9Si near the topmost outer core. If Earth’s core consists of a large amount of silicon (e.g., > 4.3 wt %) with such a high thermal conductivity, a subadiabatic heat flow across the core–mantle boundary is likely, leaving a 400- to 500-km-deep thermally stratified layer below the core–mantle boundary, and challenges proposed thermal convection in Fe-Si liquid outer core.
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Regional stratification at the top of Earth's core due to core–mantle boundary heat flux variations
Earth’s magnetic field is generated by turbulent motion in its fluid outer core. Although the bulk of the outer core is vigorously convecting and well mixed, some seismic, geomagnetic and geodynamic evidence suggests that a global stably stratified layer exists at the top of Earth’s core. Such a layer would strongly influence thermal, chemical and momentum exchange across the core–mantle boundary and thus have important implications for the dynamics and evolution of the core. Here we argue that the relevant scenario is not global stratification, but rather regional stratification arising solely from the lateral variations in heat flux at the core–mantle boundary. Using our extensive suite of numerical simulations of the dynamics of the fluid core with het- erogeneous core–mantle boundary heat flux, we predict that thermal regional inversion layers extend hundreds of kilometres into the core under anomalously hot regions of the lowermost mantle. Although the majority of the outermost core remains actively convecting, sufficiently large and strong regional inversion layers produce a one-dimensional temperature profile that mimics a globally stratified layer below the core–mantle boundary—an apparent thermal stratification despite the average heat flux across the core–mantle boundary being strongly superadiabatic.
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- Award ID(s):
- 1853196
- NSF-PAR ID:
- 10137699
- Date Published:
- Journal Name:
- Nature geoscience
- ISSN:
- 1752-0894
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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SUMMARY The Earth’s magnetic field is generated by a dynamo in the outer core and is crucial for shielding our planet from harmful radiation. Despite the established importance of the core–mantle boundary (CMB) heat flux as driver for the dynamo, open questions remain about how heat flux heterogeneities affect the magnetic field. Here, we explore the distribution of the CMB heat flux on Earth and its changes over time using compressible global 3-D mantle convection models in the geodynamic modelling software ASPECT. We discuss the use of the consistent boundary flux method as a tool to more accurately compute boundary heat fluxes in finite element simulations and the workflow to provide the computed heat flux patterns as boundary conditions in geodynamo simulations. Our models use a plate reconstruction throughout the last 1 billion years—encompassing the complete supercontinent cycle—to determine the location and sinking speed of subducted plates. The results show how mantle upwellings and downwellings create localized heat flux anomalies at the CMB that can vary drastically over Earth’s history and depend on the properties and evolution of the lowermost mantle as well as the surface subduction zone configuration. The distribution of hot and cold structures at the CMB changes throughout the supercontinent cycle in terms of location, shape and number, indicating that these structures fluctuate and might have looked very differently in Earth’s past. We estimate the resulting amplitude of spatial heat flux variations, expressed by the ratio of peak-to-peak amplitude to average heat flux, q*, to be at least 2. However, depending on the material properties and the adiabatic heat flux out of the core, q* can easily reach values >30. For a given set of material properties, q* generally varies by 30–50 per cent over time. Our results have implications for understanding the Earth’s thermal evolution and the stability of its magnetic field over geological timescales. They provide insights into the potential effects of the mantle on the magnetic field and pave the way for further exploring questions about the nucleation of the inner core and the past state of the lowermost mantle.
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unknown (Ed.)The Earth’s core–mantle boundary presents a dramatic change in materials, from silicate to metal. While little is known about chemical interactions between them, a thin layer with a lower velocity has been proposed at the topmost outer core (Eʹ layer) that is difficult to explain with a change in concentration of a single light element. Here we perform high-temperature and -pressure laser-heated diamond-anvil cell experiments and report the formation of SiO2 and FeHx from a reaction between water from hydrous minerals and Fe–Si alloys at the pressure–temperature conditions relevant to the Earth’s core–mantle boundary. We suggest that, if water has been delivered to the core–mantle boundary by subduction, this reaction could enable exchange of hydrogen and silicon between the mantle and the core. The resulting H-rich, Si-deficient layer formed at the topmost core would have a lower density, stabilizing chemical stratification at the top of the core, and a lower velocity. We suggest that such chemical exchange between the core and mantle over gigayears of deep transport of water may have contributed to the formation of the putative Eʹ layer.more » « less
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The fundamental challenge to characterize and quantify thermal transport in the strongly nonlinear regime of Rayleigh–Bénard convection – the buoyancy-driven flow of a horizontal layer of fluid heated from below – has perplexed the fluid dynamics community for decades. Rayleigh proposed controlling the temperature of thermally conducting boundaries in order to study the onset of convection, in which case vertical heat transport gauges the system response. Conflicting experimental results for ostensibly similar set-ups have confounded efforts to discriminate between two competing theories for how boundary layers and interior flows interact to determine transport through the convecting layer asymptotically far beyond onset. In a conceptually new approach, Bouillaut, Lepot, Aumaître and Gallet ( J. Fluid Mech. , vol. 861, 2019, R5) devised a procedure to radiatively heat a portion of the fluid domain bypassing rigid conductive boundaries and allowing for dissociation of thermal and viscous boundary layers. Their experiments reveal a new level of complexity in the problem suggesting that heat transport scaling predictions of both theories may be realized depending on details of the thermal forcing.more » « less
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/https://doi.org/10.1038/s41561-019-0381-z
