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Nonlinear optical materials are essential for the development of both nonlinear and quantum optics and have advanced recently from bulk crystals to integrated material platforms. In this Perspective, we provide an overview of the emerging InGaP χ(2) nonlinear integrated photonics platform and its experimental achievements. With its exceptional χ(2) nonlinearity and low optical losses, the epitaxial InGaP platform significantly enhances a wide range of second-order nonlinear optical effects, from second-harmonic generation to entangled photon pair sources, achieving efficiencies several orders of magnitude beyond the current state of the art. Moreover, the InGaP platform enables quantum nonlinear optics at the few- and single-photon levels via passive nonlinearities, which has broad implications for quantum information processing and quantum networking. We also examine the current limitations of the InGaP platform and propose potential solutions to fully unlock its capabilities.
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Large optical nonlinearity enabled by coupled metallic quantum wells
Abstract New materials that exhibit strong second-order optical nonlinearities at a desired operational frequency are of paramount importance for nonlinear optics. Giant second-order susceptibilityχ(2)has been obtained in semiconductor quantum wells (QWs). Unfortunately, the limited confining potential in semiconductor QWs causes formidable challenges in scaling such a scheme to the visible/near-infrared (NIR) frequencies for more vital nonlinear-optic applications. Here, we introduce a metal/dielectric heterostructured platform, i.e., TiN/Al2O3epitaxial multilayers, to overcome that limitation. This platform has an extremely highχ(2)of approximately 1500 pm/V at NIR frequencies. By combining the aforementioned heterostructure with the large electric field enhancement afforded by a nanostructured metasurface, the power efficiency of second harmonic generation (SHG) achieved 10−4at an incident pulse intensity of 10 GW/cm2, which is an improvement of several orders of magnitude compared to that of previous demonstrations from nonlinear surfaces at similar frequencies. The proposed quantum-engineered heterostructures enable efficient wave mixing at visible/NIR frequencies into ultracompact nonlinear optical devices.
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- Award ID(s):
- 1807891
- PAR ID:
- 10153477
- Publisher / Repository:
- Nature Publishing Group
- Date Published:
- Journal Name:
- Light: Science & Applications
- Volume:
- 8
- Issue:
- 1
- ISSN:
- 2047-7538
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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