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Graphene is now a crucial component of many device designs in electronics and optics. Just like the noble metals, this single layer of carbon atoms in a honeycomb lattice can support surface plasmons, which are central to several sensing technologies in the mid-infrared regime. As with classical metal plasmons, periodic corrugations in the graphene sheet itself can be used to launch these surface waves; however, as graphene plasmons are tightly confined, the role of unwanted surface roughness, even at a nanometer scale, cannot be ignored. In this work, we revisit our previous numerical experiments on metal plasmons launched by vanishingly small grating structures, with the addition of graphene to the structure. These simulations are conducted with a recently devised, rapid, and robust high-order spectral scheme of the authors, and with it we carefully demonstrate how the plasmonic response of a perfectly flat sheet of graphene can be significantly altered with even a tiny corrugation (on the order of merely 5 nm). With these results, we demonstrate the primary importance of fabrication techniques that produce interfaces whose deviations from flat are on the order of angstroms.
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Modeling and observation of mid-infrared nonlocality in effective epsilon-near-zero ultranarrow coaxial apertures
Abstract With advances in nanofabrication techniques, extreme-scale nanophotonic devices with critical gap dimensions of just 1–2 nm have been realized. Plasmons in such ultranarrow gaps can exhibit nonlocal response, which was previously shown to limit the field enhancement and cause optical properties to deviate from the local description. Using atomic layer lithography, we create mid-infrared-resonant coaxial apertures with gap sizes as small as 1 nm and observe strong evidence of nonlocality, including spectral shifts and boosted transmittance of the cutoff epsilon-near-zero mode. Experiments are supported by full-wave 3-D nonlocal simulations performed with the hybridizable discontinuous Galerkin method. This numerical method captures atomic-scale variations of the electromagnetic fields while efficiently handling extreme-scale size mismatch. Combining atomic-layer-based fabrication techniques with fast and accurate numerical simulations provides practical routes to design and fabricate highly-efficient large-area mid-infrared sensors, antennas, and metasurfaces.
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- Award ID(s):
- 1809240
- PAR ID:
- 10154170
- Publisher / Repository:
- Nature Publishing Group
- Date Published:
- Journal Name:
- Nature Communications
- Volume:
- 10
- Issue:
- 1
- ISSN:
- 2041-1723
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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