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  • Semiclassical approach for solving the time-dependent Schrödinger equation in spatially inhomogeneous electromagnetic pulses
Title: Semiclassical approach for solving the time-dependent Schrödinger equation in spatially inhomogeneous electromagnetic pulses
To solve the time-dependent Schrödinger equation in spatially inhomogeneous pulses of electromagnetic radiation, we propose an iterative semiclassical complex trajectory approach. In numerical applications, we validate this method agains ab initio numerical solutions by scrutinizing (a) electronic sates in combined Coulomb and spatially homogeneous laser felds and (b) sreaked photoemission from hydrogen atoms and plasmonic gold nanospheres. In comparison with sreaked photoemission calculations performed in srong-feld approximation, we demonsrate the improved reconsruction of the spatially inhomogeneous induced plasmonic infrared feld near a nanoparticle surface from sreaked photoemission spectra.  more » « less
Award ID(s):
1802085
PAR ID:
10168262
Author(s) / Creator(s):
;
Date Published:
Journal Name:
Physical review and Physical review letters index
Volume:
101
ISSN:
0094-0003
Page Range / eLocation ID:
013411
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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