skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.

Explore Research Products in the PAR
It may take a few hours for recently added research products to appear in PAR search results.


Title: Fabrication and Characterization of CdZnTeSe Nuclear Detectors
Cadmium zinc telluride selenide (CdZnTeSe) is emerging as a promising semiconductor material for low-cost production of nuclear and radiological detection systems capable of operating at room temperature. This paper presents studies of the fabrication process and detector response for gamma-ray detectors produced from high-quality CdZnTeSe crystals grown by the traveler heater method (THM). The resistivity of the CdZnTeSe is on the order of 10 GΩ-cm. The electron mobility-lifetime (μτ) product characterizing the charge-transport properties is on the order of 0.001 square-cm per volt. Energy resolutions as good as 6.5% FWHM for the 59.5-keV gamma-peak of 241 Am were recorded for planar detectors with gold contacts.  more » « less
Award ID(s):
1818732
PAR ID:
10184944
Author(s) / Creator(s):
; ; ; ; ; ;
Date Published:
Journal Name:
2019 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC)
Page Range / eLocation ID:
1 to 3
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. ; ; ; ; ; ; (, 2021 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC))
    Cadmium zinc telluride selenide (CdZnTeSe) has shown great promise in reducing the cost of semiconductor nuclear detectors that can operate at room temperature without cryogenic cooling. This is due to the high yield of detector-grade materials in the CdZnTeSe crystal growth process, which can be attributed to the much smaller numbers of Te inclusions and grain boundary network in CdZnTeSe compared to other CdTe-based semiconductors such as CdZnTe. In the present work, we study the effects of surface passivation on CdZnTe detectors using a mixture of ammonium fluoride and hydrogen peroxide solution (NH4F + H2O2 + H2O). Detectors fabricated from CdZnTeSe crystals showed very good energy resolutions: 1.1% for the 662-keV gamma peak of Cs-137 by Frisch-grid detectors, and 5.9% for the 59.6-keV gamma peak of Am-241 by planar detectors. Experimental results show that the leakage current is increased immediately after passivation and then decreases as the surfaces stabilizes. The resistivity of the CdZnTeSe is of the order of 10**10 Ω-cm. The surface passivation improved the energy resolution of planar detector by 18% for the 59.6-keV gamma peak of Am-241. 
    more » « less
  2. ; ; ; ; ; ; (, Advanced Optical Materials)
    Abstract Lead halide perovskites have recently attracted intensive attention as competitive alternative candidates of legacy compound materials CdTe, CdZnTe, and TlBr for high sensitivity energy‐resolving gamma‐ray detection at room temperature. However, the use of lead in these lead halide perovskites, which is necessary for increasing the stopping power of gamma radiation, poses a serious environmental concern due to the high toxicity of lead. In this regard, environmental‐friendly perovskite‐based gamma‐ray detector materials with key energy‐resolving capabilities are highly desired. Here, the gamma energy‐resolving performance of a new class of all‐inorganic and lead‐free Cs2AgBiBr6double perovskite single crystals (SCs) is reported. Two types of Cs2AgBiBr6SCs, prepared by Bi‐normal and Bi‐poor precursor solutions, respectively, have been grown. Their mobilities and response to gamma radiation are presented. Density of trap states in Bi‐poor Cs2AgBiBr6SCs (2.65 × 109 cm−3) is one order of magnitude lower than that in Bi‐normal Cs2AgBiBr6SCs (3.85 × 1010 cm−3). Using laser‐induced photocurrent measurements, the obtained mobility–lifetime (μ–τ) product in Bi‐poor Cs2AgBiBr6SCs is 1.47 × 10−3 cm2 V−1, indicating their great potentials for gamma‐ray detection. Further, the fabricated detector based on Bi‐poor Cs2AgBiBr6SC shows response to 59.5 keV gamma‐ray with an energy resolution of 13.91%. 
    more » « less
  3. (, EPJ Web of Conferences)
    Capone, A.; De Vincenzi, M.; Morselli, A. (Ed.)
    The IceCube Neutrino Observatory located at the geographic South Pole is composed of two detectors. One is the in-ice optical array, which measures high-energy muons from air showers and charged particles produced by the interaction of high-energy neutrinos in the ice. The other is an array of ice-Cherenkov tanks at the surface, called IceTop, which is used both as veto for the in-ice neutrino measurements and for detecting cosmic-ray air showers. In the next decade, the IceCube-Gen2 extension will increase the surface coverage including surface radio antennas and scintillator panels on the footprint of an extended optical array in the ice. The combination of the current surface and in-ice detectors can be exploited for the study of cosmic rays and the search for PeV gamma rays. The in-ice detector measures the high-energy muonic component of air showers, whereas the signal in IceTop is dominated by the electromagnetic component. The relative size of the muonic and electromagnetic components is different for gamma-and hadron-induced air showers. Thus, the gamma-hadron separation of cosmic rays is attempted using machine learning techniques including deep learning. Here, different approaches are presented. Finally, the prospects for the detection of PeV photons with IceCube-Gen2 will be discussed. 
    more » « less
  4. ; ; ; ; ; ; ; ; ; ; et al (, Acta Physica Polonica B Proceedings Supplement)
    A high-statistics \(\beta \)-decay experiment was conducted at the TRIUMF-ISAC facility using the \(8\pi \) \(\gamma \)-ray spectrometer and its ancillary detectors to study the low-spin structure of \(^{98}\)Zr. The analysis of \(\gamma \)–\(\gamma \) and \(e^-\)–\(\gamma \) coincidence data is presented. New measurements of \(\gamma \)-ray branching ratios and mixing ratios are reported for four \(J^{\pi } = 2^+\) states located above 2 MeV excitation energy in \(^{98}\)Zr. Based on these measurements, ratios of \(B\)(E2) values for transitions to lower-lying levels are determined, highlighting the preferential decay paths of these \(2^+\) states. AbstractPublished by the Jagiellonian University2025authors 
    more » « less
  5. ; ; ; ; (, The Astrophysical Journal Letters)
    Abstract Recent observations of high-energy neutrinos by IceCube and gamma rays by the Fermi Large Area Telescope (LAT) and the MAGIC telescope have suggested that neutrinos are produced in gamma-ray opaque environments in the vicinity of supermassive black holes. In this work, we present 20 MeV–1 TeV spectra of three Seyfert galaxies whose nuclei are predicted to be active in neutrinos, NGC 4151, NGC 4945, and the Circinus galaxy, using 14.4 yr of Fermi LAT data. In particular, we find evidence of sub-GeV excess emission that can be attributed to gamma rays from NGC 4945, as was also seen in NGC 1068. These spectral features are consistent with predictions of the magnetically powered corona model, and we argue that NGC 4945 is among the brightest neutrino active galaxies detectable for KM3Net and Baikal-GVD. On the other hand, in contrast to other reported results, we do not detect gamma rays from NGC 4151, which constrains neutrino emission from the accretion shock model. Future neutrino detectors such as IceCube-Gen2 and MeV gamma-ray telescopes such as AMEGO-X will be crucial for discriminating among the theoretical models. 
    more » « less
  • Citation Formats
  • MLA
  • APA
  • Chicago
  • BibTeX
  • Save / Share this Record
  • Send to Email