It is a challenging task to fabricate thermally stable Photodetectors (PDs) working in visible light spectrum range due to the degradation in photoresponse characteristics. Herein, excellent performance parameters with photoresponsivity reached up to as high as 50 AW -1 , and ultrahigh specific detectivity in excess of 2.3×10 12 Jones have been obtained simultaneously in a single photodetector based on vertical MoS 2 (v-MoS 2 ) at a high temperature of 200°C. The TiO 2 interlay layer is ascribed as the main factor to enhance the PDs performances by reducing lattice mismatch between v-MoS 2 and substrate, separating photogenerated electron-hole pairs (EHPs), and the formation of the vertical MoS 2 nanostructures. Besides, the optoelectronics performances of the v-MoS 2 /TiO 2 heterostructures based field-effect transistor (FET) have also been examined under various operating temperatures, and the mechanism on how gate voltages affect the PDs performances has also been studied. In a word, the present fabricated v-MoS 2 /TiO 2 heterostructures based FET PDs will find practical applications in high-temperature environment.
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Optoelectronic synapse using monolayer MoS2 field effect transistors
Abstract Optical data sensing, processing and visual memory are fundamental requirements for artificial intelligence and robotics with autonomous navigation. Traditionally, imaging has been kept separate from the pattern recognition circuitry. Optoelectronic synapses hold the special potential of integrating these two fields into a single layer, where a single device can record optical data, convert it into a conductance state and store it for learning and pattern recognition, similar to the optic nerve in human eye. In this work, the trapping and de-trapping of photogenerated carriers in the MoS 2 /SiO 2 interface of a n-channel MoS 2 transistor was employed to emulate the optoelectronic synapse characteristics. The monolayer MoS 2 field effect transistor (FET) exhibits photo-induced short-term and long-term potentiation, electrically driven long-term depression, paired pulse facilitation (PPF), spike time dependent plasticity, which are necessary synaptic characteristics. Moreover, the device’s ability to retain its conductance state can be modulated by the gate voltage, making the device behave as a photodetector for positive gate voltages and an optoelectronic synapse at negative gate voltages.
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- Award ID(s):
- 1845331
- PAR ID:
- 10211260
- Date Published:
- Journal Name:
- Scientific Reports
- Volume:
- 10
- Issue:
- 1
- ISSN:
- 2045-2322
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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