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1. Collective Thomson scattering measurement of plasma evolution during the current pulse in a laser-triggered switch

   https://doi.org/10.1063/5.0131471  

   Gottfried, Jacob A. ; Rose, Charles E. ; Simpson, Sean ; Yalin, Azer P. ( December 2022 , Applied Physics Letters)

   High-voltage laser-triggered switches (HV-LTSs) are used in pulsed-power applications where low jitter and precise timing are required. The switches allow operation in the megaampere, megavolt regime while maintaining low insertion losses. Currently, there is a lack of detailed plasma measurements in these switches, yet such measurements are needed to elucidate the detailed physics, which include a range of processes such as laser breakdown, streamer formation and growth, current flow, plasma evolution, and cooling. Detailed spatially- and temporally resolved measurements of plasma properties within the switches could contribute to validating and advancing numeric models of these systems. This contribution presents laser Thomson scattering measurements of the electron number density and temperature evolution in a HV-LTS. The switch was operated at 6 kV with current flow for a duration of 145 ns and a peak current density of 0.2 MA/cm2 into a matched load. The Thomson scattering diagnostic system uses a 532 nm probe from an Nd:YAG laser allowing a temporal resolution of ∼10 ns. We find that during the switch current pulse, the plasma electron temperature rose from a starting value of 8.1 ± 1.6 eV (due to cooling of the earlier trigger laser plasma) to a peak value of 26 ± 5 eV with an associated increase in the electron density from 8.6 ± 1.7 × 1017 to 3.1 ± 0.6 × 1018 cm−3.

    

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2. Spectral attenuation coefficients from measurements of light transmission in bare ice on the Greenland Ice Sheet

   https://doi.org/10.5194/tc-15-1931-2021  

   Cooper, Matthew G. ; Smith, Laurence C. ; Rennermalm, Asa K. ; Tedesco, Marco ; Muthyala, Rohi ; Leidman, Sasha Z. ; Moustafa, Samiah E. ; Fayne, Jessica V. ( January 2021 , The Cryosphere)

   Abstract. Light transmission into bare glacial ice affects surfaceenergy balance, biophotochemistry, and light detection and ranging (lidar)laser elevation measurements but has not previously been reported for theGreenland Ice Sheet. We present measurements of spectral transmittance at350–900 nm in bare glacial ice collected at a field site in the westernGreenland ablation zone (67.15∘ N, 50.02∘ W). Empirical irradianceattenuation coefficients at 350–750 nm are ∼ 0.9–8.0 m−1 for ice at 12–124 cm depth. The absorption minimum is at∼ 390–397 nm, in agreement with snow transmissionmeasurements in Antarctica and optical mapping of deep ice at the SouthPole. From 350–530 nm, our empirical attenuation coefficients are nearly1 order of magnitude larger than theoretical values for optically pureice. The estimated absorption coefficient at 400 nm suggests the ice volumecontained a light-absorbing particle concentration equivalent to∼ 1–2 parts per billion (ppb) of black carbon, which is similar topre-industrial values found in remote polar snow. The equivalent mineraldust concentration is ∼ 300–600 ppb, which is similar to values forNorthern Hemisphere warm periods with low aeolian activity inferred from icecores. For a layer of quasi-granular white ice (weathering crust)extending from the surface to ∼ 10 cm depth, attenuationcoefficients are 1.5 to 4 times larger than for deeper bubbly ice. Owing tohigher attenuation in this layer of near-surface granular ice, opticalpenetration depth at 532 nm is 14 cm (20 %) lower than asymptoticattenuation lengths for optically pure bubbly ice. In addition to thetraditional concept of light scattering on air bubbles, our results implythat the granular near-surface ice microstructure of weathering crust isan important control on radiative transfer in bare ice on the Greenland IceSheet ablation zone, and we provide new values of flux attenuation,absorption, and scattering coefficients to support model development andvalidation. 

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3. Thomson scattering diagnostics of nonthermal plasma from particle-in-cell simulations

   Farrell, Audrey ; Zhang, Chaojie ; Wu, Yipeng ; Nie, Zan ; Nambu, Noa ; Sinclair, Mitchell ; Marsh, Kenneth ; Joshi, Chandrasekhar ( April 2023 , Advanced Accelerator Concepts Workshop 2022)

   Optical Thomson scattering is now a mature diagnostic tool for precisely measuring local plasma density and temperature. These measurements typically take advantage of a simplified analytical model of the scattered spectrum, which is built upon the assumption that each plasma species is in thermal equilibrium. However, this assumption fails for most laboratory plasmas of interest, which are often produced through high field ionization of atoms via ultrashort laser pulses and vulnerable to several kinetic instabilities. While it is possible to analytically model the Thomson scattered spectrum for some non-Maxwellian distribution functions, it is often not practical to do so for laboratory plasmas with highly complex and unstable distribution functions. We present a new method for predicting the Thomson scattered spectrum from any plasma directly from fully kinetic particle-in-cell simulations. This approach allows us to model the contributions of kinetic instabilities to the Thomson spectrum that aren’t taken into account in Maxwellian theory. We demonstrate this method’s capability to capture nonthermal features in the Thomson spectrum by simulating a simple bumpon- tail plasma as well as a more complex laser-ionized plasma. The versatility of this approach makes it an effective aid in the experimental design of Thomson diagnostics to directly characterize kinetic instabilities in laboratory plasmas. Index Terms—plasma measurement, low-temperature plasmas, plasma diagnostics, plasma simulation, plasma stability, plasma density, plasma temperature 

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4. Hyper-Raman optical activity of biologically relevant chiral molecules

   https://doi.org/10.1117/12.2545530  

   Marble, Christopher B. ; Xu, Xingqi ; Keppler, Mark A. ; Gil, Eddie M. ; Petrov, Georgi I. ; Wang, Dawei ; Yakovlev, Vladislav V. ; Razeghi, Manijeh ; Lewis, Jay S. ; Khodaparast, Giti A. ; et al ( March 2020 , Hyper-Raman optical activity of biologically relevant chiral molecules)

   The optical activity of Raman scattering provides insight into the absolute configuration and conformation of chiral molecules. Applications of Raman optical activity (ROA) are limited by long integration times due to a relatively low sensitivity of the scattered light to chirality (typically 10^-3 to 10^-5). We apply ROA techniques to hyper-Raman scattering using incident circularly polarized light and a right-angle scattering geometry. We explore the sensitivity of hyper- Raman scattering to chirality as compared to spontaneous Raman optical activity. Using the excitation wavelength at around 532 nm, the photobleaching is minimized, while the hyper-Raman scattering benefits from the electronic resonant enhancement. For S/R-2-butanol and L/D-tartaric acid, we were unable to detect the hyper-Raman optical activity at the sensitivity level of 1%. We also explored parasitic thermal effects which can be mitigating by varying the repetition rate of the laser source used for excitation of hyper-Raman scattering. 

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5. In-situ coating of silicon-rich films on tokamak plasma-facing components with real-time Si material injection

   https://doi.org/10.1088/1741-4326/acee98  

   Effenberg, F. ; Abe, S. ; Sinclair, G. ; Abrams, T. ; Bortolon, A. ; Wampler, W. R. ; Laggner, F. M. ; Rudakov, D. L. ; Bykov, I. ; Lasnier, C. J. ; et al ( August 2023 , Nuclear Fusion)

   Experiments have been conducted in the DIII-D tokamak to explore thein-situgrowth of silicon-rich layers as a potential technique for real-time replenishment of surface coatings on plasma-facing components (PFCs) during steady-state long-pulse reactor operation. Silicon (Si) pellets of 1 mm diameter were injected into low- and high-confinement (L-mode and H-mode) plasma discharges with densities ranging from 3.9–$7.5\times {10}^{19}$m⁻³and input powers ranging from 5.5 to 9 MW. The small Si pellets were delivered with the impurity granule injector at frequencies ranging from 4 to 16 Hz corresponding to mass flow rates of 5–19 mg s⁻¹(1–$4.2\times {10}^{20}$Si s⁻¹) at cumulative amounts of up to 34 mg of Si per five-second discharge. Graphite samples were exposed to the scrape-off layer and private flux region plasmas through the divertor material evaluation system to evaluate the Si deposition on the divertor targets. The Si II emission at the sample correlates with silicon injection and suggests net surface Si-deposition in measurable amounts. Post-mortem analysis showed Si-rich coatings containing silicon oxides, of which SiO₂is the dominant component. No evidence of SiC was found, which is attributed to low divertor surface temperatures. Thein-situand ex-situ analysis found that Si-rich coatings of at least 0.4–1.2 nm thickness have been deposited at 0.4–0.7 nm s⁻¹. The technique is estimated to coat a surface area of at least 0.94 m²on the outer divertor. These results demonstrate the potential of using real-time material injection to form Si-enriched layers on divertor PFCs during reactor operation.

    

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