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1. Energetic Electron Precipitation Driven by Electromagnetic Ion Cyclotron Waves from ELFIN’s Low Altitude Perspective

   https://doi.org/10.1007/s11214-023-00984-w  

   Angelopoulos, V. ; Zhang, X. -J. ; Artemyev, A. V. ; Mourenas, D. ; Tsai, E. ; Wilkins, C. ; Runov, A. ; Liu, J. ; Turner, D. L. ; Li, W. ; et al ( July 2023 , Space Science Reviews)

   We review comprehensive observations of electromagnetic ion cyclotron (EMIC) wave-driven energetic electron precipitation using data collected by the energetic electron detector on the Electron Losses and Fields InvestigatioN (ELFIN) mission, two polar-orbiting low-altitude spinning CubeSats, measuring 50-5000 keV electrons with good pitch-angle and energy resolution. EMIC wave-driven precipitation exhibits a distinct signature in energy-spectrograms of the precipitating-to-trapped flux ratio: peaks at >0.5 MeV which are abrupt (bursty) (lasting ∼17 s, or$\Delta L\sim 0.56$$\Delta L\sim 0.56$) with significant substructure (occasionally down to sub-second timescale). We attribute the bursty nature of the precipitation to the spatial extent and structuredness of the wave field at the equator. Multiple ELFIN passes over the same MLT sector allow us to study the spatial and temporal evolution of the EMIC wave - electron interaction region. Case studies employing conjugate ground-based or equatorial observations of the EMIC waves reveal that the energy of moderate and strong precipitation at ELFIN approximately agrees with theoretical expectations for cyclotron resonant interactions in a cold plasma. Using multiple years of ELFIN data uniformly distributed in local time, we assemble a statistical database of ∼50 events of strong EMIC wave-driven precipitation. Most reside at$L\sim 5-7$$L\sim 5-7$at dusk, while a smaller subset exists at$L\sim 8-12$$L\sim 8-12$at post-midnight. The energies of the peak-precipitation ratio and of the half-peak precipitation ratio (our proxy for the minimum resonance energy) exhibit an$L$$L$-shell dependence in good agreement with theoretical estimates based on prior statistical observations of EMIC wave power spectra. The precipitation ratio’s spectral shape for the most intense events has an exponential falloff away from the peak (i.e., on either side of$\sim 1.45$$\sim 1.45$MeV). It too agrees well with quasi-linear diffusion theory based on prior statistics of wave spectra. It should be noted though that this diffusive treatment likely includes effects from nonlinear resonant interactions (especially at high energies) and nonresonant effects from sharp wave packet edges (at low energies). Sub-MeV electron precipitation observed concurrently with strong EMIC wave-driven >1 MeV precipitation has a spectral shape that is consistent with efficient pitch-angle scattering down to ∼ 200-300 keV by much less intense higher frequency EMIC waves at dusk (where such waves are most frequent). At ∼100 keV, whistler-mode chorus may be implicated in concurrent precipitation. These results confirm the critical role of EMIC waves in driving relativistic electron losses. Nonlinear effects may abound and require further investigation.

    

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2. Revealing the Cooperative Relationship between Spin, Energy, and Polarization Parameters toward Developing High‐Efficiency Exciplex Light‐Emitting Diodes

   https://doi.org/10.1002/adma.201904114  

   Wang, Miaosheng ; Huang, Yi‐Hsuan ; Lin, Kai‐Siang ; Yeh, Tzu‐Hung ; Duan, Jiashun ; Ko, Tzu‐Yu ; Liu, Shun‐Wei ; Wong, Ken‐Tsung ; Hu, Bin ( September 2019 , Advanced Materials)

   Experimental studies to reveal the cooperative relationship between spin, energy, and polarization through intermolecular charge‐transfer dipoles to harvest nonradiative triplets into radiative singlets in exciplex light‐emitting diodes are reported. Magneto‐photoluminescence studies reveal that the triplet‐to‐singlet conversion in exciplexes involves an artificially generated spin‐orbital coupling (SOC). The photoinduced electron parametric resonance measurements indicate that the intermolecular charge‐transfer occurs with forming electric dipoles (D^+•→A^−•), providing the ionic polarization to generate SOC in exciplexes. By having different singlet‐triplet energy differences (ΔE_ST) in 9,9′‐diphenyl‐9H,9′H‐3,3′‐bicarbazole (BCzPh):3′,3′″,3′″″‐(1,3,5‐triazine‐2,4,6‐triyl)tris(([1,1′‐biphenyl]‐3‐carbonitrile)) (CN‐T2T) (ΔE_ST= 30 meV) and BCzPh:bis‐4,6‐(3,5‐di‐3‐pyridylphenyl)‐2‐methyl‐pyrimidine (B3PYMPM) (ΔE_ST= 130 meV) exciplexes, the SOC generated by the intermolecular charge‐transfer states shows large and small values (reflected by different internal magnetic parameters: 274 vs 17 mT) with high and low external quantum efficiency maximum, EQE_max(21.05% vs 4.89%), respectively. To further explore the cooperative relationship of spin, energy, and polarization parameters, different photoluminescence wavelengths are selected to concurrently change SOC, ΔE_ST, and polarization while monitoring delayed fluorescence. When the electron clouds become more deformed at a longer emitting wavelength due to reduced dipole (D^+•→A^−•) size, enhanced SOC, increased orbital polarization, and decreased ΔE_STcan simultaneously occur to cooperatively operate the triplet‐to‐singlet conversion.

    

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3. ΔK =0 M1 Excitation Strength of the Well-Deformed Nucleus 164Dy from K Mixing

   T. Beck, V. Werner ( August 2020 , Physical review letters)

   The size of a ΔK ¼ 0 M1 excitation strength has been determined for the first time in a predominantly axially deformed even-even nucleus. It has been obtained from the observation of a rare K-mixing situation between two close-lying Jπ ¼ 1þ states of the nucleus 164Dy with components characterized by intrinsic projection quantum numbers K ¼ 0 and K ¼ 1. Nuclear resonance fluorescence induced by quasimonochromatic linearly polarized γ-ray beams provided evidence for K mixing of the 1þ states at 3159.1(3) and 3173.6(3) keV in excitation energy from their γ-decay branching ratios into the ground-state band. The ΔK ¼ 0 transition strength of BðM1; 0 þ 1 → 1 þ K¼0 Þ ¼ 0.008ð1Þμ2 N was inferred from a mixing analysis of their M1 transition rates into the ground-state band. It is in agreement with predictions from the quasiparticle phonon nuclear model. This determination represents first experimental information on the M1 excitation strength of a nuclear quantum state with a negative R-symmetry quantum number. 

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4. 20 Ne(α,p) 23 Na studied to constrain type Ia nucleosynthesis

   https://doi.org/10.1088/1742-6596/2586/1/012110  

   Boomershine, C N ; Bardayan, D W ; Carmichael, S ; Caves, L ; Davis, A ; deBoer, R J ; Gula, A ; Howard, K ; Kelmar, R ; Mitchell, A ; et al ( September 2023 , Journal of Physics: Conference Series)

   The²⁰Ne(α,p)²³Na reaction rate is important in determining the final abundances of various nuclei produced in type Ia supernovae. Previously, the ground state cross section was calculated from time reversal reaction experiments using detailed balance. The reaction rates extracted from these studies do not consider contributions from the population of excited states, and therefore, are only estimates. A resonance scan, populating both the ground and first excited states, was performed for the²⁰Ne(α,p)²³Na reaction, measuring between 2.9 and 5 MeV center of mass energies at the Nuclear Science Lab at the University of Notre Dame. Data analysis is underway and preliminary results show substantial contribution from the excited state reaction.

    

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5. Experimental study of the proton-transfer reaction C + H 2 + → CH + + H and its isotopic variant (D 2 + )

   https://doi.org/10.1039/D0CP04810K  

   Hillenbrand, Pierre-Michel ; Bowen, Kyle P. ; Dayou, Fabrice ; Miller, Kenneth A. ; de Ruette, Nathalie ; Urbain, Xavier ; Savin, Daniel W. ( December 2020 , Physical Chemistry Chemical Physics)

   We report absolute integral cross section (ICS) measurements using a dual-source merged-fast-beams apparatus to study the titular reactions over the relative translational energy range of E r ∼ 0.01–10 eV. We used photodetachment of C − to produce a pure beam of atomic C in the ground electronic 3 P term, with statistically populated fine-structure levels. The H 2 + and D 2 + were formed in an electron impact ionization source, with well known vibrational and rotational distributions. The experimental work is complemented by a theoretical study of the CH 2 + electronic system in the reactant and product channels, which helps to clarify the possible reaction mechanisms underlying the ICS measurements. Our measurements provide evidence that the reactions are barrierless and exoergic. They also indicate the apparent absence of an intermolecular isotope effect, to within the total experimental uncertainties. Capture models, taking into account either the charge-induced dipole interaction potential or the combined charge-quadrupole and charge-induced dipole interaction potentials, produce reaction cross sections that lie a factor of ∼4 above the experimental results. Based on our theoretical study, we hypothesize that the reaction is most likely to proceed adiabatically through the 1 4 A′ and 1 4 A′′ states of CH 2 + via the reaction C( 3 P) + H 2 + ( 2 Σ+g) → CH + ( 3 Π) + H( 2 S). We also hypothesize that at low collision energies only H 2 + ( v ≤ 2) and D 2 + ( v ≤ 3) contribute to the titular reactions, due to the onset of dissociative charge transfer for higher vibrational v levels. Incorporating these assumptions into the capture models brings them into better agreement with the experimental results. Still, for energies ≲0.1 eV where capture models are most relevant, the modified charge-induced dipole model yields reaction cross sections with an incorrect energy dependence and lying ∼10% below the experimental results. The capture cross section obtained from the combined charge-quadrupole and charge-induced dipole model better matches the measured energy dependence but lies ∼30–50% above the experimental results. These findings provide important guidance for future quasiclassical trajectory and quantum mechanical treatments of this reaction. 

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