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Title: Antiferromagnetic proximity coupling between semiconductor quantum emitters in WSe 2 and van der Waals ferromagnets
van der Waals ferromagnets have gained significant interest due to their unique ability to provide magnetic response even at the level of a few monolayers. Particularly in combination with 2D semiconductors, such as the transition metal dichalcogenide WSe 2 , one can create heterostructures that feature unique magneto-optical response in the exciton emission through the magnetic proximity effect. Here we use 0D quantum emitters in WSe 2 to probe for the ferromagnetic response in heterostructures with Fe 3 GT and Fe 5 GT ferromagnets through an all-optical read-out technique that does not require electrodes. The spectrally narrow spin-doublet of the WSe 2 quantum emitters allowed to fully resolve the hysteretic magneto-response in the exciton emission, revealing the characteristic signature of both ferro- and antiferromagnetic proximity coupling that originates from the interplay among Fe 3 GT or Fe 5 GT, a thin surface oxide, and the spin doublets of the quantum emitters. Our work highlights the utility of 0D quantum emitters for probing interface magnetic dipoles in vdW heterostructures with high precision. The observed hysteretic magneto response in the exciton emission of quantum emitters adds further new degrees of freedom for spin and g -factor manipulation of quantum states.  more » « less
Award ID(s):
1809235
PAR ID:
10288191
Author(s) / Creator(s):
; ; ; ; ; ; ;
Date Published:
Journal Name:
Nanoscale
Volume:
13
Issue:
2
ISSN:
2040-3364
Page Range / eLocation ID:
832 to 841
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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