skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Title: Smartphone-powered efficient water disinfection at the point of use
Abstract Clean water free of bacteria is a precious resource in areas where no centralized water facilities are available. Conventional chlorine disinfection is limited by chemical transportation, storage, and the production of carcinogenic by-products. Here, a smartphone-powered disinfection system is developed for point-of-use (POU) bacterial inactivation. The integrated system uses the smartphone battery as a power source, and a customized on-the-go (OTG) hardware connected to the phone to realize the desired electrical output. Through a downloadable mobile application, the electrical output, either constant current (20–1000 µA) or voltage (0.7–2.1 V), can be configured easily through a user-friendly graphical interface on the screen. The disinfection device, a coaxial-electrode copper ionization cell (CECIC), inactivates bacteria by low levels of electrochemically generated copper with low energy consumption. The strategy of constant current control is applied in this study to solve the problem of uncontrollable copper release by previous constant voltage control. With the current control, a high inactivation efficiency ofE. coli(~6 logs) is achieved with a low level of effluent Cu (~200 µg L−1) in the water samples within a range of salt concentration (0.2–1 mmol L−1). The smartphone-based power workstation provides a versatile and accurate electrical output with a simple graphical user interface. The disinfection device is robust, highly efficient, and does not require complex equipment. As smartphones are pervasive in modern life, the smartphone-powered CECIC system could provide an alternative decentralized water disinfection approach like rural areas and outdoor activities.  more » « less
Award ID(s):
1845354
PAR ID:
10307624
Author(s) / Creator(s):
; ; ; ;
Publisher / Repository:
Nature Publishing Group
Date Published:
Journal Name:
npj Clean Water
Volume:
3
Issue:
1
ISSN:
2059-7037
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Chlorine disinfection inevitably generates carcinogenic by-products. Alternative non-chlorine-based techniques in centralized treatment plants cannot produce residual antimicrobial power in water disinfection systems. Here, we propose locally enhanced electric field treatment (LEEFT) for chemical-free water disinfection in pipes. A tubular LEEFT device with coaxial electrodes is rationally developed for easy adaption to current water distribution systems as a segment of the pipelines. The center electrode is modified with perpendicularly grown nanowires, so that the electric field strength near the tips of the nanowires is significantly enhanced for pathogen inactivation. We have demonstrated >6-log inactivation of bacteria with 1 V, a small voltage that can be generated in situ by flowing water. 
    more » « less
  2. We propose a special design enclosure device that promotes isotropic distribution of germicidal UV-C light for the effective disinfection of difficult to reach surfaces. We used experimental and computational approaches to investigate the disinfection efficacy of this device againstEscherichia coliandListeria innocua. Stainless steel, Copper metal, and a Copper polymer were used as solid substrates of varying roughness and hydrophobicity. Bacteria reductions of up to 6.9 log CFU were achieved at various locations relative to the UV-C source after 3 min of treatment (20–990 mJ/cm2cumulative fluence depending on the location). Inactivation kinetics was nonlinear and followed the Weibull model (0.77 ≤R2≤ 0.97). Optical ray tracing simulation was used to generate maps of spatial light distribution, which were then coupled with microbial inactivation kinetics to create spatial maps of inactivation. The modeling approach used accurately predicted microbial inactivation at various locations, with only small discrepancies (±8%) between predicted and experimental data. These findings demonstrate that the proposed device is suitable for disinfecting various hard to reach surfaces, with numerous possible applications in the food and healthcare industries. Additionally, the modeling approach used here can be used to aid in the design of a highly effective Ultraviolet treatment system. 
    more » « less
  3. Abstract As the overuse of chemicals in our disinfection processes becomes an ever-growing concern, alternative approaches to reduce and replace the usage of chemicals is warranted. Electric field treatment has shown promising potential to have synergistic effects with standard chemical-based methods as they both target the cell membrane specifically. In this study, we use a lab-on-a-chip device to understand, observe, and quantify the synergistic effect between electric field treatment and copper inactivation. Observations in situ, and at a single cell level, ensure us that the combined approach has an enhancement effect leading more bacteria to be weakened by electric field treatment and susceptible to inactivation by copper ion permeation. The synergistic effects of electric field treatment and copper can be visually concluded here, enabling the further study of this technology to optimally develop, mature, and scale for its various applications in the future. 
    more » « less
  4. Deformable energy devices capable of efficiently scavenging ubiquitous mechanical signals enable the realization of self-powered wearable electronic systems for emerging human-integrated technologies. Triboelectric nanogenerators (TENGs) utilizing soft polymers with embedded additives and engineered dielectric properties emerge as ideal candidates for such applications. However, the use of solid filler materials in the state-of-the-art TENGs limits the devices' mechanical deformability and long-term durability. The current structural design for TENGs faces the dilemma where the enhanced dielectric constant of the TENG's contact layer leads to an undesirable saturation of the surface charge density. Here, we present a novel scheme to address the above issues, by exploring a liquid-metal-inclusion based TENG (LMI-TENG) where inherently deformable core–shell LMIs are incorporated into wearable high-dielectric-constant polymers. Through a holistic approach integrating theoretical and experimental efforts, we identified the parameter space for designing an LMI-TENG with co-optimized output and mechanical deformability. As a proof of concept, we demonstrated an LMI-TENG based wireless media control system for a self-powered user interface. The device architecture and design scheme presented here provide a promising solution towards the realization of self-powered human-integrated technologies. 
    more » « less
  5. Legionella pneumophila is a virulent bacterial pathogen that can cause a severe and deadly form of pneumonia called Legionnaires’ disease. Documented cases of Legionnaires’ disease have been rising since 2000. Risk of infection increases when L. pneumophila are harbored inside free-living amoebae, which are resistant to traditional disinfection processes. The ability of amoebae to phagocytose L. pneumophila allows amoebae to act as ‘Trojan horses’ for pathogen transport. This project aims to extract an unintended benefit from low-intensity microwave (MW) radiation (already found in many homes across economic cross-sections) by employing nanomaterials (e.g., silver, copper oxide, and carbon nanotubes) that are capable of harnessing such radiation and localizing the otherwise dissipated energy. In this alternative technology, we hypothesize that amoebae will be lysed via localized interfacial heating, and the released L. pneumophila will be inactivated subsequently by heat, metal ions (from nanoparticle dissolution), and reactive oxygen species (ROS) produced in the process. Traditionally, inactivation of up to 3-logs of planktonic L. pneumophila with dissolved silver requires hours of contact time. This study reports rapid inactivation (in minutes) of 3-log or higher when the planktonic L. pneumophila is subjected to AgNPs (5 mg/L) and MW radiation (2,450 MHz; 70 W). Ensuing phases of this project will incorporate copper oxide nanoparticles – which are anticipated to increase toxicity akin to copper-silver ionization systems currently employed in hospitals for L. pneumophila control – and enhance inactivation potency with potentially lower microwave radiation input and/or a lower concentration of nanoparticles. Ultimately, the nanomaterials will be immobilized on a plaster of Paris or ceramic surface for flow-through applications for lysing amoebae and inactivating L. pneumophila. 
    more » « less