We present experiments on large air cavities spanning a wide range of sizes relative to the Hinze scale $$d_{H}$$ , the scale at which turbulent stresses are balanced by surface tension, disintegrating in turbulence. For cavities with initial sizes $$d_0$$ much larger than $$d_{H}$$ (probing up to $$d_0/d_{H} = 8.3$$ ), the size distribution of bubbles smaller than $$d_{H}$$ follows $$N(d) \propto d^{-3/2}$$ , with $$d$$ the bubble diameter. The capillary instability of ligaments involved in the deformation of the large bubbles is shown visually to be responsible for the creation of the small bubbles. Turning to dynamical, three-dimensional measurements of individual break-up events, we describe the break-up child size distribution and the number of child bubbles formed as a function of $$d_0/d_{H}$$ . Then, to model the evolution of a population of bubbles produced by turbulent bubble break-up, we propose a population balance framework in which break-up involves two physical processes: an inertial deformation to the parent bubble that sets the size of large child bubbles, and a capillary instability that sets the size of small child bubbles. A Monte Carlo approach is used to construct the child size distribution, with simulated stochastic break-ups constrained by our experimental measurements and the understanding of the role of capillarity in small bubble production. This approach reproduces the experimental time evolution of the bubble size distribution during the disintegration of large air cavities in turbulence.
more »
« less
Sub-Hinze scale bubble production in turbulent bubble break-up
We study bubble break-up in homogeneous and isotropic turbulence by direct numerical simulations of the two-phase incompressible Navier–Stokes equations. We create the turbulence by forcing in physical space and introduce the bubble once a statistically stationary state is reached. We perform a large ensemble of simulations to investigate the effect of the Weber number (the ratio of turbulent and surface tension forces) on bubble break-up dynamics and statistics, including the child bubble size distribution, and discuss the numerical requirements to obtain results independent of grid size. We characterize the critical Weber number below which no break-up occurs and the associated Hinze scale $$d_h$$ . At Weber number close to stable conditions (initial bubble sizes $$d_0\approx d_h$$ ), we observe binary and tertiary break-ups, leading to bubbles mostly between $$0.5d_h$$ and $$d_h$$ , a signature of a production process local in scale. For large Weber numbers ( $$d_0> 3d_h$$ ), we observe the creation of a wide range of bubble radii, with numerous child bubbles between $$0.1d_h$$ and $$0.3d_h$$ , an order of magnitude smaller than the parent bubble. The separation of scales between the parent and child bubble is a signature of a production process non-local in scale. The formation mechanism of these sub-Hinze scale bubbles relates to rapid large deformation and successive break-ups: the first break-up in a sequence leaves highly deformed bubbles which will break again, without recovering a spherical shape and creating an array of much smaller bubbles. We discuss the application of this scenario to the production of sub-Hinze bubbles under breaking waves.
more »
« less
- Award ID(s):
- 1844932
- PAR ID:
- 10308883
- Date Published:
- Journal Name:
- Journal of Fluid Mechanics
- Volume:
- 917
- ISSN:
- 0022-1120
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
null (Ed.)We experimentally investigate the breakup mechanisms and probability of Hinze-scale bubbles in turbulence. The Hinze scale is defined as the critical bubble size based on the critical mean Weber number, across which the bubble breakup probability was believed to have an abrupt transition from being dominated by turbulence stresses to being suppressed completely by the surface tension. In this work, to quantify the breakup probability of bubbles with sizes close to the Hinze scale and to examine different breakup mechanisms, both bubbles and their surrounding tracer particles were simultaneously tracked. From the experimental results, two Weber numbers, one calculated from the slip velocity between the two phases and the other acquired from local velocity gradients, are separated and fitted with models that can be linked back to turbulence characteristics. Moreover, we also provide an empirical model to link bubble deformation to the two Weber numbers by extending the relationship obtained from potential flow theory. The proposed relationship between bubble aspect ratio and the Weber numbers seems to work consistently well for a range of bubble sizes. Furthermore, the time traces of bubble aspect ratio and the two Weber numbers are connected using the linear forced oscillator model. Finally, having access to the distributions of these two Weber numbers provides a unique way to extract the breakup probability of bubbles with sizes close to the Hinze scale.more » « less
-
Bubble-mediated gas exchange in turbulent flow is critical in bubble column chemical reactors as well as for ocean–atmosphere gas exchange related to air entrained by breaking waves. Understanding the transfer rate from a single bubble in turbulence at large Péclet numbers (defined as the ratio between the rate of advection and diffusion of gas) is important as it can be used for improving models on a larger scale. We characterize the mass transfer of dilute gases from a single bubble in a homogeneous isotropic turbulent flow in the limit of negligible bubble volume variations. We show that the mass transfer occurs within a thin diffusive boundary layer at the bubble–liquid interface, whose thickness decreases with an increase in turbulent Péclet number, $$\widetilde {{Pe}}$$ . We propose a suitable time scale $$\theta$$ for Higbie ( Trans. AIChE , vol. 31, 1935, pp. 365–389) penetration theory, $$\theta = d_0/\tilde {u}$$ , based on $$d_0$$ the bubble diameter and $$\tilde {u}$$ a characteristic turbulent velocity, here $$\tilde {u}=\sqrt {3}\,u_{{rms}}$$ , where $$u_{{rms}}$$ is the large-scale turbulence fluctuations. This leads to a non-dimensional transfer rate $${Sh} = 2(3)^{1/4}\sqrt {\widetilde {{Pe}}/{\rm \pi} }$$ from the bubble in the isotropic turbulent flow. The theoretical prediction is verified by direct numerical simulations of mass transfer of dilute gas from a bubble in homogeneous and isotropic turbulence, and very good agreement is observed as long as the thin boundary layer is properly resolved.more » « less
-
Abstract From air-sea gas exchange, oil pollution, to bioreactors, the ubiquitous fragmentation of bubbles/drops in turbulence has been modeled by relying on the classical Kolmogorov-Hinze paradigm since the 1950s. This framework hypothesizes that bubbles/drops are broken solely by eddies of the same size, even though turbulence is well known for its wide spectrum of scales. Here, by designing an experiment that can physically and cleanly disentangle eddies of various sizes, we report the experimental evidence to challenge this hypothesis and show that bubbles are preferentially broken by the sub-bubble-scale eddies. Our work also highlights that fragmentation cannot be quantified solely by the stress criterion or the Weber number; The competition between different time scales is equally important. Instead of being elongated slowly and persistently by flows at their own scales, bubbles are fragmented in turbulence by small eddies via a burst of intense local deformation within a short time.more » « less
-
We experimentally investigate the rise velocity of finite-sized bubbles in turbulence with a high energy dissipation rate of $$\unicode[STIX]{x1D716}\gtrsim 0.5~\text{m}^{2}~\text{s}^{-3}$$ . In contrast to a 30–40 % reduction in rise velocity previously reported in weak turbulence (the Weber number ( $We$ ) is much smaller than the Eötvös number ( $Eo$ ); $$We\ll 1more » « less
An official website of the United States government

