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The success of nematic liquid crystals in displays and optical applications is due to the combination of their optical uniaxiality, fluidity, elasticity, responsiveness to electric fields and controllable coupling of the molecular orientation at the interface with solid surfaces. The discovery of a polar nematic phase opens new possibilities for liquid crystal-based applications, but also requires a new study of how this phase couples with surfaces. Here we explore the surface alignment of the ferroelectric nematic phase by testing different rubbed and unrubbed substrates that differ in coupling strength and anchoring orientation and find a variety of behaviors – in terms of nematic orientation, topological defects and electric field response – that are specific to the ferroelectric nematic phase and can be understood as a consequence of the polar symmetry breaking. In particular, we show that by using rubbed polymer surfaces it is easy to produce cells with a planar polar preferential alignment and that cell electrostatics ( e.g. grounding the electrodes) has a remarkable effect on the overall homogeneity of the ferroelectric ordering.
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Liquid-crystal-based topological photonics
Liquid crystals are complex fluids that allow exquisite control of light propagation thanks to their orientational order and optical anisotropy. Inspired by recent advances in liquid-crystal photo-patterning technology, we propose a soft-matter platform for assembling topological photonic materials that holds promise for protected unidirectional waveguides, sensors, and lasers. Crucial to our approach is to use spatial variations in the orientation of the nematic liquid-crystal molecules to emulate the time modulations needed in a so-called Floquet topological insulator. The varying orientation of the nematic director introduces a geometric phase that rotates the local optical axes. In conjunction with suitably designed structural properties, this geometric phase leads to the creation of topologically protected states of light. We propose and analyze in detail soft photonic realizations of two iconic topological systems: a Su–Schrieffer–Heeger chain and a Chern insulator. The use of soft building blocks potentially allows for reconfigurable systems that exploit the interplay between topological states of light and the underlying responsive medium.
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- Award ID(s):
- 2011854
- PAR ID:
- 10313844
- Date Published:
- Journal Name:
- Proceedings of the National Academy of Sciences
- Volume:
- 118
- Issue:
- 4
- ISSN:
- 0027-8424
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
-
Accepted Manuscript
- Journal Article:
- https://doi.org/10.1073/pnas.2020525118
