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1. Biomass combustion produces ice-active minerals in biomass-burning aerosol and bottom ash

   https://doi.org/10.1073/pnas.1922128117  

   Jahn, Leif G.; Polen, Michael J.; Jahl, Lydia G.; Brubaker, Thomas A.; Somers, Joshua; Sullivan, Ryan C. (September 2020, Proceedings of the National Academy of Sciences)

   null (Ed.)

   Ice nucleation and the resulting cloud glaciation are significant atmospheric processes that affect the evolution of clouds and their properties including radiative forcing and precipitation, yet the sources and properties of atmospheric ice nucleants are poorly constrained. Heterogeneous ice nucleation caused by ice-nucleating particles (INPs) enables cloud glaciation at temperatures above the homogeneous freezing regime that starts near −35 °C. Biomass burning is a significant global source of atmospheric particles and a highly variable and poorly understood source of INPs. The nature of these INPs and how they relate to the fuel composition and its combustion are critical gaps in our understanding of the effects of biomass burning on the environment and climate. Here we show that the combustion process transforms inorganic elements naturally present in the biomass (not soil or dust) to form potentially ice-active minerals in both the bottom ash and emitted aerosol particles. These particles possess ice-nucleation activities high enough to be relevant to mixed-phase clouds and are active over a wide temperature range, nucleating ice at up to −13 °C. Certain inorganic elements can thus serve as indicators to predict the production of ice nucleants from the fuel. Combustion-derived minerals are an important but understudied source of INPs in natural biomass-burning aerosol emissions in addition to lofted primary soil and dust particles. These discoveries and insights should advance the realistic incorporation of biomass-burning INPs into atmospheric cloud and climate models. These mineral components produced in biomass-burning aerosol should also be studied in relation to other atmospheric chemistry processes, such as facilitating multiphase chemical reactions and nutrient availability. 

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2. Increasing boreal fires reduce future global warming and sea ice loss

   https://doi.org/10.1073/pnas.2424614122  

   Blanchard-Wrigglesworth, Edward; DeRepentigny, Patricia; Frierson, Dargan_M W (June 2025, Proceedings of the National Academy of Sciences)

   Biomass burning can affect climate via the emission of aerosols and their subsequent impact on radiation, cloud microphysics, and surface and atmospheric albedo. Biomass burning emissions (BBEs) over the boreal region have strongly increased during the last decade and are expected to continue increasing as the climate warms. Climate models simulate aerosol processes, yet historical and future Coupled Model Intercomparison Project (CMIP) simulations have no active fire component, and BBEs are prescribed as external forcings. Here, we show that CMIP6 used future boreal BBEs scenarios with unrealistic near-zero trends that have a large impact on climate trends. By running sensitivity experiments with ramped up boreal emissions based on observed trends, we find that increasing boreal BBEs reduces global warming by 12% and Arctic warming by 38%, reducing the loss of sea ice. Tropical precipitation shifts southward as a result of the hemispheric difference in boreal aerosol forcing and subsequent temperature response. These changes stem from the impact of aerosols on clouds, increasing cloud droplet number concentration, cloud optical depth, and low cloud cover, ultimately reducing surface shortwave flux over northern latitudes. Our results highlight the importance of realistic boreal BBEs in climate model simulations and the need for improved understanding of boreal emission trends and aerosol–climate interactions. 

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3. Ice‐Nucleating Particles Are Emitted by Raindrop Impact

   https://doi.org/10.1029/2024JD042584  

   Mignani, C; Hill, T_C J; Nieto‐Caballero, M; Barry, K R; Bryan, N C; Marinescu, P J; Dolan, B; Sullivan, A P; Hernandez, M; Bosco‐Lauth, A; et al (June 2025, Journal of Geophysical Research: Atmospheres)

   Abstract Ice‐nucleating particles (INPs) play a key role in ice formation and cloud microphysics and thus significantly impact the water cycle and the climate. However, our understanding of atmospheric INPs, particularly their sources, emissions, and spatiotemporal variability, is incomplete. While the enhancement of atmospheric INP concentrations with rainfall has been previously shown, a mechanistic understanding of the process is lacking. Here, we link detailed precipitation observations with near‐surface atmospheric INP concentrations at a semiarid grassland site in Colorado. Considering the during‐precipitation air samples, INP concentrations positively correlate with cumulative rainfall kinetic energy and amount, suggesting that INP aerosolization is induced by raindrop and hailstone impact. By additionally analyzing the INP content of precipitation water, terrestrial source samples, and heat‐treated samples, we demonstrate that local plants are the most plausible source of rain‐induced INPs during a precipitation event. Should INPs aerosolized by precipitation rise to cloud height, they could influence cloud ice fraction and initiate precipitation resulting in an aerosol‐cloud‐precipitation feedback. 

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4. Large changes in biomass burning over the last millennium inferred from paleoatmospheric ethane in polar ice cores

   https://doi.org/10.1073/pnas.1807172115  

   Nicewonger, Melinda R.; Aydin, Murat; Prather, Michael J.; Saltzman, Eric S. (December 2018, Proceedings of the National Academy of Sciences)

   Biomass burning drives changes in greenhouse gases, climate-forcing aerosols, and global atmospheric chemistry. There is controversy about the magnitude and timing of changes in biomass burning emissions on millennial time scales from preindustrial to present and about the relative importance of climate change and human activities as the underlying cause. Biomass burning is one of two notable sources of ethane in the preindustrial atmosphere. Here, we present ice core ethane measurements from Antarctica and Greenland that contain information about changes in biomass burning emissions since 1000 CE (Common Era). The biomass burning emissions of ethane during the Medieval Period (1000–1500 CE) were higher than present day and declined sharply to a minimum during the cooler Little Ice Age (1600–1800 CE). Assuming that preindustrial atmospheric reactivity and transport were the same as in the modern atmosphere, we estimate that biomass burning emissions decreased by 30 to 45% from the Medieval Period to the Little Ice Age. The timing and magnitude of this decline in biomass burning emissions is consistent with that inferred from ice core methane stable carbon isotope ratios but inconsistent with histories based on sedimentary charcoal and ice core carbon monoxide measurements. This study demonstrates that biomass burning emissions have exceeded modern levels in the past and may be highly sensitive to changes in climate. 

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5. Large changes in biomass burning over the last millennium inferred from paleoatmospheric ethane in polar ice cores

   Melinda R. Nicewonger, Murat Aydin (December 2018, Proceedings of the National Academy of Sciences of the United States of America)

   Biomass burning drives changes in greenhouse gases, climate-forcing aerosols, and global atmospheric chemistry. There is controversy about the magnitude and timing of changes in biomass burning emissions on millennial time scales from preindustrial to present and about the relative importance of climate change and human activities as the underlying cause. Biomass burning is one of two notable sources of ethane in the preindustrial atmosphere. Here, we present ice core ethane measurements from Antarctica and Greenland that contain information about changes in biomass burning emissions since 1000 CE (Common Era). The biomass burning emissions of ethane during the Medieval Period (1000-1500 CE) were higher than present day and declined sharply to a minimum during the cooler Little Ice Age (1600-1800 CE). Assuming that preindustrial atmospheric reactivity and transport were the same as in the modern atmosphere, we estimate that biomass burning emissions decreased by 30 to 45% from the Medieval Period to the Little Ice Age. The timing and magnitude of this decline in biomass burning emissions is consistent with that inferred from ice core methane stable carbon isotope ratios, but inconsistent with histories based on sedimentary charcoal and ice core carbon monoxide measurements. This study demonstrates that biomass burning emissions have exceeded modern levels in the past and may be highly sensitive to changes in climate. 

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