Solar-driven interfacial evaporation shows great prospects for seawater desalination with its rapid fast evaporation rate and high photothermal conversion efficiency. Here, a sustainable, biodegradable, non-toxic, and highly efficient full ocean biomass-based solar-driven evaporator is reported, which is composed of chitosan (CS) hydrogel as the hydratable skeleton and cuttlefish ink (CI) as the photothermal material. Under solar irradiation, the cuttlefish ink powder harvests solar energy and heats the surrounding water. Simultaneously, the water in the three-dimensional network of chitosan hydrogel is rapidly replenished by the interconnected porous structure and the hydrophilic functional groups attached to the polymer chains. With its enlarged evaporation surface, high solar absorptance, adequate water transportation, good salt drainage, and heat localization, the CI/CS-based evaporator achieves a remarkable evaporation rate of 4.1 kg m −2 h −1 under one sun irradiance (1 kW m −2 ) with high-quality freshwater yields. This full ocean biomass-based evaporator with abundant raw material availability provides new possibilities for an efficient, stable, sustainable, and environmentally friendly solar evaporator with guaranteed water quality.
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Sustainable off-grid desalination of hypersaline waters using Janus wood evaporators
Solar-thermal evaporation is a promising technology for energy-efficient desalination, but salt accumulation on solar absorbers and system longevity are the major challenges that hinder its widespread application. In this study, we present a sustainable Janus wood evaporator that overcomes these challenges and achieves a record-high evaporation efficiencies in hypersaline water, one of the most difficult water sources to treat via desalination. The Janus wood evaporator has asymmetric surface wettability, where the top layer acts as a hydrophobic solar absorber with water blockage and salt resistance, while the bottom hydrophilic wood layer allows for rapid water replenishment and superior thermal insulation. An evaporation efficiency of 82.0% is achieved for 20% NaCl solution under 1 sun, and persistent salt-resistance is observed during a 10-cycle long-term test. To ensure the environmental impact of the Janus wood evaporator, for the first time, a life cycle assessment (LCA) is conducted to compare this Janus wood evaporator with the emerging Janus evaporators, indicating a functional and more sustainable opportunity for off-grid desalination and humanitarian efforts.
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- Award ID(s):
- 2011750
- PAR ID:
- 10325158
- Date Published:
- Journal Name:
- Energy & Environmental Science
- Volume:
- 14
- Issue:
- 10
- ISSN:
- 1754-5692
- Page Range / eLocation ID:
- 5347 to 5357
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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