Title: Resonant light enhances phase coherence in a cavity QED simulator of fermionic superfluidity
Cavity QED experiments are natural hosts for non-equilibrium phases of matter supported by photon-mediated interactions. In this work, we consider a cavity QED simulation of the BCS model of superfluidity, by studying regimes where the cavity photons act as dynamical degrees of freedom instead of mere mediators of the interaction via virtual processes. We find an enhancement of long time coherence following a quench whenever the cavity frequency is tuned into resonance with the atoms. We discuss how this is equivalent to enhancement of non-equilibrium superfluidity and highlight similarities to an analogous phenomena recently studied in solid state quantum optics. We also discuss the conditions for observing this enhanced resonant pairing in experiments by including the effect of photon losses and inhomogeneous coupling in our analysis. more »« less
Arvanitaki, Asimina; Dimopoulos, Savas; Galanis, Marios; Racco, Davide; Simon, Olivier; Thompson, Jedidiah O.(
, Journal of High Energy Physics)
A<sc>bstract</sc>
One contribution to any dark sector’s abundance comes from its gravitational production during inflation. If the dark sector is weakly coupled to the inflaton and the Standard Model, this can be its only production mechanism. For non-interacting dark sectors, such as a free massive fermion or a free massive vector field, this mechanism has been studied extensively. In this paper we show, via the example of dark massive QED, that the presence of interactions can result in a vastly different mass for the dark matter (DM) particle, which may well coincide with the range probed by upcoming experiments.
In the context of dark QED we study the evolution of the energy density in the dark sector after inflation. Inflation produces a cold vector condensate consisting of an enormous number of bosons, which via interesting processes — Schwinger pair production, strong field electromagnetic cascades, and plasma dynamics — transfers its energy to a small number of “dark electrons” and triggers thermalization of the dark sector. The resulting dark electron DM mass range is from 50 MeV to 30 TeV, far different from both the 10−5eV mass of the massive photon dark matter in the absence of dark electrons, and from the 109GeV dark electron mass in the absence of dark photons. This can significantly impact the search strategies for dark QED and, more generally, theories with a self-interacting DM sector. In the presence of kinetic mixing, a dark electron in this mass range can be searched for with upcoming direct detection experiments, such as SENSEI-100g and OSCURA.
Roso, Luis; Lera, Roberto; Ravichandran, Smrithan; Longman, Andrew; He, Calvin Z.; Pérez-Hernández, José Antonio; Apiñaniz, Jon I.; Smith, Lucas D.; Fedosejevs, Robert; Hill, III, Wendell T.(
, New Journal of Physics)
Abstract
In this paper we will show that photon–photon collision experiments using extreme lasers can provide measurable effects giving fundamental information about the essence of QED, its Lagrangian. A possible scenario with two counterpropagating ultra-intense lasers for an experiment to detect scattering between optical photons is analyzed. We discuss the importance of the pulse widths and waists, the best scenario for overlapping the beams and signal detection, as well as ways to distinguish the signal from the noise. This would need a high-precision measurement, with control of temporal jitter and noise. We conclude that such experiment is barely feasible at 1023 W cm−2and very promising at 1024 W cm−2.
We report the development of a composite cavity QED system, in which silicon vacancy centers in a diamond membrane as thin as 100 nm couple to optical whispering gallery modes (WGMs) of a silica microsphere with a diameter of order 50 µm. The membrane induces a linewidth broadening of 3 MHz for equatorial and off-resonant WGMs, while the overall linewidth of the composite system remains below 40 MHz. Photoluminescence experiments in the cavity QED setting demonstrate the efficient coupling of optical emissions from silicon vacancy centers into the WGMs. Additional analysis indicates that the composite system can be used to achieve the good cavity limit in cavity QED, enabling an experimental platform for applications such as state transfer between spins and photons.
Amaladhasan, Dalrin Ampritta; Heyn, Claudia; Hoyle, Christopher R.; El Haddad, Imad; Elser, Miriam; Pieber, Simone M.; Slowik, Jay G.; Amorim, Antonio; Duplissy, Jonathan; Ehrhart, Sebastian; et al(
, Atmospheric Chemistry and Physics)
Abstract. This study presents a characterization of the hygroscopic growth behaviour and effects of different inorganic seed particles on the formation of secondary organic aerosols (SOAs) from the dark ozone-initiated oxidation of isoprene at low NOx conditions. We performed simulations of isoprene oxidation using a gas-phase chemical reaction mechanism based onthe Master Chemical Mechanism (MCM) in combination with an equilibriumgas–particle partitioning model to predict the SOA concentration. Theequilibrium model accounts for non-ideal mixing in liquid phases, includingliquid–liquid phase separation (LLPS), and is based on the AIOMFAC (Aerosol Inorganic–Organic Mixtures Functional groups Activity Coefficients) model for mixture non-ideality and the EVAPORATION (Estimation of VApour Pressure of ORganics, Accounting for Temperature,Intramolecular, and Non-additivity effects) model for pure compound vapourpressures. Measurements from the Cosmics Leaving Outdoor Droplets (CLOUD)chamber experiments, conducted at the European Organization for NuclearResearch (CERN) for isoprene ozonolysis cases, were used to aid inparameterizing the SOA yields at different atmospherically relevanttemperatures, relative humidity (RH), and reacted isoprene concentrations. To represent the isoprene-ozonolysis-derived SOA, a selection of organicsurrogate species is introduced in the coupled modelling system. The modelpredicts a single, homogeneously mixed particle phase at all relativehumidity levels for SOA formation in the absence of any inorganic seedparticles. In the presence of aqueous sulfuric acid or ammonium bisulfateseed particles, the model predicts LLPS to occur below ∼ 80 % RH, where the particles consist of an inorganic-rich liquid phase andan organic-rich liquid phase; however, this includes significant amounts of bisulfate and water partitioned to the organic-rich phase. The measurements show an enhancement in the SOA amounts at 85 % RH, compared to 35 % RH, for both the seed-free and seeded cases. The model predictions of RH-dependent SOA yield enhancements at 85 % RH vs. 35 % RH are 1.80 for a seed-free case, 1.52 for the case with ammonium bisulfate seed, and 1.06 for the case with sulfuric acid seed. Predicted SOA yields are enhanced in the presence of an aqueous inorganic seed, regardless of the seed type (ammonium sulfate, ammonium bisulfate, or sulfuric acid) in comparison with seed-free conditions at the same RH level. We discuss the comparison of model-predicted SOA yields with a selection of other laboratory studies on isoprene SOA formation conducted at different temperatures and for a variety of reacted isoprene concentrations. Those studies were conducted at RH levels at or below 40 % with reported SOA mass yields ranging from 0.3 % up to 9.0 %, indicating considerable variations. A robust feature of our associated gas–particle partitioning calculations covering the whole RH range is the predicted enhancement of SOA yield at high RH (> 80 %) compared to low RH (dry) conditions, which is explained by the effect of particle water uptake and its impact on the equilibrium partitioning of all components.
Recent experiments demonstrate the control of chemical reactivities by coupling molecules inside an optical microcavity. In contrast, transition state theory predicts no change of the reaction barrier height during this process. Here, we present a theoretical explanation of the cavity modification of the ground state reactivity in the vibrational strong coupling (VSC) regime in polariton chemistry. Our theoretical results suggest that the VSC kinetics modification is originated from the non-Markovian dynamics of the cavity radiation mode that couples to the molecule, leading to the dynamical caging effect of the reaction coordinate and the suppression of reaction rate constant for a specific range of photon frequency close to the barrier frequency. We use a simple analytical non-Markovian rate theory to describe a single molecular system coupled to a cavity mode. We demonstrate the accuracy of the rate theory by performing direct numerical calculations of the transmission coefficients with the same model of the molecule-cavity hybrid system. Our simulations and analytical theory provide a plausible explanation of the photon frequency dependent modification of the chemical reactivities in the VSC polariton chemistry.
Kelly, S.P., Thompson, J.K., Rey, A.M., and Marino, J. Resonant light enhances phase coherence in a cavity QED simulator of fermionic superfluidity. Retrieved from https://par.nsf.gov/biblio/10341875. ArXivorg .10.48550/arXiv.2202.05851 Web. doi:10.48550/arXiv.2202.05851.
Kelly, S.P., Thompson, J.K., Rey, A.M., & Marino, J. Resonant light enhances phase coherence in a cavity QED simulator of fermionic superfluidity. ArXivorg, (10.48550/arXiv.2202.05851). Retrieved from https://par.nsf.gov/biblio/10341875. https://doi.org/10.48550/arXiv.2202.05851
@article{osti_10341875,
place = {Country unknown/Code not available},
title = {Resonant light enhances phase coherence in a cavity QED simulator of fermionic superfluidity},
url = {https://par.nsf.gov/biblio/10341875},
DOI = {10.48550/arXiv.2202.05851},
abstractNote = {Cavity QED experiments are natural hosts for non-equilibrium phases of matter supported by photon-mediated interactions. In this work, we consider a cavity QED simulation of the BCS model of superfluidity, by studying regimes where the cavity photons act as dynamical degrees of freedom instead of mere mediators of the interaction via virtual processes. We find an enhancement of long time coherence following a quench whenever the cavity frequency is tuned into resonance with the atoms. We discuss how this is equivalent to enhancement of non-equilibrium superfluidity and highlight similarities to an analogous phenomena recently studied in solid state quantum optics. We also discuss the conditions for observing this enhanced resonant pairing in experiments by including the effect of photon losses and inhomogeneous coupling in our analysis.},
journal = {ArXivorg},
number = {10.48550/arXiv.2202.05851},
author = {Kelly, S.P. and Thompson, J.K. and Rey, A.M. and Marino, J},
}
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