Spin defects in hexagonal boron nitride, and specifically the negatively charged boron vacancy (VB‐) centers, are emerging candidates for quantum sensing. However, the VB‐defects suffer from low quantum efficiency and, as a result, exhibit weak photoluminescence. In this work, a scalable approach is demonstrated to dramatically enhance the VB‐emission by coupling to a plasmonic gap cavity. The plasmonic cavity is composed of a flat gold surface and a silver cube, with few‐layer hBN flakes positioned in between. Employing these plasmonic cavities, two orders of magnitude are extracted in photoluminescence enhancement associated with a corresponding twofold enhancement in optically detected magnetic resonance contrast. The work will be pivotal to progress in quantum sensing employing 2D materials, and in realization of nanophotonic devices with spin defects in hexagonal boron nitride.
- Award ID(s):
- 2110591
- PAR ID:
- 10346213
- Date Published:
- Journal Name:
- Photonics
- Volume:
- 9
- Issue:
- 2
- ISSN:
- 2304-6732
- Page Range / eLocation ID:
- 61
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
Abstract -
A variety of pulse sequences have been described for converting nuclear spin magnetisation into long-lived singlet order for nuclear spin-1/2 pairs. Existing sequences operate well in two extreme parameter regimes. The magnetisation-to-singlet (M2S) pulse sequence performs a robust conversion of nuclear spin magnetisation into singlet order in the near-equivalent limit, meaning that the difference in chemical shift frequencies of the two spins is much smaller than the spin–spin coupling. Other pulse sequences operate in the strong-inequivalence regime, where the shift difference is much larger than the spin–spin coupling. However both sets of pulse sequences fail in the intermediate regime, where the chemical shift difference and the spin–spin coupling are roughly equal in magnitude. We describe a generalised version of M2S, called gM2S, which achieves robust singlet order excitation for spin systems ranging from the near-equivalence limit well into the intermediate regime. This closes an important gap left by existing pulse sequences. The efficiency of the gM2S sequence is demonstrated numerically and experimentally for near-equivalent and intermediate-regime cases.more » « less
-
Photon-mediated interactions between quantum systems are essential for realizing quantum networks and scalable quantum information processing. We demonstrate such interactions between pairs of silicon-vacancy (SiV) color centers coupled to a diamond nanophotonic cavity. When the optical transitions of the two color centers are tuned into resonance, the coupling to the common cavity mode results in a coherent interaction between them, leading to spectrally resolved superradiant and subradiant states. We use the electronic spin degrees of freedom of the SiV centers to control these optically mediated interactions. Such controlled interactions will be crucial in developing cavity-mediated quantum gates between spin qubits and for realizing scalable quantum network nodes.
-
Abstract Deterministic positioning single site-controlled high symmetric InGaAs quantum dots (QDs) in (111)B-oriented GaAs photonic crystal cavities with nanometer-scale accuracy provides an idea component for building integrated quantum photonic circuits. However, it has been a long-standing challenge of improving cavity
Q -factors in such systems. Here, by optimizing the trade-off between the cavity loss and QD spectral quality, we demonstrate our site-controlled QD-nanocavity system operating in the intermediate coupling regime mediated by phonon scattering, with the dynamic coexistence of strong and weak coupling. The cavity-exciton detuning-dependent micro-photoluminescence spectrum reveals concurrence of a trend of exciton-polariton mode avoided crossing, as a signature of Rabi doublet of the strongly coupled system. Meanwhile, a trend of keeping constant or slight blue shift of coupled exciton–cavity mode(CM) energy across zero-detuning is ascribed to the formation of collective states mediated by phonon-assisted coupling, and their rare partial out-of-synchronization linewidth-narrowing is linked to their coexisting strong-weak coupling regime. We further reveal the pump power-dependent anti-bunching photon statistical dynamics of this coexisting strong-weak coupled system and the optical features of strongly confined exciton-polaritons, and dark-exciton-like states. These observations demonstrate the potential capabilities of site-controlled QD-cavity systems as deterministic quantum nodes for on-chip quantum information processing and provide guidelines for future device optimization for achieving the strong coupling regime. -
Abstract Optical forces are known to arise in a universal fashion in many and diverse physical settings. As such, they are successfully employed over a wide range of applications in areas like biophotonics, optomechanics and integrated optics. While inter-elemental optical forces in few-mode photonic networks have been so far systematically analyzed, little is known, if any, as to how they manifest themselves in highly multimoded optical environments. In this work, by means of statistical mechanics, we formally address this open problem in optically thermalized weakly nonlinear heavily multimode tight-binding networks. The outlined thermodynamic formulation allows one to obtain in an elegant manner analytical results for the exerted thermodynamic pressures in utterly complex arrangements-results that are either computationally intensive or impossible to obtain otherwise. Thus, we derive simple closed-form expressions for the thermodynamic optical pressures displayed among elements, which depend only on the internal energy as well as the coupling coefficients involved. In all cases, our theoretical results are in excellent agreement with numerical computations. Our study may pave the way towards a deeper understanding of these complex processes and could open up avenues in harnessing radiation forces in multimode optomechanical systems.more » « less