An official website of the United States government
We propose a method to adiabatically control an atomic ensemble using a decoherence-free subspace (DFS) within a dissipative cavity. We can engineer a specific eigenstate of the system's Lindblad jump operators by injecting a field into the cavity which deconstructively interferes with the emission amplitude of the ensemble. In contrast to previous adiabatic DFS proposals, our scheme creates a DFS in the presence of collective decoherence. We therefore have the ability to engineer states that have high multi-particle entanglements which may be exploited for quantum information science or metrology. We further demonstrate a more optimized driving scheme that utilizes the knowledge of possible diabatic evolution gained from the so-called adiabatic criteria. This allows us to evolve to a desired state with exceptionally high fidelity on a time scale that does not depend on the number of atoms in the ensemble. By engineering the DFS eigenstate adiabatically, our method allows for faster state preparation than previous schemes that rely on damping into a desired state solely using dissipation.
more »
« less
A proposed test of quantum dissipation theory using Kapitza–Dirac electron diffraction
Abstract Decoherence can be provided by a dissipative environment as described by the Caldeira–Leggett equation. This equation is foundational to the theory of quantum dissipation. However, no experimental test has been performed that measures for one physical system both the dissipation and the decoherence. Anglin and Zurek predicted that a resistive surface could provide such a dissipative environment for a free electron wave passing close to it. We propose that the electron wave’s coherence and energy loss can be measured simultaneously by using Kapitza–Dirac scattering for varying light intensity.
more »
« less
- Award ID(s):
- 1912504
- PAR ID:
- 10346941
- Date Published:
- Journal Name:
- New Journal of Physics
- Volume:
- 24
- Issue:
- 6
- ISSN:
- 1367-2630
- Page Range / eLocation ID:
- 063033
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Abstract Analytical solutions for 2D and slab turbulence energies in the solar corona are presented, including a derivation of the corresponding correlation lengths, with implications for the proton and electron temperatures in the solar corona. These solutions are derived by solving the transport equations for 2D and slab turbulence energies and their correlation lengths, as well as proton and electron pressures. The solutions assume background profiles for the solar wind speed, solar wind mass density, and Alfvén velocity. Our analytical solutions can be related to those obtained from joint Parker Solar Probe and Solar Orbiter Metis coronagraph observations, as reported in Telloni et al. We find that the solution for 2D turbulence energy in the absence of nonlinear dissipation decreases more slowly compared to the dissipative solution. The solution for slab turbulence energy with no dissipation exhibits a more rapid increase compared to the dissipative solution. The proton heating rate is found to be about 82% of the total plasma heating rate at 6.3R⊙, which gradually decreases with increasing distance, eventually becoming ∼80% of the total plasma heating rate at ∼13R⊙, consistent with that found by Bandyopadhyay et al. (2023). These analytical solutions provide valuable insight for our understanding of turbulence, and its effect on proton and electron heating rates, in the solar corona. We compare the numerically solved turbulent transport equations for the 2D and slab turbulence energies, correlation lengths, and proton and electron pressures with the analytical solutions, finding good agreement between them.more » « less
-
Photoluminescence (PL) is one of the key experimental characterizations of optoelectronic materials, including conjugated polymers (CPs). In this study, a simplified model of an undoped cis-polyacetylene (cis-PA) oligomer was selected and used to explain the mechanism of photoluminescence (PL) of the CPs. Using a combination of the ab initio electronic structure and a time-dependent density matrix methodology, the photo-induced time-dependent excited state dynamics were computed. We explored the phonon-induced relaxation of the photoexcited state for a single oligomer of cis-PA. Here, the dissipative Redfield equation of the motion was used to compute the dissipative excited state dynamics of electronic degrees of freedom. This equation used the nonadiabatic couplings as parameters. The computed excited state dynamics showed that the relaxation rate of the electron is faster than the relaxation rate of the hole. The dissipative excited-state dynamics were combined with radiative recombination channels to predict the PL spectrum. The simulated results showed that the absorption and emission spectra both have a similar transition. The main result is that the computed PL spectrum demonstrates two mechanisms of light emission originating from (i) the inter-band transitions, corresponding to the same range of transition energies as the absorption spectrum and (ii) intra-band transitions not available in the absorption spectra. However, the dissipative Redfield equation of the motion was used to compute the electronic degrees of freedom of the nonadiabatic couplings, which helped to process the time propagation of the excited dynamic state. This excited dynamic state shows that the relaxation rate of the electron is faster than the relaxation rate of the hole, which can be used for improving organic semiconductor materials for photovoltaic and LED applications.more » « less
-
Long electron spin coherence lifetimes are crucial for high sensitivity and resolution in many pulse electron paramagnetic resonance (EPR) experiments aimed at measuring hyperfine and dipolar couplings, as well as in potential quantum sensing applications of molecular spin qubits. In immobilized systems, methyl groups contribute significantly to electron spin decoherence as a result of methyl torsional quantum tunneling. We examine the electron spin decoherence dynamics of the nitroxide radical 2,2,6,6-tetramethylpiperidin-1-oxyl (TEMPO) in both a methyl-free solvent and a methyl-containing solvent at cryogenic temperature. We model nitroxide and solvent methyl effects on decoherence using cluster correlation expansion (CCE) simulations extended to include methyl tunneling and compare the calculations to experimental data. We show that by using the methyl tunneling frequency as a fit parameter, experimental Hahn echo decays can be reproduced fairly well, allowing structural properties to be investigated in silico. In addition, we examine the Hahn echo of a hypothetical system with an unpaired electron and a single methyl to determine the effect of geometric configuration on methyl-driven electron spin decoherence. The simulations show that a methyl group contributes the most to electron spin decoherence if it is located between 2.5 and 6–7 Å from the electron spin, with its orientation being of secondary importance.more » « less
-
Abstract We study quantum decoherence numerically in a system consisting of a relativistic quantum field theory coupled to a measuring device that is itself coupled to an environment. The measuring device and environment are treated as quantum, non-relativistic particles. We solve the Schrödinger equation for the wave function of this tripartite system using exact diagonalization. Although computational limitations on the size of the Hilbert space prevent us from exploring the regime where the device and environment consist of a truly macroscopic number of degrees of freedom, we nevertheless see clear evidence of decoherence: after tracing out the environment, the density matrix describing the system and measuring device evolves quickly towards a matrix that is close to diagonal in a subspace of pointer states. We measure the speed with which decoherence spreads in the relativistic quantum field theory for a range of parameters. We find that it is less than the speed of light but faster than the speed of the massive charges in the initial state.more » « less
- Free Publicly Accessible Full Text
-
Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1088/1367-2630/ac79c4
