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Abstract Controls on pristine aerosol over the Southern Ocean (SO) are critical for constraining the strength of global aerosol indirect forcing. Observations of summertime SO clouds and aerosols in synoptically varied conditions during the 2018 SOCRATES aircraft campaign reveal novel mechanisms influencing pristine aerosol‐cloud interactions. The SO free troposphere (3–6 km) is characterized by widespread, frequent new particle formation events contributing to much larger concentrations (≥1,000 mg⁻¹) of condensation nuclei (diameters > 0.01 μm) than in typical sub‐tropical regions. Synoptic‐scale uplift in warm conveyor belts and sub‐polar vortices lifts marine biogenic sulfur‐containing gases to free‐tropospheric environments favorable for generating Aitken‐mode aerosol particles (0.01–0.1 μm). Free‐tropospheric Aitken particles subside into the boundary layer, where they grow in size to dominate the sulfur‐based cloud condensation nuclei (CCN) driving SO cloud droplet number concentrations (N_d ∼ 60–100 cm⁻³). Evidence is presented for a hypothesized Aitken‐buffering mechanism which maintains persistently high summertime SON_dagainst precipitation removal through CCN replenishment from activation and growth of boundary layer Aitken particles. Nudged hindcasts from the Community Atmosphere Model (CAM6) are found to underpredict Aitken and accumulation mode aerosols andN_d, impacting summertime cloud brightness and aerosol‐cloud interactions and indicating incomplete representations of aerosol mechanisms associated with ocean biology. 

Abstract Stratocumulus clouds over the Southern Ocean have fewer droplets and are more likely to exist in the predominately supercooled phase than clouds at similar temperatures over northern oceans. One likely reason is that this region has few continental and anthropogenic sources of cloud‐nucleating particles that can form droplets and ice. In this work, we present an overview of aerosol particle types over the Southern Ocean, including new measurements made below, in and above clouds in this region. These measurements and others indicate that biogenic sulfur‐based particles >0.1 μm diameter contribute the majority of cloud condensation nuclei number concentrations in summer. Ice nucleating particles tend to have more organic components, likely from sea‐spray. Both types of cloud nucleating particles may increase in a warming climate likely to have less sea ice, more phytoplankton activity, and stronger winds over the Southern Ocean near Antarctica. Taken together, clouds over the Southern Ocean may become more reflective and partially counter the region's expected albedo decrease due to diminishing sea ice. However, detailed modeling studies are needed to test this hypothesis due to the complexity of ocean‐cloud‐climate feedbacks in the region. 

Abstract Modeling the shortwave radiation balance over the Southern Ocean region remains a challenge for Earth system models. To investigate whether this is related to the representation of aerosol‐cloud interactions, we compared measurements of the total number concentration of sea spray‐generated particles within the Southern Ocean region to model predictions thereof. Measurements were conducted from a container laboratory aboard the R/VTangaroathroughout an austral summer voyage to the Ross Sea. We used source‐receptor modeling to calculate the sensitivity of our measurements to upwind surface fluxes. From this approach, we could constrain empirical parameterizations of sea spray surface flux based on surface wind speed and sea surface temperature. A newly tuned parameterization for the flux of sea spray particles based on the near‐surface wind speed is presented. Comparisons to existing model parameterizations revealed that present model parameterizations led to overestimations of sea spray concentrations. In contrast to previous studies, we found that including sea surface temperature as an explanatory variable did not substantially improve model‐measurement agreement. To test whether or not the parameterization may be applicable globally, we conducted a regression analysis using a database of in situ whitecap measurements. We found that the key fitting parameter within this regression agreed well with the parameterization of sea spray flux. Finally, we compared calculations from the best model of surface flux to boundary layer measurements collected onboard an aircraft throughout the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES), finding good agreement overall. 

Abstract The bulk microphysical properties and number distribution functions (N(D)) of supercooled liquid water (SLW) and ice inside and between ubiquitous generating cells (GCs) observed over the Southern Ocean (SO) during the Southern Ocean Clouds Radiation Aerosol Transport Experimental Study (SOCRATES) measured by in situ cloud probes onboard the NCAR/NSF G‐V aircraft are compared. SLW was detected inside all GCs with an average liquid water content of 0.31 ± 0.19 g m⁻³, 11% larger than values between GCs. TheN(D)of droplets (maximum dimensionD < 50 μm) inside and between GCs had only slight differences. For ice particles, on the other hand, the mean concentration (median mass diameter) withD > 200 μm inside GCs was 2.0 ± 3.3 L⁻¹(323 ± 263 μm), 65% (37%) larger than values outside GCs. AsDincreases, the percentage differences became larger (up to ~500%). The more and larger ice particles inside GCs suggest the GC updrafts provide a favorable environment for particle growth by deposition and riming and that mixing processes are less efficient at redistributing larger particles. The horizontal scale of observed GCs ranged from 200 to 600 m with a mean of 395 ± 162 m, smaller than GC widths observed in previous studies. This study expands knowledge of the microphysical properties and processes acting in GCs over a wider range of conditions than previously available. 

Abstract Weather and climate models are challenged by uncertainties and biases in simulating Southern Ocean (SO) radiative fluxes that trace to a poor understanding of cloud, aerosol, precipitation and radiative processes, and their interactions. Projects between 2016 and 2018 used in-situ probes, radar, lidar and other instruments to make comprehensive measurements of thermodynamics, surface radiation, cloud, precipitation, aerosol, cloud condensation nuclei (CCN) and ice nucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase cloudsnucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase clouds common to this pristine environment. Data including soundings were collected from the NSF/NCAR G-V aircraft flying north-south gradients south of Tasmania, at Macquarie Island, and on the RV Investigator and RSV Aurora Australis. Synergistically these data characterize boundary layer and free troposphere environmental properties, and represent the most comprehensive data of this type available south of the oceanic polar front, in the cold sector of SO cyclones, and across seasons. Results show a largely pristine environments with numerous small and few large aerosols above cloud, suggesting new particle formation and limited long-range transport from continents, high variability in CCN and cloud droplet concentrations, and ubiquitous supercooled water in thin, multi-layered clouds, often with small-scale generating cells near cloud top. These observations demonstrate how cloud properties depend on aerosols while highlighting the importance of confirmed low clouds were responsible for radiation biases. The combination of models and observations is examining how aerosols and meteorology couple to control SO water and energy budgets.