More Like this

1. Electrically powered motions of toron crystallites in chiral liquid crystals

   https://doi.org/10.1073/pnas.1922198117  

   Sohn, Hayley R. O. ; Smalyukh, Ivan I. ( March 2020 , Proceedings of the National Academy of Sciences)

   Malleability of metals is an example of how the dynamics of defects like dislocations induced by external stresses alters material properties and enables technological applications. However, these defects move merely to comply with the mechanical forces applied on macroscopic scales, whereas the molecular and atomic building blocks behave like rigid particles. Here, we demonstrate how motions of crystallites and the defects between them can arise within the soft matter medium in an oscillating electric field applied to a chiral liquid crystal with polycrystalline quasi-hexagonal arrangements of self-assembled topological solitons called “torons.” Periodic oscillations of electric field applied perpendicular to the plane of hexagonal lattices prompt repetitive shear-like deformations of the solitons, which synchronize the electrically powered self-shearing directions. The temporal evolution of deformations upon turning voltage on and off is not invariant upon reversal of time, prompting lateral translations of the crystallites of torons within quasi-hexagonal periodically deformed lattices. We probe how these motions depend on voltage and frequency of oscillating field applied in an experimental geometry resembling that of liquid crystal displays. We study the interrelations between synchronized deformations of the soft solitonic particles and their arrays, and the ensuing dynamics and giant number fluctuations mediated by motions ofmore »crystallites, five–seven defects pairs, and grain boundaries in the orderly organizations of solitons. We discuss how our findings may lead to technological and fundamental science applications of dynamic self-assemblies of topologically protected but highly deformable particle-like solitons.

   « less
2. Topological transformations of Hopf solitons in chiral ferromagnets and liquid crystals

   https://doi.org/10.1073/pnas.1716887115  

   Tai, Jung-Shen B. ; Ackerman, Paul J. ; Smalyukh, Ivan I. ( January 2018 , Proceedings of the National Academy of Sciences)

   Liquid crystals are widely known for their facile responses to external fields, which forms a basis of the modern information display technology. However, switching of molecular alignment field configurations typically involves topologically trivial structures, although singular line and point defects often appear as short-lived transient states. Here, we demonstrate electric and magnetic switching of nonsingular solitonic structures in chiral nematic and ferromagnetic liquid crystals. These topological soliton structures are characterized by Hopf indices, integers corresponding to the numbers of times that closed-loop-like spatial regions (dubbed “preimages”) of two different single orientations of rod-like molecules or magnetization are linked with each other. We show that both dielectric and ferromagnetic response of the studied material systems allow for stabilizing a host of topological solitons with different Hopf indices. The field transformations during such switching are continuous when Hopf indices remain unchanged, even when involving transformations of preimages, but discontinuous otherwise.
3. Multiplicative topological phases

   https://doi.org/10.1038/s42005-022-01022-x  

   Cook, Ashley M. ; Moore, Joel E. ( October 2022 , Communications Physics)

   Symmetry-protected topological phases of matter have challenged our understanding of condensed matter systems and harbour exotic phenomena promising to address major technological challenges. Considerable understanding of these phases of matter has been gained recently by considering additional protecting symmetries, different types of quasiparticles, and systems out of equilibrium. Here, we show that symmetries could be enforced not just on full Hamiltonians, but also on their components. We construct a large class of previously unidentified multiplicative topological phases of matter characterized by tensor product Hilbert spaces similar to the Fock space of multiple particles. To demonstrate our methods, we introduce multiplicative topological phases of matter based on the foundational Hopf and Chern insulator phases, the multiplicative Hopf and Chern insulators (MHI and MCI), respectively. The MHI shows the distinctive properties of the parent phases as well as non-trivial topology of a child phase. We also comment on a similar structure in topological superconductors as these multiplicative phases are protected in part by particle-hole symmetry. The MCI phase realizes topologically protected gapless states that do not extend from the valence bands to the conduction bands for open boundary conditions, which respects to the symmetries protecting topological phase. The band connectivity discoveredmore »in MCI could serve as a blueprint for potential multiplicative topology with exotic properties.

   « less
4. Electrically driven three-dimensional solitary waves as director bullets in nematic liquid crystals

   https://doi.org/10.1038/s41467-018-05101-y  

   Li, Bing-Xiang ; Borshch, Volodymyr ; Xiao, Rui-Lin ; Paladugu, Sathyanarayana ; Turiv, Taras ; Shiyanovskii, Sergij V. ; Lavrentovich, Oleg D. ( July 2018 , Nature Communications)

   Electric field-induced collective reorientation of nematic molecules is of importance for fundamental science and practical applications. This reorientation is either homogeneous over the area of electrodes, as in displays, or periodically modulated, as in electroconvection. The question is whether spatially localized three-dimensional solitary waves of molecular reorientation could be created. Here we demonstrate that the electric field can produce particle-like propagating solitary waves representing self-trapped “bullets” of oscillating molecular director. These director bullets lack fore-aft symmetry and move with very high speed perpendicularly to the electric field and to the initial alignment direction. The bullets are true solitons that preserve spatially confined shapes and survive collisions. The solitons are topologically equivalent to the uniform state and have no static analogs, thus exhibiting a particle–wave duality. Their shape, speed, and interactions depend strongly on the material parameters, which opens the door for a broad range of future studies.
5. Surface anchoring as a control parameter for stabilizing torons, skyrmions, twisted walls, fingers and their hybrids in chiral nematics

   Tai, Jung-Shen ; Smalyukh, Ivan I. ( January 2020 , Physical review)

   Chiral condensed matter systems, such as liquid crystals and magnets, exhibit a host of spatially localized topological structures that emerge from the medium’s tendency to twist and its competition with confinement and field coupling effects. We show that the strength of perpendicular surface boundary conditions can be used to control the structure and topology of solitonic and other localized field configurations. By combining numerical modeling and threedimensional imaging of the director field, we reveal structural stability diagrams and intertransformation of twisted walls and fingers, torons and skyrmions and their crystalline organizations upon changing boundary conditions. Our findings provide a recipe for controllably realizing skyrmions, torons and hybrid solitonic structures possessing features of both of them, which will aid in fundamental explorations and technological uses of such topological solitons. Moreover, with limited examples, we discuss how similar principles can be systematically used to tune stability of twisted walls versus cholesteric fingers and hopfions versus skyrmions, torons and twistions.