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  • One-step biosynthesis of a bilayered graphene oxide embedded bacterial nanocellulose hydrogel for versatile photothermal membrane applications
Title: One-step biosynthesis of a bilayered graphene oxide embedded bacterial nanocellulose hydrogel for versatile photothermal membrane applications
We introduce the facile one-step biosynthesis of a bilayer structured hydrogel composite of reduced-graphene oxide (rGO) and bacterial nanocellulose (BNC) for multiple photothermal water treatment applications. One-step in situ biosynthesis of a bilayered hydrogel was achieved via modification of BNC growth medium supplemented with an optimized concentration of corn steep liquor as a growth enhancer. A two-stage, growth rate-controlled formation mechanism for the bilayer structure was revealed. The final cleaned and freeze-dried reduced-GO embedded BNC bilayer membrane enables versatile applications such as filtration (tested using gold nanoparticles, Escherichia coli cells, and plasmid DNA), photothermal disinfection of entrapped E. coli , and solar water evaporation. Comparable particle rejection (up to ≈4 nm) and water flux (146 L h −1 m −2 ) to ultrafiltration were observed. Entrapment and photothermal inactivation of E. coli cells were accomplished within 10 min of solar exposure (one sun). Such treatment can potentially suppress membrane biofouling. The steam generation capacity was 1.96 kg m −2 h −1 . Our simple and scalable approach opens a new path for biosynthesis of nanostructured materials for environmental and biomedical applications.  more » « less
Award ID(s):
1545756
PAR ID:
10386327
Author(s) / Creator(s):
; ; ; ;
Date Published:
Journal Name:
Environmental Science: Nano
Volume:
9
Issue:
5
ISSN:
2051-8153
Page Range / eLocation ID:
1639 to 1650
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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