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1. Observations of clouds, aerosols, precipitation, and surface radiation over the Southern Ocean: An overview of CAPRICORN, MARCUS, MICRE and SOCRATES

   https://doi.org/10.1175/BAMS-D-20-0132.1  

   McFarquhar, Greg M. ; Bretherton, Chris ; Marchand, Roger ; Protat, Alain ; DeMott, Paul J. ; Alexander, Simon P. ; Roberts, Greg C. ; Twohy, Cynthia H. ; Toohey, Darin ; Siems, Steve ; et al ( November 2020 , Bulletin of the American Meteorological Society)

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   Abstract Weather and climate models are challenged by uncertainties and biases in simulating Southern Ocean (SO) radiative fluxes that trace to a poor understanding of cloud, aerosol, precipitation and radiative processes, and their interactions. Projects between 2016 and 2018 used in-situ probes, radar, lidar and other instruments to make comprehensive measurements of thermodynamics, surface radiation, cloud, precipitation, aerosol, cloud condensation nuclei (CCN) and ice nucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase cloudsnucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase clouds common to this pristine environment. Data including soundings were collected from the NSF/NCAR G-V aircraft flying north-south gradients south of Tasmania, at Macquarie Island, and on the RV Investigator and RSV Aurora Australis. Synergistically these data characterize boundary layer and free troposphere environmental properties, and represent the most comprehensive data of this type available south of the oceanic polar front, in the cold sector of SO cyclones, and across seasons. Results show a largely pristine environments with numerous small and few large aerosols above cloud, suggesting new particle formation and limited long-range transport from continents, high variability in CCN and cloud droplet concentrations, and ubiquitous supercooled water in thin, multi-layered clouds, often with small-scale generating cells near cloud top. These observations demonstrate how cloud properties depend on aerosols while highlighting the importance of confirmed low clouds were responsible for radiation biases. The combination of models and observations is examining how aerosols and meteorology couple to control SO water and energy budgets. 

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2. Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA)

   Wang, Jian ; Dong, Xiquan et ( January 2021 , Bulletin of the American Meteorological Society)

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   With their extensive coverage, marine low clouds greatly impact global climate. Presently, marine low clouds are poorly represented in global climate models, and the response of marine low clouds to changes in atmospheric greenhouse gases and aerosols remains the major source of uncertainty in climate simulations. The Eastern North Atlantic (ENA) is a region of persistent but diverse subtropical marine boundary layer clouds, whose albedo and precipitation are highly susceptible to perturbations in aerosol properties. In addition, the ENA is periodically impacted by continental aerosols, making it an excellent location to study the cloud condensation nuclei (CCN) budget in a remote marine region periodically perturbed by anthropogenic emissions, and to investigate the impacts of long-range transport of aerosols on remote marine clouds. The Aerosol and Cloud Experiments in Eastern North Atlantic (ACE-ENA) campaign was motivated by the need of comprehensive in-situ measurements for improving the understanding of marine boundary layer CCN budget, cloud and drizzle microphysics, and the impact of aerosol on marine low cloud and precipitation. The airborne deployments took place from June 21 to July 20, 2017 and January 15 to February 18, 2018 in the Azores. The flights were designed to maximize the synergy between in-situ airborne measurements and ongoing long-term observations at a ground site. Here we present measurements, observation strategy, meteorological conditions during the campaign, and preliminary findings. Finally, we discuss future analyses and modeling studies that improve the understanding and representation of marine boundary layer aerosols, clouds, precipitation, and the interactions among them. 

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3. A Characterization of Clouds and Precipitation Over the Southern Ocean From Synoptic to Micro Scales During the CAPRICORN Field Campaigns

   https://doi.org/10.1029/2022JD036796  

   Montoya Duque, E. ; Huang, Y. ; Siems, S. T. ; May, P. T. ; Protat, A. ; McFarquhar, G. M. ( September 2022 , Journal of Geophysical Research: Atmospheres)

   The persistent Southern Ocean (SO) shortwave radiation biases in climate models and reanalyses have been associated with the poor representation of clouds, precipitation, aerosols, the atmospheric boundary layer, and their intrinsic interactions. Capitalizing on shipborne observations collected during the Clouds Aerosols Precipitation Radiation and atmospheric Composition Over the Southern Ocean 2016 and 2018 field campaigns, this research investigates and characterizes cloud and precipitation processes from synoptic to micro scales. Distinct cloud and precipitation regimes are found to correspond to the seven thermodynamic clusters established using a K‐means clustering technique, while less distinctions are evident using the cyclone and (cold) front compositing methods. Cloud radar and disdrometer data reveal that light precipitation is common over the SO with higher intensities associated with cyclonic and warm frontal regions. Multiple lines of evidence suggest the presence of diverse microphysical features in several cloud regimes, including the likely dominance of ice aggregation in deep precipitating clouds. Signatures of mixed phase, and in some cases, riming were detected in shallow convective clouds away from the frontal conditions. Two of the K‐means clusters with contrasting cloud and precipitation properties are observed over the high‐latitude SO and coastal Antarctica, suggesting distinct physical processes therein. Through a single case study, in‐situ and remote‐sensing data collected by an overflight of the Southern Ocean Clouds Radiation Aerosol Transport Experimental Study were also evaluated and complement the ship‐based analysis.

    

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4. Impacts of long-range transport of aerosols on marine-boundary-layer clouds in the eastern North Atlantic

   https://doi.org/10.5194/acp-20-14741-2020  

   Wang, Yuan ; Zheng, Xiaojian ; Dong, Xiquan ; Xi, Baike ; Wu, Peng ; Logan, Timothy ; Yung, Yuk L. ( January 2020 , Atmospheric Chemistry and Physics)

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   Abstract. Vertical profiles of aerosols are inadequately observed and poorlyrepresented in climate models, contributing to the current large uncertaintyassociated with aerosol–cloud interactions. The US Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Aerosol and CloudExperiments in the Eastern North Atlantic (ACE-ENA) aircraft field campaignnear the Azores islands provided ample observations of verticaldistributions of aerosol and cloud properties. Here we utilize the in situaircraft measurements from the ACE-ENA and ground-based remote-sensing dataalong with an aerosol-aware Weather Research and Forecast (WRF) model tocharacterize the aerosols due to long-range transport over a remote regionand to assess their possible influence on marine-boundary-layer (MBL)clouds. The vertical profiles of aerosol and cloud properties measured viaaircraft during the ACE-ENA campaign provide detailed information revealingthe physical contact between transported aerosols and MBL clouds. TheEuropean Centre for Medium-Range Weather Forecasts Copernicus Atmosphere Monitoring Service (ECMWF-CAMS) aerosol reanalysis data can reproduce the key features of aerosolvertical profiles in the remote region. The cloud-resolving WRF sensitivityexperiments with distinctive aerosol profiles suggest that the transportedaerosols and MBL cloud interactions (ACIs) require not only aerosol plumes to get close to the marine-boundary-layer top but also large cloud topheight variations. Based on those criteria, the observations show that theoccurrence of ACIs involving the transport of aerosol over the eastern NorthAtlantic (ENA) is about 62 % in summer. For the case with noticeable long-range-transport aerosol effects on MBL clouds, the susceptibilities of dropleteffective radius and liquid water content are −0.11 and +0.14,respectively. When varying by a similar magnitude, aerosols originatingfrom the boundary layer exert larger microphysical influence on MBL cloudsthan those entrained from the free troposphere. 

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5. Investigation of aerosol–cloud interactions under different absorptive aerosol regimes using Atmospheric Radiation Measurement (ARM) southern Great Plains (SGP) ground-based measurements

   https://doi.org/10.5194/acp-20-3483-2020  

   Zheng, Xiaojian ; Xi, Baike ; Dong, Xiquan ; Logan, Timothy ; Wang, Yuan ; Wu, Peng ( January 2020 , Atmospheric Chemistry and Physics)

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   Abstract. The aerosol indirect effect on cloud microphysical and radiative propertiesis one of the largest uncertainties in climate simulations. In order toinvestigate the aerosol–cloud interactions, a total of 16 low-level stratuscloud cases under daytime coupled boundary-layer conditions are selectedover the southern Great Plains (SGP) region of the United States. Thephysicochemical properties of aerosols and their impacts on cloudmicrophysical properties are examined using data collected from theDepartment of Energy Atmospheric Radiation Measurement (ARM) facility at the SGP site. The aerosol–cloud interaction index (ACIr) is used to quantify the aerosol impacts with respect to cloud-droplet effective radius. The mean value of ACIr calculated from all selected samples is0.145±0.05 and ranges from 0.09 to 0.24 at a range of cloudliquid water paths (LWPs; LWP=20–300 g m−2). The magnitude of ACIr decreases with an increasing LWP, which suggests a diminished cloud microphysical response to aerosol loading, presumably due to enhanced condensational growth processes and enlarged particle sizes. The impact of aerosols with different light-absorbing abilities on the sensitivity of cloud microphysical responses is also investigated. In the presence of weak light-absorbing aerosols, the low-level clouds feature a higher number concentration of cloud condensation nuclei (NCCN) and smaller effective radii (re), while the opposite is true for strong light-absorbing aerosols. Furthermore, the mean activation ratio of aerosols to CCN (NCCN∕Na) for weakly (strongly) absorbing aerosols is 0.54 (0.45), owing to the aerosol microphysical effects, particularly the different aerosol compositions inferred by their absorptive properties. In terms of the sensitivity of cloud-droplet number concentration (Nd) to NCCN, the fraction of CCN that converted to cloud droplets (Nd∕NCCN) for the weakly (strongly) absorptive regime is 0.69 (0.54). The measured ACIr values in the weakly absorptive regime arerelatively higher, indicating that clouds have greater microphysicalresponses to aerosols, owing to the favorable thermodynamic condition. Thereduced ACIr values in the strongly absorptive regime are due to the cloud-layer heating effect induced by strong light-absorbing aerosols. Consequently, we expect larger shortwave radiative cooling effects from clouds in the weakly absorptive regime than those in the strongly absorptive regime. 

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