skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Title: Ultra-low-power second-order nonlinear optics on a chip
Abstract Second-order nonlinear optical processes convert light from one wavelength to another and generate quantum entanglement. Creating chip-scale devices to efficiently control these interactions greatly increases the reach of photonics. Existing silicon-based photonic circuits utilize the third-order optical nonlinearity, but an analogous integrated platform for second-order nonlinear optics remains an outstanding challenge. Here we demonstrate efficient frequency doubling and parametric oscillation with a threshold of tens of micro-watts in an integrated thin-film lithium niobate photonic circuit. We achieve degenerate and non-degenerate operation of the parametric oscillator at room temperature and tune its emission over one terahertz by varying the pump frequency by hundreds of megahertz. Finally, we observe cascaded second-order processes that result in parametric oscillation. These resonant second-order nonlinear circuits will form a crucial part of the emerging nonlinear and quantum photonics platforms.  more » « less
Award ID(s):
1918549
PAR ID:
10402261
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ;
Date Published:
Journal Name:
Nature Communications
Volume:
13
Issue:
1
ISSN:
2041-1723
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Silicon is a common material for photonics due to its favorable optical properties in the telecom and mid-wave IR bands, as well as compatibility with a wide range of complementary metal–oxide semiconductor (CMOS) foundry processes. Crystalline inversion symmetry precludes silicon from natively exhibiting second-order nonlinear optical processes. In this work, we build on recent works in silicon photonics that break this material symmetry using large bias fields, thereby enabling χ (2) interactions. Using this approach, we demonstrate both second-harmonic generation (with a normalized efficiency of 0.20%W −1 cm −2 ) and, to our knowledge, the first degenerate χ (2) optical parametric amplifier (with an estimated normalized gain of 0.6dBW −1/2 cm −1 ) using silicon-on-insulator waveguides fabricated in a CMOS-compatible commercial foundry. We expect this technology to enable the integration of novel nonlinear optical devices such as optical parametric amplifiers, oscillators, and frequency converters into large-scale, hybrid photonic–electronic systems by leveraging the extensive ecosystem of CMOS fabrication. 
    more » « less
  2. Optical nonlinearity plays a pivotal role in quantum information processing using photons, from heralded single-photon sources and coherent wavelength conversion to long-sought quantum repeaters. Despite the availability of strong dipole coupling to quantum emitters, achieving strong bulk optical nonlinearity is highly desirable. Here, we realize quantum nanophotonic integrated circuits in thin-film InGaP with, to our knowledge, a record-high ratio of 1.5 % between the single-photon nonlinear coupling rate ( g / 2 π = 11.2 M H z ) and cavity-photon loss rate. We demonstrate second-harmonic generation with an efficiency of 71200 ± 10300 % / W in the InGaP photonic circuit and photon-pair generation via degenerate spontaneous parametric downconversion with an ultrahigh rate exceeding 27.5 MHz/µW—an order of magnitude improvement of the state of the art—and a large coincidence-to-accidental ratio up to 1.4 × 10 4 . Our work shows InGaP as a potentially transcending platform for quantum nonlinear optics and quantum information applications. 
    more » « less
  3. By-design access to laser wavelength, especially with integrated photonics, is critical to advance quantum sensors, such as optical clocks and quantum-information systems, and open opportunities in optical communication. Semiconductor-laser gain provides exemplary efficiency and integration but merely in developed wavelength bands. Alternatively, nonlinear optics requires control of phase matching, but the principle of nonlinear conversion of a pump laser to a designed wavelength is extensible. We report on laser-wavelength access by versatile customization of optical-parametric oscillation (OPO) with a photonic-crystal ring resonator (PhCR). Leveraging the exquisite control of laser propagation provided by a photonic crystal in a traveling-wave ring resonator, we enable OPO generation across a wavelength range of 1234–2093 nm with a 1550-nm pump and 1016–1110 nm with a 1064-nm pump. Moreover, our platform offers pump-to-sideband conversion efficiency of > 10 % and negligible additive optical-frequency noise across the output range. From laser design to simulation of nonlinear dynamics, we use a Lugiato–Lefever framework that predicts the system characteristics, including bidirectional OPO generation in the PhCR and conversion efficiency in agreement with our observations. Our experiments introduce broadband lasers by design with PhCR OPOs, providing critical functionalities in integrated photonics. 
    more » « less
  4. Many uses of lasers place the highest importance on access to specific wavelength bands. For example, mobilizing optical-atomic clocks for a leap in sensing requires compact lasers at frequencies spread across the visible and near-infrared. Integrated photonics enables high-performance, scalable laser platforms. However, customizing laser-gain media to support wholly new bands is challenging and often prohibitively mismatched in scalability to early quantum-based sensing and information systems. Here, we demonstrate a tantalum pentoxide microresonator optical-parametric oscillator (OPO) that converts a pump laser to an output wave within a frequency span exceeding an octave. We control phase matching for oscillation by nanopatterning the microresonator to open a photonic-crystal bandgap on the mode of the pump laser. The photonic crystal splits only the pump mode and preserves the broader mode structure of the resonator, thus affording a single parameter to control output waves across the octave span using a nearly fixed frequency pump laser. We also demonstrate tuning the oscillator in free-spectral-range steps, more finely with temperature, and minimal additive frequency noise of the laser-conversion process. Our work shows that nanophotonic structures offer control of laser conversion in microresonators, bridging phase-matching of nonlinear optics and application requirements for laser designs. 
    more » « less
  5. Photonic integrated circuits with second-order (χ(2)) nonlinearities are rapidly scaling to remarkably low powers. At this time, state-of-the-art devices achieve saturated nonlinear interactions with thousands of photons when driven by continuous-wave lasers, and further reductions in these energy requirements enabled by the use of ultrafast pulses may soon push nonlinear optics into the realm of single-photon nonlinearities. This tutorial reviews these recent developments in ultrafast nonlinear photonics, discusses design strategies for realizing few-photon nonlinear interactions, and presents a unified treatment of ultrafast quantum nonlinear optics using a framework that smoothly interpolates from classical behaviors to the few-photon scale. These emerging platforms for quantum optics fundamentally differ from typical realizations in cavity quantum electrodynamics due to the large number of coupled optical modes. Classically, multimode behaviors have been well studied in nonlinear optics, with famous examples including soliton formation and supercontinuum generation. In contrast, multimode quantum systems exhibit a far greater variety of behaviors, and yet closed-form solutions are even sparser than their classical counterparts. In developing a framework for ultrafast quantum optics, we identify what behaviors carry over from classical to quantum devices, what intuition must be abandoned, and what new opportunities exist at the intersection of ultrafast and quantum nonlinear optics. Although this article focuses on establishing connections between the classical and quantum behaviors of devices withχ(2)nonlinearities, the frameworks developed here are general and are readily extended to the description of dynamical processes based on third-orderχ(3)nonlinearities. 
    more » « less